Thermal Expansion and Magnetostriction of Laves-Phase Alloys: Fingerprints of Ferrimagnetic Phase Transitions

Zhou, Chao; Bao, Huixin; Matsushita, Yoshitaka; Chang, Tieyan; Chen, Kaiyun; Zhang, Yin; Tian, Fanghua; Zuo, Wenliang; Song, Xiaoping; Yang, Sen; Ren, Yang; Ren, Xiaobing

doi:10.3390/ma12111755

Title: Thermal Expansion and Magnetostriction of Laves-Phase Alloys: Fingerprints of Ferrimagnetic Phase Transitions

Abstract

The magneto–elastic coupling effect correlates to the changes of moment and lattice upon magnetic phase transition. Here, we report that, in the pseudo-binary Laves-phase Tb_1-xDy_xCo₂ system (x = 0.0, 0.7, and 1.0), thermal expansion and magnetostriction can probe the ferrimagnetic transitions from cubic to rhombohedral phase (in TbCo₂), from cubic to tetragonal phase (in DyCo₂), and from cubic to rhombohedral then to tetragonal phase (in Tb_0.3Dy_0.7Co₂). Furthermore, a Landau polynomial approach is employed to qualitatively investigate the thermal expansion upon the paramagnetic (cubic) to ferrimagnetic (rhombohedral or tetragonal) transition, and the calculated thermal expansion curves agree with the experimental curves. Our work illustrates the correlation between crystal symmetry, magnetostriction, and thermal expansion in ferrimagnetic Laves-phase alloys and provides a new perspective to investigate ferrimagnetic transitions.

Authors:

Zhou, Chao ^[1]; Bao, Huixin ^[1];

^[2]; Chang, Tieyan ^[1]; Chen, Kaiyun ^[3]; Zhang, Yin ^[1]; Tian, Fanghua ^[1]; Zuo, Wenliang ^[1]; Song, Xiaoping ^[1]; Yang, Sen ^[1]; Ren, Yang ^[4]; Ren, Xiaobing ^[5]

Xi’an Jiaotong Univ. (China)
National Inst. for Materials Science (NIMS), Hyogo (Japan)
Univ. of Melbourne (Australia)
Argonne National Lab. (ANL), Argonne, IL (United States)
National Inst. for Materials Science (NIMS), Tsukuba (Japan)

Publication Date:: Thu May 30 00:00:00 EDT 2019

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; National Natural Science Foundation of China (NSFC)

OSTI Identifier:: 1578039

Grant/Contract Number:: AC02-06CH11357

Resource Type:: Accepted Manuscript

Journal Name:: Materials

Additional Journal Information:: Journal Volume: 12; Journal Issue: 11; Journal ID: ISSN 1996-1944

Publisher:: MDPI

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; Laves-phase alloy; ferrimagnetic transition; magnetostriction; thermal expansion

Citation Formats


                    Zhou, Chao, Bao, Huixin, Matsushita, Yoshitaka, Chang, Tieyan, Chen, Kaiyun, Zhang, Yin, Tian, Fanghua, Zuo, Wenliang, Song, Xiaoping, Yang, Sen, Ren, Yang, and Ren, Xiaobing. Thermal Expansion and Magnetostriction of Laves-Phase Alloys: Fingerprints of Ferrimagnetic Phase Transitions.  United States: N. p., 2019. 
Web.  doi:10.3390/ma12111755.

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                    Zhou, Chao, Bao, Huixin, Matsushita, Yoshitaka, Chang, Tieyan, Chen, Kaiyun, Zhang, Yin, Tian, Fanghua, Zuo, Wenliang, Song, Xiaoping, Yang, Sen, Ren, Yang, & Ren, Xiaobing. Thermal Expansion and Magnetostriction of Laves-Phase Alloys: Fingerprints of Ferrimagnetic Phase Transitions.  United States.  https://doi.org/10.3390/ma12111755

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                    Zhou, Chao, Bao, Huixin, Matsushita, Yoshitaka, Chang, Tieyan, Chen, Kaiyun, Zhang, Yin, Tian, Fanghua, Zuo, Wenliang, Song, Xiaoping, Yang, Sen, Ren, Yang, and Ren, Xiaobing. Thu .  
"Thermal Expansion and Magnetostriction of Laves-Phase Alloys: Fingerprints of Ferrimagnetic Phase Transitions".  United States.  https://doi.org/10.3390/ma12111755.  https://www.osti.gov/servlets/purl/1578039.

