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Title: Attosecond transient absorption spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy

Journal Article · · Physical Chemistry Chemical Physics. PCCP
DOI: https://doi.org/10.1039/C9CP03951A · OSTI ID:1576833
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  1. Stanford PULSE Institute, SLAC National Accelerator Laboratory, USA, SLAC National Accelerator Laboratory, USA
  2. SLAC National Accelerator Laboratory, USA, Department of Physics, Stanford University, USA
  3. Stanford PULSE Institute, SLAC National Accelerator Laboratory, USA
  4. SLAC National Accelerator Laboratory, USA
  5. Stanford PULSE Institute, SLAC National Accelerator Laboratory, USA, Max-Planck-Institut für Quantenoptik, Germany
  6. Paul Scherrer Institut, Switzerland
  7. The Blackett Laboratory, Department of Physics, Imperial College London, UK
  8. Physics Department, University of Connecticut, USA
  9. Paul Scherrer Institut, Switzerland, LUXS Laboratory for Ultrafast X-ray Sciences, École Polytechnique Fédérale de Lausanne, Switzerland
  10. Stanford PULSE Institute, SLAC National Accelerator Laboratory, USA, Department of Physics, Stanford University
  11. Department of Physics, The Ohio State University, USA
  12. Institut für Physik und CINSaT, Universität Kassel, Germany, Helmholtz-Zentrum Berlin, Germany
  13. KLA Tencor Corporation, USA
  14. Zentrum für Synchrotronstrahlung, Technische Universität Dortmund, Germany
  15. Stanford PULSE Institute, SLAC National Accelerator Laboratory, USA, Department of Applied Physics, Stanford University

Recently demonstrated isolated attosecond XFEL pulses should allow the probing of ultrafast electron dynamics at X-ray wavelengths. The authors use ghost imaging to enable high-resolution transient absorption spectroscopy at fluctuating XFEL sources.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Grant/Contract Number:
AC02-76SF00515; FG02-04ER15614; SC0012376
OSTI ID:
1576833
Journal Information:
Physical Chemistry Chemical Physics. PCCP, Journal Name: Physical Chemistry Chemical Physics. PCCP; ISSN 1463-9076; ISSN PPCPFQ
Publisher:
Royal Society of ChemistryCopyright Statement
Country of Publication:
United Kingdom
Language:
English

References (40)

Electron Correlation in Real Time journal December 2011
K- and L-edge X-ray absorption spectroscopy (XAS) and resonant inelastic X-ray scattering (RIXS) determination of differential orbital covalency (DOC) of transition metal sites journal August 2017
Probing ultrafast dynamics with attosecond transient absorption journal March 2015
Attosecond Electron Dynamics in Molecules journal May 2017
Ultrafast X-ray Absorption Spectroscopy journal April 2004
Time-resolved atomic inner-shell spectroscopy journal October 2002
Ghost imaging with atoms journal November 2016
The generation, characterization and applications of broadband isolated attosecond pulses journal February 2014
Attosecond molecular dynamics: fact or fiction? journal February 2014
What will it take to observe processes in 'real time'? journal February 2014
Infrared spectroscopy with visible light journal January 2016
Ghost imaging in the time domain journal February 2016
Probing ultrafast ππ*/nπ* internal conversion in organic chromophores via K-edge resonant absorption journal June 2017
Tunable isolated attosecond X-ray pulses with gigawatt peak power from a free-electron laser journal December 2019
A perspective for investigating photo-induced molecular dynamics from within with femtosecond free electron lasers journal January 2017
Remote spectral measurement using entangled photons journal December 2003
High‐resolution and symmetry‐resolved N and O K ‐edge absorption spectra of NO journal December 1992
A co-axial velocity map imaging spectrometer for electrons journal November 2018
Transient absorption spectroscopy using high harmonic generation: a review of ultrafast X-ray dynamics in molecules and solids
  • Geneaux, Romain; Marroux, Hugo J. B.; Guggenmos, Alexander
  • Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2145 https://doi.org/10.1098/rsta.2017.0463
journal April 2019
Development of ultrafast capabilities for X-ray free-electron lasers at the linac coherent light source
  • Coffee, Ryan N.; Cryan, James P.; Duris, Joseph
  • Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2145 https://doi.org/10.1098/rsta.2018.0386
journal April 2019
Ghost imaging with paired x-ray photons journal June 2018
Ghost Spectroscopy with Classical Thermal Light Emitted by a Superluminescent Diode journal February 2018
Attosecond Time-Resolved Autoionization of Argon journal October 2010
Fourier-Transform Ghost Imaging with Hard X Rays journal September 2016
Experimental X-Ray Ghost Imaging journal September 2016
Electron Ghost Imaging journal September 2018
Attosecond physics journal February 2009
The physics of x-ray free-electron lasers journal March 2016
Single-pixel imaging via compressive sampling journal March 2008
Attosecond Control and Measurement: Lightwave Electronics journal August 2007
Ultrafast electron dynamics in phenylalanine initiated by attosecond pulses journal October 2014
Time-resolved x-ray absorption spectroscopy with a water window high-harmonic source journal January 2017
Femtosecond x-ray spectroscopy of an electrocyclic ring-opening reaction journal April 2017
Real-Time Probing of Electron Dynamics Using Attosecond Time-Resolved Spectroscopy journal May 2016
Ghost imaging: from quantum to classical to computational journal January 2010
X-ray ghost imaging with a laboratory source journal January 2017
X-ray computational ghost imaging with single-pixel detector journal January 2019
Supercontinuum spectral-domain ghost imaging journal January 2018
Tabletop x-ray ghost imaging with ultra-low radiation journal January 2018
Distributed Optimization and Statistical Learning via the Alternating Direction Method of Multipliers book January 2011