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Title: Nonvolatile Electric Control of the Anomalous Hall Effect in an Ultrathin Magnetic Metal

Abstract

Abstract Low‐dimensional magnetism has been boosted by the recent discovery of the ferromagnetism in layered two‐dimensional (2D) semiconductors. Although the macroscopic magnetic moments of 2D ferromagnets are weak, the anomalous Hall effect (AHE) can serve as a versatile electric probe to their magnetic properties. Here, the nonvolatile electric‐field manipulation of the AHE in an ultrathin metallic ferromagnet with perpendicular magnetic anisotropy at room temperature is reported, which is achieved by the electrostatic modulation of the longitudinal resistivity via a ferroelectric substrate without varying magnetization. Therefore, this work demonstrates an electric‐field‐controlled room‐temperature memory device based on the zero‐magnetic‐field anomalous Hall resistance of an ultrathin ferromagnet. More importantly, the experimental results disentangle magnetization and anomalous Hall resistance. As a result, the study reveals a linear decrease of anomalous Hall conductivity with normal conductivity, which is distinct from previous scaling relations. Accordingly, this work manifests a universe avenue to harnessing the AHE in low‐dimensional magnetic materials.

Authors:
 [1];  [1];  [1];  [1];  [1];  [1];  [2];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1]; ORCiD logo [1]
  1. School of Materials Science and Engineering Beihang University Beijing 100191 China
  2. Department of Materials Science and Engineering Harbin Institute of Technology Shenzhen 518055 China
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1579451
Grant/Contract Number:  
DE‐AC02‐05CH11231
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Advanced Electronic Materials
Additional Journal Information:
Journal Name: Advanced Electronic Materials Journal Volume: 6 Journal Issue: 2; Journal ID: ISSN 2199-160X
Publisher:
Wiley Blackwell (John Wiley & Sons)
Country of Publication:
United States
Language:
English

Citation Formats

Feng, Zexin, Yan, Han, Wang, Xiaoning, Guo, Huixin, Qin, Peixin, Zhou, Xiaorong, Chen, Zuhuang, Wang, Hui, Jiao, Zhengying, Leng, Zhaoguogang, Hu, Zexiang, Zhang, Xin, Wu, Haojiang, Chen, Hongyu, Wang, Jingmin, Zhang, Tianli, Jiang, Chengbao, and Liu, Zhiqi. Nonvolatile Electric Control of the Anomalous Hall Effect in an Ultrathin Magnetic Metal. United States: N. p., 2019. Web. doi:10.1002/aelm.201901084.
Feng, Zexin, Yan, Han, Wang, Xiaoning, Guo, Huixin, Qin, Peixin, Zhou, Xiaorong, Chen, Zuhuang, Wang, Hui, Jiao, Zhengying, Leng, Zhaoguogang, Hu, Zexiang, Zhang, Xin, Wu, Haojiang, Chen, Hongyu, Wang, Jingmin, Zhang, Tianli, Jiang, Chengbao, & Liu, Zhiqi. Nonvolatile Electric Control of the Anomalous Hall Effect in an Ultrathin Magnetic Metal. United States. https://doi.org/10.1002/aelm.201901084
Feng, Zexin, Yan, Han, Wang, Xiaoning, Guo, Huixin, Qin, Peixin, Zhou, Xiaorong, Chen, Zuhuang, Wang, Hui, Jiao, Zhengying, Leng, Zhaoguogang, Hu, Zexiang, Zhang, Xin, Wu, Haojiang, Chen, Hongyu, Wang, Jingmin, Zhang, Tianli, Jiang, Chengbao, and Liu, Zhiqi. Mon . "Nonvolatile Electric Control of the Anomalous Hall Effect in an Ultrathin Magnetic Metal". United States. https://doi.org/10.1002/aelm.201901084.
@article{osti_1579451,
title = {Nonvolatile Electric Control of the Anomalous Hall Effect in an Ultrathin Magnetic Metal},
author = {Feng, Zexin and Yan, Han and Wang, Xiaoning and Guo, Huixin and Qin, Peixin and Zhou, Xiaorong and Chen, Zuhuang and Wang, Hui and Jiao, Zhengying and Leng, Zhaoguogang and Hu, Zexiang and Zhang, Xin and Wu, Haojiang and Chen, Hongyu and Wang, Jingmin and Zhang, Tianli and Jiang, Chengbao and Liu, Zhiqi},
abstractNote = {Abstract Low‐dimensional magnetism has been boosted by the recent discovery of the ferromagnetism in layered two‐dimensional (2D) semiconductors. Although the macroscopic magnetic moments of 2D ferromagnets are weak, the anomalous Hall effect (AHE) can serve as a versatile electric probe to their magnetic properties. Here, the nonvolatile electric‐field manipulation of the AHE in an ultrathin metallic ferromagnet with perpendicular magnetic anisotropy at room temperature is reported, which is achieved by the electrostatic modulation of the longitudinal resistivity via a ferroelectric substrate without varying magnetization. Therefore, this work demonstrates an electric‐field‐controlled room‐temperature memory device based on the zero‐magnetic‐field anomalous Hall resistance of an ultrathin ferromagnet. More importantly, the experimental results disentangle magnetization and anomalous Hall resistance. As a result, the study reveals a linear decrease of anomalous Hall conductivity with normal conductivity, which is distinct from previous scaling relations. Accordingly, this work manifests a universe avenue to harnessing the AHE in low‐dimensional magnetic materials.},
doi = {10.1002/aelm.201901084},
journal = {Advanced Electronic Materials},
number = 2,
volume = 6,
place = {United States},
year = {Mon Dec 16 00:00:00 EST 2019},
month = {Mon Dec 16 00:00:00 EST 2019}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1002/aelm.201901084