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@article{osti_1578039,

  title        = {Thermal Expansion and Magnetostriction of Laves-Phase Alloys: Fingerprints of Ferrimagnetic Phase Transitions},

  author       = {Zhou, Chao and Bao, Huixin and Matsushita, Yoshitaka and Chang, Tieyan and Chen, Kaiyun and Zhang, Yin and Tian, Fanghua and Zuo, Wenliang and Song, Xiaoping and Yang, Sen and Ren, Yang and Ren, Xiaobing},

  abstractNote = {The magneto–elastic coupling effect correlates to the changes of moment and lattice upon magnetic phase transition. Here, we report that, in the pseudo-binary Laves-phase Tb1-xDyxCo2 system (x = 0.0, 0.7, and 1.0), thermal expansion and magnetostriction can probe the ferrimagnetic transitions from cubic to rhombohedral phase (in TbCo2), from cubic to tetragonal phase (in DyCo2), and from cubic to rhombohedral then to tetragonal phase (in Tb0.3Dy0.7Co2). Furthermore, a Landau polynomial approach is employed to qualitatively investigate the thermal expansion upon the paramagnetic (cubic) to ferrimagnetic (rhombohedral or tetragonal) transition, and the calculated thermal expansion curves agree with the experimental curves. Our work illustrates the correlation between crystal symmetry, magnetostriction, and thermal expansion in ferrimagnetic Laves-phase alloys and provides a new perspective to investigate ferrimagnetic transitions.},

  doi          = {10.3390/ma12111755},

  journal      = {Materials},

  number       = 11,

  volume       = 12,

  place        = {United States},

  year         = {Thu May 30 00:00:00 EDT 2019},

  month        = {Thu May 30 00:00:00 EDT 2019}

}

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Magnetostriction of some cubic rare earth-Co ₂ compounds in high magnetic fields
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Magnetostriction Curves of Polycrystalline Ferromagnetics
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Title: Thermal Expansion and Magnetostriction of Laves-Phase Alloys: Fingerprints of Ferrimagnetic Phase Transitions

Abstract

Citation Formats

Magnetostriction and Magnetomechanical Effects journal, January 1955

Magnetostriction Curves of Polycrystalline Ferromagnetics journal, August 1958

Magnetostriction of some cubic rare earth-Co 2 compounds in high magnetic fields journal, September 1975

Rhombohedral distortion in highly magnetostrictive Laves phase compounds conference, January 1976

Magnetoelastic properties of (Rare-Earth)–Co2 compounds. II. The anisotropic magnetostriction journal, March 1976

Magnetoelastic properties of (rare-earth)Co2 compounds. I. Exchange-striction journal, February 1976

Magnetostriction and structural distortion in rare-earth intermetallics journal, May 1977

Magnetic properties and spontaneous distortion in TbCo 2 journal, May 1979

The magnetic behaviour of rare-earth—transition metal compounds journal, February 1992

Magnetic phase transitions and magnetovolume anomalies in DyCo2 and GdMn2 compounds under pressure journal, February 1995

A structural phase transition induced by an external magnetic field journal, February 1995

Ferromagnetic shape memory in the NiMnGa system journal, January 1999

Noncubic crystallographic symmetry of a cubic ferromagnet: Simultaneous structural change at the ferromagnetic transition journal, January 2008

Large Magnetostriction from Morphotropic Phase Boundary in Ferromagnets journal, May 2010

Morphotropic Phase Boundaries in Ferromagnets: Tb 1 − x Dy x Fe 2 Alloys journal, July 2013

Inverse effect of morphotropic phase boundary on the magnetostriction of ferromagnetic Tb 1 − x Gd x Co 2 journal, March 2014

Interaction Between the d Shells in the Transition Metals journal, February 1951

Magnetic and Magnetomechanical Properties of CoAl$_{\rm x}$Fe$_{2 - {\rm x}}$O$_{4}$for Stress Sensor and Actuator Applications journal, October 2009

Effect of temperature variation on the magnetostrictive properties of CoAlxFe2−xO4 journal, May 2010

Coupled magnetoelastic theory of magnetic and magnetostrictive hysteresis journal, July 1993

Permalloy, an alloy of remarkable magnetic properties journal, May 1923

Magnetostriction in Permalloy journal, July 1926

Physical Theory of Ferromagnetic Domains journal, October 1949

Strain-induced metal–insulator phase coexistence in perovskite manganites journal, March 2004

