Imaging stress and magnetism at high pressures using a nanoscale quantum sensor
Abstract
Pressure alters the physical, chemical, and electronic properties of matter. The diamond anvil cell enables tabletop experiments to investigate a diverse landscape of high-pressure phenomena. In this work, we introduce and use a nanoscale sensing platform that integrates nitrogen-vacancy (NV) color centers directly into the culet of diamond anvils. We demonstrate the versatility of this platform by performing diffraction-limited imaging of both stress fields and magnetism as a function of pressure and temperature. We quantify all normal and shear stress components and demonstrate vector magnetic field imaging, enabling measurement of the pressure-driven phase transition in iron and the complex pressure-temperature phase diagram of gadolinium. A complementary NV-sensing modality using noise spectroscopy enables the characterization of phase transitions even in the absence of static magnetic signatures.
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Center for Novel Pathways to Quantum Coherence in Materials (NPQC); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States); Univ. of California, San Diego, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC); USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1579407
- Alternate Identifier(s):
- OSTI ID: 1591844; OSTI ID: 1633878
- Grant/Contract Number:
- AC02-05CH11231; NA0003842
- Resource Type:
- Published Article
- Journal Name:
- Science
- Additional Journal Information:
- Journal Name: Science Journal Volume: 366 Journal Issue: 6471; Journal ID: ISSN 0036-8075
- Publisher:
- AAAS
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Hsieh, S., Bhattacharyya, P., Zu, C., Mittiga, T., Smart, T. J., Machado, F., Kobrin, B., Höhn, T. O., Rui, N. Z., Kamrani, M., Chatterjee, S., Choi, S., Zaletel, M., Struzhkin, V. V., Moore, J. E., Levitas, V. I., Jeanloz, R., and Yao, N. Y. Imaging stress and magnetism at high pressures using a nanoscale quantum sensor. United States: N. p., 2019.
Web. doi:10.1126/science.aaw4352.
Hsieh, S., Bhattacharyya, P., Zu, C., Mittiga, T., Smart, T. J., Machado, F., Kobrin, B., Höhn, T. O., Rui, N. Z., Kamrani, M., Chatterjee, S., Choi, S., Zaletel, M., Struzhkin, V. V., Moore, J. E., Levitas, V. I., Jeanloz, R., & Yao, N. Y. Imaging stress and magnetism at high pressures using a nanoscale quantum sensor. United States. https://doi.org/10.1126/science.aaw4352
Hsieh, S., Bhattacharyya, P., Zu, C., Mittiga, T., Smart, T. J., Machado, F., Kobrin, B., Höhn, T. O., Rui, N. Z., Kamrani, M., Chatterjee, S., Choi, S., Zaletel, M., Struzhkin, V. V., Moore, J. E., Levitas, V. I., Jeanloz, R., and Yao, N. Y. Thu .
"Imaging stress and magnetism at high pressures using a nanoscale quantum sensor". United States. https://doi.org/10.1126/science.aaw4352.
@article{osti_1579407,
title = {Imaging stress and magnetism at high pressures using a nanoscale quantum sensor},
author = {Hsieh, S. and Bhattacharyya, P. and Zu, C. and Mittiga, T. and Smart, T. J. and Machado, F. and Kobrin, B. and Höhn, T. O. and Rui, N. Z. and Kamrani, M. and Chatterjee, S. and Choi, S. and Zaletel, M. and Struzhkin, V. V. and Moore, J. E. and Levitas, V. I. and Jeanloz, R. and Yao, N. Y.},
abstractNote = {Pressure alters the physical, chemical, and electronic properties of matter. The diamond anvil cell enables tabletop experiments to investigate a diverse landscape of high-pressure phenomena. In this work, we introduce and use a nanoscale sensing platform that integrates nitrogen-vacancy (NV) color centers directly into the culet of diamond anvils. We demonstrate the versatility of this platform by performing diffraction-limited imaging of both stress fields and magnetism as a function of pressure and temperature. We quantify all normal and shear stress components and demonstrate vector magnetic field imaging, enabling measurement of the pressure-driven α↔ϵ phase transition in iron and the complex pressure-temperature phase diagram of gadolinium. A complementary NV-sensing modality using noise spectroscopy enables the characterization of phase transitions even in the absence of static magnetic signatures.},
doi = {10.1126/science.aaw4352},
journal = {Science},
number = 6471,
volume = 366,
place = {United States},
year = {Thu Dec 12 00:00:00 EST 2019},
month = {Thu Dec 12 00:00:00 EST 2019}
}
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https://doi.org/10.1126/science.aaw4352
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