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Cited by: 8 works
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Works referenced in this record:

Discovery of intrinsic ferromagnetism in two-dimensional van der Waals crystals
journal, April 2017


Crossover Behavior of the Anomalous Hall Effect and Anomalous Nernst Effect in Itinerant Ferromagnets
journal, August 2007


Gate-tunable room-temperature ferromagnetism in two-dimensional Fe3GeTe2
journal, October 2018


Voltage control of magnetism in multiferroic heterostructures
journal, February 2014

  • Liu, Ming; Sun, Nian X.
  • Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 372, Issue 2009
  • DOI: 10.1098/rsta.2012.0439

Epitaxial Growth of Intermetallic MnPt Films on Oxides and Large Exchange Bias
journal, November 2015

  • Liu, Zhiqi; Biegalski, Michael D.; Hsu, Shang-Lin
  • Advanced Materials, Vol. 28, Issue 1
  • DOI: 10.1002/adma.201502606

Nonlinear anomalous Hall effect in few-layer WTe2
journal, February 2019


Two-dimensional itinerant ferromagnetism in atomically thin Fe3GeTe2
journal, August 2018


Electrically reversible cracks in an intermetallic film controlled by an electric field
journal, January 2018


Dominant role of oxygen vacancies in electrical properties of unannealed LaAlO 3 /SrTiO 3 interfaces
journal, February 2014

  • Liu, Z. Q.; Sun, L.; Huang, Z.
  • Journal of Applied Physics, Vol. 115, Issue 5
  • DOI: 10.1063/1.4863800

Observation of the nonlinear Hall effect under time-reversal-symmetric conditions
journal, December 2018


Perpendicular magnetic anisotropy in Pd/Co and Pt/Co thin‐film layered structures
journal, May 1988

  • Carcia, P. F.
  • Journal of Applied Physics, Vol. 63, Issue 10
  • DOI: 10.1063/1.340404

Electrical switching of the topological anomalous Hall effect in a non-collinear antiferromagnet above room temperature
journal, March 2018


Multiferroic materials and magnetoelectric physics: symmetry, entanglement, excitation, and topology
journal, November 2015


Summary Abstract: Perpendicular magnetic anisotropy in Co/Pd and Co/Pt superlattices
journal, July 1987

