The sensitivity of Cu for electrochemical carbon dioxide reduction to hydrocarbons as revealed by high throughput experiments

doi:10.1039/C9TA10111J

Title: The sensitivity of Cu for electrochemical carbon dioxide reduction to hydrocarbons as revealed by high throughput experiments

Abstract

Electrochemical CO₂ reduction to valuable products is a centerpiece of future energy technologies that relies on identification of new catalysts. Here, we present accelerated screening of Cu bimetallic alloys, revealing remarkable sensitivity to alloy concentration that indicates the migration of alloying elements to critical sites for hydrocarbon formation.

Authors:

^[1];

^[2]

California Institute of Technology (CalTech), Pasadena, CA (United States). Joint Center for Artificial Photosynthesis (JCAP)
California Institute of Technology (CalTech), Pasadena, CA (United States). Joint Center for Artificial Photosynthesis (JCAP), and Division of Engineering and Applied Science

Publication Date:: 2019-11-14

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1575099

Grant/Contract Number:: SC0004993

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Journal of Materials Chemistry. A

Additional Journal Information:: Journal Name: Journal of Materials Chemistry. A Journal Volume: 7 Journal Issue: 47; Journal ID: ISSN 2050-7488

Publisher:: Royal Society of Chemistry

Country of Publication:: United Kingdom

Language:: English

Citation Formats


                    Lai, Yungchieh, Jones, Ryan J. R., Wang, Yu, Zhou, Lan, Richter, Matthias H., and Gregoire, John. The sensitivity of Cu for electrochemical carbon dioxide reduction to hydrocarbons as revealed by high throughput experiments.  United Kingdom: N. p., 2019. 
        Web.  doi:10.1039/C9TA10111J.

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                    Lai, Yungchieh, Jones, Ryan J. R., Wang, Yu, Zhou, Lan, Richter, Matthias H., & Gregoire, John. The sensitivity of Cu for electrochemical carbon dioxide reduction to hydrocarbons as revealed by high throughput experiments.  United Kingdom.  doi:10.1039/C9TA10111J.

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                    Lai, Yungchieh, Jones, Ryan J. R., Wang, Yu, Zhou, Lan, Richter, Matthias H., and Gregoire, John. Thu .  
        "The sensitivity of Cu for electrochemical carbon dioxide reduction to hydrocarbons as revealed by high throughput experiments".  United Kingdom.  doi:10.1039/C9TA10111J.

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@article{osti_1575099,

  title        = {The sensitivity of Cu for electrochemical carbon dioxide reduction to hydrocarbons as revealed by high throughput experiments},

  author       = {Lai, Yungchieh and Jones, Ryan J. R. and Wang, Yu and Zhou, Lan and Richter, Matthias H. and Gregoire, John},

  abstractNote = {Electrochemical CO2 reduction to valuable products is a centerpiece of future energy technologies that relies on identification of new catalysts. Here, we present accelerated screening of Cu bimetallic alloys, revealing remarkable sensitivity to alloy concentration that indicates the migration of alloying elements to critical sites for hydrocarbon formation.},

  doi          = {10.1039/C9TA10111J},

  journal      = {Journal of Materials Chemistry. A},

  number       = 47,

  volume       = 7,

  place        = {United Kingdom},

  year         = {2019},

  month        = {11}

}

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DOI: 10.1039/C9TA10111J

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Title: The sensitivity of Cu for electrochemical carbon dioxide reduction to hydrocarbons as revealed by high throughput experiments

Abstract

Citation Formats

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