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Title: Schalten in Metall‐organischen Gerüsten

Abstract

Abstract Aufgrund ihrer einstellbaren Poren und nahezu grenzenlosen Strukturdiversität, die sich aus dem Design verschiedener organischer Linker und metallischer Strukturbaueinheiten ableitet, haben sich Metall‐organische Gerüste (MOFs) in den vergangenen Jahren zu einem intensiv beforschten Gebiet entwickelt. Zu den größten Aufgaben gehören schaltbare MOFs und ihre Anwendung. Schaltbare MOFs sind “intelligente” Materialien, die bei Exposition gegenüber externen Stimuli eine deutliche, reversible, chemische Veränderung ihrer Struktur durchlaufen, was interessante technische Anwendungen ermöglicht. Obwohl dieser Prozess des Schaltens Ähnlichkeiten mit Flexibilität aufweist, haben sich nur sehr wenige Studien speziell mit Schalten beschäftigt, wohingegen sich eine recht große Zahl von Arbeiten und Übersichten mit der Flexibilität in MOFs beschäftigt. Dieser Aufsatz konzentriert sich auf die Eigenschaften und das allgemeine Design schaltbarer MOFs. Dabei wird die Schaltaktivität basierend auf der Ursache des Schaltens beschrieben: Licht, Spincrossover, Redoxchemie, Temperatur und Benetzbarkeit.

Authors:
 [1]; ORCiD logo [2];  [1]; ORCiD logo [3]
  1. Department of Chemistry Faculty of Sciences Tarbiat Modares University P.O. Box 14155-4838 Teheran Iran
  2. Department of Chemistry Texas A&,M University College Station TX 77843 USA
  3. Department of Chemistry Texas A&,M University College Station TX 77843 USA, Department of Materials Science and Engineering Texas A&,M University College Station TX 77843 USA
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1576806
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Angewandte Chemie
Additional Journal Information:
Journal Name: Angewandte Chemie Journal Volume: 132 Journal Issue: 12; Journal ID: ISSN 0044-8249
Publisher:
Wiley Blackwell (John Wiley & Sons)
Country of Publication:
Germany
Language:
English

Citation Formats

Bigdeli, Fahime, Lollar, Christina T., Morsali, Ali, and Zhou, Hong‐Cai. Schalten in Metall‐organischen Gerüsten. Germany: N. p., 2019. Web. doi:10.1002/ange.201900666.
Bigdeli, Fahime, Lollar, Christina T., Morsali, Ali, & Zhou, Hong‐Cai. Schalten in Metall‐organischen Gerüsten. Germany. https://doi.org/10.1002/ange.201900666
Bigdeli, Fahime, Lollar, Christina T., Morsali, Ali, and Zhou, Hong‐Cai. Mon . "Schalten in Metall‐organischen Gerüsten". Germany. https://doi.org/10.1002/ange.201900666.
@article{osti_1576806,
title = {Schalten in Metall‐organischen Gerüsten},
author = {Bigdeli, Fahime and Lollar, Christina T. and Morsali, Ali and Zhou, Hong‐Cai},
abstractNote = {Abstract Aufgrund ihrer einstellbaren Poren und nahezu grenzenlosen Strukturdiversität, die sich aus dem Design verschiedener organischer Linker und metallischer Strukturbaueinheiten ableitet, haben sich Metall‐organische Gerüste (MOFs) in den vergangenen Jahren zu einem intensiv beforschten Gebiet entwickelt. Zu den größten Aufgaben gehören schaltbare MOFs und ihre Anwendung. Schaltbare MOFs sind “intelligente” Materialien, die bei Exposition gegenüber externen Stimuli eine deutliche, reversible, chemische Veränderung ihrer Struktur durchlaufen, was interessante technische Anwendungen ermöglicht. Obwohl dieser Prozess des Schaltens Ähnlichkeiten mit Flexibilität aufweist, haben sich nur sehr wenige Studien speziell mit Schalten beschäftigt, wohingegen sich eine recht große Zahl von Arbeiten und Übersichten mit der Flexibilität in MOFs beschäftigt. Dieser Aufsatz konzentriert sich auf die Eigenschaften und das allgemeine Design schaltbarer MOFs. Dabei wird die Schaltaktivität basierend auf der Ursache des Schaltens beschrieben: Licht, Spincrossover, Redoxchemie, Temperatur und Benetzbarkeit.},
doi = {10.1002/ange.201900666},
journal = {Angewandte Chemie},
number = 12,
volume = 132,
place = {Germany},
year = {2019},
month = {12}
}

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