Nonmetallic metal toward a pressure-induced bad-metal state in two-dimensional Cu 3 LiRu 2 O 6

Huang, Bin; Liu, Ziyi; Han, Yifeng; Zhao, Shuang; Wu, Meixia; Frank, Corey E.; Greenblatt, Martha; Croft, Mark; Quackenbush, Nicholas F.; Liu, Sizhan; Tyson, Trevor A.; Zhang, Lei; Sun, Junliang; Shan, Pengfei; Dai, Jianhong; Yu, Xiaohui; Cheng, Jinguang; Li, Man-Rong

doi:10.1039/C9CC06691H

Title: Nonmetallic metal toward a pressure-induced bad-metal state in two-dimensional Cu ₃ LiRu ₂ O ₆

Abstract

The two-dimensional honeycomb layered nonmetallic metal Cu ₃ LiRu ₂ O ₆ exhibits Pauli-like paramagnetic and Mott variable range hopping semiconduction behaviors, which can be significantly suppressed toward a bad-metal state by pressure up to 35 GPa.

Authors:

Huang, Bin ^[1]; Liu, Ziyi ^[2]; Han, Yifeng ^[1]; Zhao, Shuang ^[1]; Wu, Meixia ^[1];

^[3];

^[3]; Croft, Mark ^[4]; Quackenbush, Nicholas F. ^[5]; Liu, Sizhan ^[6]; Tyson, Trevor A. ^[6]; Zhang, Lei ^[7];

^[7]; Shan, Pengfei ^[8]; Dai, Jianhong ^[2]; Yu, Xiaohui ^[8];

^[8];

^[1]

Key Laboratory of Bioinorganic and Synthetic Chemistry of Ministry of Education, School of Chemistry, Sun Yat-Sen University, Guangzhou 510275, P. R. China
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, P. R. China
Department of Chemistry and Chemical Biology, Rutgers, The State University of New Jersey, Piscataway, USA
Department of Physics and Astronomy, Rutgers, The State University of New Jersey, Piscataway, USA
Materials Measurement Science Division, Material Measurement Laboratory, National Institute of Standards and Technology, Gaithersburg, USA
Department of Physics, New Jersey Institute of Technology, Newark, USA
College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, P. R. China
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, P. R. China, School of Physical Sciences

Publication Date:: 2020-01-01

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1577379

Grant/Contract Number:: SC0012704

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: ChemComm

Additional Journal Information:: Journal Name: ChemComm Journal Volume: 56 Journal Issue: 2; Journal ID: ISSN 1359-7345

Publisher:: Royal Society of Chemistry (RSC)

Country of Publication:: United Kingdom

Language:: English

Citation Formats


                    Huang, Bin, Liu, Ziyi, Han, Yifeng, Zhao, Shuang, Wu, Meixia, Frank, Corey E., Greenblatt, Martha, Croft, Mark, Quackenbush, Nicholas F., Liu, Sizhan, Tyson, Trevor A., Zhang, Lei, Sun, Junliang, Shan, Pengfei, Dai, Jianhong, Yu, Xiaohui, Cheng, Jinguang, and Li, Man-Rong. Nonmetallic metal toward a pressure-induced bad-metal state in two-dimensional Cu 3 LiRu 2 O 6.  United Kingdom: N. p., 2020. 
        Web.  doi:10.1039/C9CC06691H.

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                    Huang, Bin, Liu, Ziyi, Han, Yifeng, Zhao, Shuang, Wu, Meixia, Frank, Corey E., Greenblatt, Martha, Croft, Mark, Quackenbush, Nicholas F., Liu, Sizhan, Tyson, Trevor A., Zhang, Lei, Sun, Junliang, Shan, Pengfei, Dai, Jianhong, Yu, Xiaohui, Cheng, Jinguang, & Li, Man-Rong. Nonmetallic metal toward a pressure-induced bad-metal state in two-dimensional Cu 3 LiRu 2 O 6.  United Kingdom.  doi:https://doi.org/10.1039/C9CC06691H

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                    Huang, Bin, Liu, Ziyi, Han, Yifeng, Zhao, Shuang, Wu, Meixia, Frank, Corey E., Greenblatt, Martha, Croft, Mark, Quackenbush, Nicholas F., Liu, Sizhan, Tyson, Trevor A., Zhang, Lei, Sun, Junliang, Shan, Pengfei, Dai, Jianhong, Yu, Xiaohui, Cheng, Jinguang, and Li, Man-Rong. Wed .  
        "Nonmetallic metal toward a pressure-induced bad-metal state in two-dimensional Cu 3 LiRu 2 O 6".  United Kingdom.  doi:https://doi.org/10.1039/C9CC06691H.

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@article{osti_1577379,

  title        = {Nonmetallic metal toward a pressure-induced bad-metal state in two-dimensional Cu 3 LiRu 2 O 6},

  author       = {Huang, Bin and Liu, Ziyi and Han, Yifeng and Zhao, Shuang and Wu, Meixia and Frank, Corey E. and Greenblatt, Martha and Croft, Mark and Quackenbush, Nicholas F. and Liu, Sizhan and Tyson, Trevor A. and Zhang, Lei and Sun, Junliang and Shan, Pengfei and Dai, Jianhong and Yu, Xiaohui and Cheng, Jinguang and Li, Man-Rong},

  abstractNote = {The two-dimensional honeycomb layered nonmetallic metal Cu 3 LiRu 2 O 6 exhibits Pauli-like paramagnetic and Mott variable range hopping semiconduction behaviors, which can be significantly suppressed toward a bad-metal state by pressure up to 35 GPa.},

  doi          = {10.1039/C9CC06691H},

  journal      = {ChemComm},

  number       = 2,

  volume       = 56,

  place        = {United Kingdom},

  year         = {2020},

  month        = {1}

}

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DOI: https://doi.org/10.1039/C9CC06691H

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Title: Nonmetallic metal toward a pressure-induced bad-metal state in two-dimensional Cu 3 LiRu 2 O 6

Abstract

Citation Formats

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Zigzag Magnetic Order in the Iridium Oxide Na 2 IrO 3 journal, February 2013

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Cu 2 IrO 3 : A New Magnetically Frustrated Honeycomb Iridate journal, October 2017

New-Type Phase Transition of Li 2 RuO 3 with Honeycomb Structure journal, March 2007

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Title: Nonmetallic metal toward a pressure-induced bad-metal state in two-dimensional Cu ₃ LiRu ₂ O ₆

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Interlayer tuning of electronic and magnetic properties in honeycomb ordered Ag3LiRu2O6
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X-ray diffraction line broadening: modeling and applications to high-Tc superconductors
journal, May 1993

Structure and bonding in lithium ruthenate, Li2RuO3
journal, June 1988

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journal, July 1993

Iridium containing honeycomb Delafossites by topotactic cation exchange
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journal, February 2018

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journal, March 2014

On AgRhO2, and the new quaternary delafossites AgLi1/3M2/3O2, syntheses and analyses of real structures
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P-type electrical conduction in transparent thin films of CuAlO2
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