Physical metallurgy of Ti–Ni-based shape memory alloys journal, July 2005

Physical Theory of Ferromagnetic Domains journal, August 1950

The magnetic behaviour of rare-earth—transition metal compounds journal, February 1992

Physical metallurgy of Ti–Ni-based shape memory alloys journal, July 2005

Effect of temperature variation on the magnetostrictive properties of CoAlxFe2−xO4 journal, May 2010

Magnetostriction and Magnetomechanical Effects journal, January 1955

Magnetostriction of some cubic rare earth-Co 2 compounds in high magnetic fields journal, September 1975

Magnetostriction Curves of Polycrystalline Ferromagnetics journal, August 1958

Interaction between the d -Shells in the Transition Metals. II. Ferromagnetic Compounds of Manganese with Perovskite Structure journal, May 1951

Spontaneous Volume Magnetostriction of RCo 2 Compounds journal, October 1976

Magnetostriction and Magnetomechanical Effects
journal, January 1955

Magnetostriction Curves of Polycrystalline Ferromagnetics
journal, August 1958

Magnetostriction of some cubic rare earth-Co ₂ compounds in high magnetic fields
journal, September 1975

Rhombohedral distortion in highly magnetostrictive Laves phase compounds
conference, January 1976

Magnetoelastic properties of (Rare-Earth)–Co2 compounds. II. The anisotropic magnetostriction
journal, March 1976

Magnetoelastic properties of (rare-earth)Co2 compounds. I. Exchange-striction
journal, February 1976

Magnetostriction and structural distortion in rare-earth intermetallics
journal, May 1977

Magnetic properties and spontaneous distortion in TbCo ₂
journal, May 1979

The magnetic behaviour of rare-earth—transition metal compounds
journal, February 1992

Magnetic phase transitions and magnetovolume anomalies in DyCo2 and GdMn2 compounds under pressure
journal, February 1995

A structural phase transition induced by an external magnetic field
journal, February 1995

Ferromagnetic shape memory in the NiMnGa system
journal, January 1999

Noncubic crystallographic symmetry of a cubic ferromagnet: Simultaneous structural change at the ferromagnetic transition
journal, January 2008

Large Magnetostriction from Morphotropic Phase Boundary in Ferromagnets
journal, May 2010

Morphotropic Phase Boundaries in Ferromagnets: ${Tb}_{1 - x} {Dy}_{x} {Fe}_{2}$ Alloys
journal, July 2013

Inverse effect of morphotropic phase boundary on the magnetostriction of ferromagnetic Tb $_{1 - x}$ Gd $_{x}$ Co $_{2}$
journal, March 2014

Interaction Between the $d$ Shells in the Transition Metals
journal, February 1951

Magnetic and Magnetomechanical Properties of CoAl$_{\rm x}$Fe$_{2 - {\rm x}}$O$_{4}$for Stress Sensor and Actuator Applications
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Effect of temperature variation on the magnetostrictive properties of CoAlxFe2−xO4
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Coupled magnetoelastic theory of magnetic and magnetostrictive hysteresis
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Permalloy, an alloy of remarkable magnetic properties
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Magnetostriction in Permalloy
journal, July 1926

Physical Theory of Ferromagnetic Domains
journal, October 1949

Strain-induced metal–insulator phase coexistence in perovskite manganites
journal, March 2004

Physical metallurgy of Ti–Ni-based shape memory alloys
journal, July 2005

Physical Theory of Ferromagnetic Domains
journal, August 1950

The magnetic behaviour of rare-earth—transition metal compounds
journal, February 1992

Physical metallurgy of Ti–Ni-based shape memory alloys
journal, July 2005

Effect of temperature variation on the magnetostrictive properties of CoAlxFe2−xO4
journal, May 2010

Magnetostriction and Magnetomechanical Effects
journal, January 1955

Magnetostriction of some cubic rare earth-Co ₂ compounds in high magnetic fields
journal, September 1975

Magnetostriction Curves of Polycrystalline Ferromagnetics
journal, August 1958

Interaction between the $d$ -Shells in the Transition Metals. II. Ferromagnetic Compounds of Manganese with Perovskite Structure
journal, May 1951

Spontaneous Volume Magnetostriction of RCo ₂ Compounds
journal, October 1976