  • Carcia, Peter F.
  • Journal of Vacuum Science & Technology A: Vacuum, Surfaces, and Films, Vol. 5, Issue 4
  • DOI: 10.1116/1.574896

Electric-Field Control of Magnetic Order: From FeRh to Topological Antiferromagnetic Spintronics
journal, November 2018

  • Feng, Zexin; Yan, Han; Liu, Zhiqi
  • Advanced Electronic Materials, Vol. 5, Issue 1
  • DOI: 10.1002/aelm.201800466

Proper Scaling of the Anomalous Hall Effect
journal, August 2009


Anomalous Hall effect in Fe (001) epitaxial thin films over a wide range in conductivity
journal, January 2009


Electric Control of the Hall effect in Pt/Bi0.9La0.1FeO3 bilayers
journal, February 2016

  • Gao, Rongli; Fu, Chunlin; Cai, Wei
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep20330

Metal-Insulator Transition in SrTiO 3 x Thin Films Induced by Frozen-Out Carriers
journal, September 2011


A piezoelectric, strain-controlled antiferromagnetic memory insensitive to magnetic fields
journal, January 2019


Electrically Tunable Anomalous Hall Effect in Pt Thin Films
journal, November 2013


Recent Progress in Multiferroic Magnetoelectric Composites: from Bulk to Thin Films
journal, February 2011


Antiferromagnetic Piezospintronics
journal, April 2019

  • Liu, Zhiqi; Feng, Zexin; Yan, Han
  • Advanced Electronic Materials, Vol. 5, Issue 7
  • DOI: 10.1002/aelm.201900176

Layer-dependent ferromagnetism in a van der Waals crystal down to the monolayer limit
journal, June 2017

  • Huang, Bevin; Clark, Genevieve; Navarro-Moratalla, Efrén
  • Nature, Vol. 546, Issue 7657
  • DOI: 10.1038/nature22391

Domain engineered switchable strain states in ferroelectric (011) [Pb(Mg 1/3 Nb 2/3 )O 3 ] (1−x) -[PbTiO 3 ] x (PMN-PT, x≈0.32) single crystals
journal, June 2011

  • Zhao, Ping; Bao, Mingqiang; Bur, Alexandre
  • Journal of Applied Physics, Vol. 109, Issue 12
  • DOI: 10.1063/1.3595670

Reversible electrical-field control of magnetization and anomalous Hall effect in Co/PMN-PT hybrid heterostructures
journal, April 2018

  • Wang, J.; Huang, Q. K.; Lu, S. Y.
  • Applied Physics Letters, Vol. 112, Issue 15
  • DOI: 10.1063/1.5022381

Anisotropic magnetotransport at the SrTiO3/LaAlO3 interface
journal, October 2009


Magnetism in two-dimensional van der Waals materials
journal, October 2018


Electric-field control of anomalous and topological Hall effects in oxide bilayer thin films
journal, January 2018


Large resistivity modulation in mixed-phase metallic systems
journal, January 2015

  • Lee, Yeonbae; Liu, Z. Q.; Heron, J. T.
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms6959

Electron Accumulation and Emergent Magnetism in LaMnO 3 / SrTiO 3 Heterostructures
journal, October 2017


Full Electroresistance Modulation in a Mixed-Phase Metallic Alloy
journal, March 2016


Multiferroic magnetoelectric composites: Historical perspective, status, and future directions
journal, February 2008

  • Nan, Ce-Wen; Bichurin, M. I.; Dong, Shuxiang
  • Journal of Applied Physics, Vol. 103, Issue 3
  • DOI: 10.1063/1.2836410

Integration of the noncollinear antiferromagnetic metal Mn3Sn onto ferroelectric oxides for electric-field control
journal, December 2019


Spin Torque Study of the Spin Hall Conductivity and Spin Diffusion Length in Platinum Thin Films with Varying Resistivity
journal, March 2016


Anomalous Hall effect
journal, May 2010


Electrically tuneable nonlinear anomalous Hall effect in two-dimensional transition-metal dichalcogenides WTe 2 and MoTe 2
journal, July 2018