skip to main content
DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

This content will become publicly available on November 14, 2020

Title: Nature and impact of stripe freezing in La 1.67 Sr 0.33 NiO 4

Abstract

La 1.67Sr 0.33NiO 4 develops charge and spin stripe orders at temperatures of roughly 200 K, with modulation wave vectors that are temperature independent. Here, various probes of spin and charge response have provided independent evidence for some sort of change below ~50 K. In combination with a new set of neutron scattering measurements, we propose a unified interpretation of all of these observations in terms of a freezing of Ni-centered charges stripes, together with a glassy ordering of the spin stripes that shows up in neutron scattering as a slight rotation of the average spin direction.

Authors:
 [1];  [1];  [2];  [3]; ORCiD logo [3]
  1. Univ. of Colorado at Boulder, Boulder, CO (United States). Dept. of Physics
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Neutron Scattering Div.
  3. Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics & Materials Science Dept.
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1574920
Report Number(s):
BNL-212349-2019-JAAM
Journal ID: ISSN 2469-9950; PRBMDO
Grant/Contract Number:  
SC0012704
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 100; Journal Issue: 19; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Merritt, A. M., Reznik, D., Garlea, V. O., Gu, G. D., and Tranquada, John M. Nature and impact of stripe freezing in La1.67Sr0.33NiO4. United States: N. p., 2019. Web. doi:10.1103/PhysRevB.100.195122.
Merritt, A. M., Reznik, D., Garlea, V. O., Gu, G. D., & Tranquada, John M. Nature and impact of stripe freezing in La1.67Sr0.33NiO4. United States. doi:10.1103/PhysRevB.100.195122.
Merritt, A. M., Reznik, D., Garlea, V. O., Gu, G. D., and Tranquada, John M. Thu . "Nature and impact of stripe freezing in La1.67Sr0.33NiO4". United States. doi:10.1103/PhysRevB.100.195122.
@article{osti_1574920,
title = {Nature and impact of stripe freezing in La1.67Sr0.33NiO4},
author = {Merritt, A. M. and Reznik, D. and Garlea, V. O. and Gu, G. D. and Tranquada, John M.},
abstractNote = {La1.67Sr0.33NiO4 develops charge and spin stripe orders at temperatures of roughly 200 K, with modulation wave vectors that are temperature independent. Here, various probes of spin and charge response have provided independent evidence for some sort of change below ~50 K. In combination with a new set of neutron scattering measurements, we propose a unified interpretation of all of these observations in terms of a freezing of Ni-centered charges stripes, together with a glassy ordering of the spin stripes that shows up in neutron scattering as a slight rotation of the average spin direction.},
doi = {10.1103/PhysRevB.100.195122},
journal = {Physical Review B},
number = 19,
volume = 100,
place = {United States},
year = {2019},
month = {11}
}

Journal Article:
Free Publicly Available Full Text
This content will become publicly available on November 14, 2020
Publisher's Version of Record

Save / Share:

Works referenced in this record:

Neutron scattering studies on stripe phases in non-cuprate materials
journal, November 2012


Charge-ordered states in (La,Sr ) 2 NiO 4 for hole concentrations n h =1/3 and 1/2
journal, March 1994


Charge Modulation in L a 1.67 S r 0.33 Ni O 4 : A Bulk Thermodynamic Study
journal, January 1996


Melting of Quasi-Two-Dimensional Charge Stripes in La 5 / 3 Sr 1 / 3 NiO 4
journal, September 1997


Stripe order at low temperatures in La 2 x Sr x NiO 4 with 0.289 x 0.5
journal, January 2000


Critical Fluctuations and Quenched Disordered Two-Dimensional Charge Stripes in La 5 / 3 Sr 1 / 3 NiO 4
journal, April 2000


Optical spectroscopy of the charge-ordering transition in La 1.67 Sr 0.33 NiO 4
journal, November 1996


Spin Correlations among the Charge Carriers in an Ordered Stripe Phase
journal, December 2003


Weak ferromagnetic spin and charge stripe order in La 5 3 Sr 1 3 Ni O 4
journal, September 2005


Freezing of a Stripe Liquid
journal, March 2002


High-Energy Spin Dynamics in L a 1.69 S r 0.31 N i O 4
journal, April 2003


Charge and canted spin order in La 2 x Sr x NiO 4 ( x = 0.275 and 1 3 )
journal, January 2001


Field-induced staggered magnetic order in La 2 NiO 4.133
journal, March 1997


Neutron-diffraction study of stripe order in La 2 NiO 4 + δ with δ = 2 15
journal, January 1998


Isotropic O 1s prepeak as evidence for polarons in La2NiO4 + δ
journal, March 1995


O 1 s near-edge x-ray absorption of La 2 x Sr x NiO 4 + δ : Holes, polarons, and excitons
journal, April 1996


Spectroscopy of Stripe Order in La 1.8 Sr 0.2 NiO 4 Using Resonant Soft X-Ray Diffraction
journal, October 2005


Magnetism of Stripe-Ordered La 5 / 3 Sr 1 / 3 NiO 4
journal, April 1999


Charge order, dielectric response, and local structure of La5/3Sr1/3NiO4 system
journal, November 2009

  • Filippi, M.; Kundys, B.; Agrestini, S.
  • Journal of Applied Physics, Vol. 106, Issue 10
  • DOI: 10.1063/1.3260222

Similarity of Slow Stripe Fluctuations between Sr-Doped Cuprates and Oxygen-Doped Nickelates
journal, October 1999


Recent progress on HYSPEC, and its polarization analysis capabilities
journal, January 2015


Direct observation of dynamic charge stripes in La2–xSrxNiO4
journal, March 2014

  • Anissimova, S.; Parshall, D.; Gu, G. D.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4467

DAVE: A Comprehensive Software Suite for the Reduction, Visualization, and Analysis of Low Energy Neutron Spectroscopic Data
journal, November 2009

  • Azuah, Richard Tumanjong; Kneller, Larry R.; Qiu, Yiming
  • Journal of Research of the National Institute of Standards and Technology, Vol. 114, Issue 6
  • DOI: 10.6028/jres.114.025

Mantid—Data analysis and visualization package for neutron scattering and μ SR experiments
journal, November 2014

  • Arnold, O.; Bilheux, J. C.; Borreguero, J. M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 764
  • DOI: 10.1016/j.nima.2014.07.029

Horace : Software for the analysis of data from single crystal spectroscopy experiments at time-of-flight neutron instruments
journal, October 2016

  • Ewings, R. A.; Buts, A.; Le, M. D.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 834
  • DOI: 10.1016/j.nima.2016.07.036

Cooperative ordering of holes and spins in La 2 NiO 4.125
journal, August 1995


Evidence for a Nematic Phase in La 1.75 Sr 0.25 NiO 4
journal, April 2017


Spin dynamics in stripe-ordered La 5 / 3 Sr 1 / 3 NiO 4
journal, March 2003


Mapping spin-wave dispersions in stripe-ordered La 2 x Sr x Ni O 4 ( x = 0.275 , 0.333)
journal, August 2005


Incommensurate stripe order in La 2 x Sr x NiO 4 with x =0.225
journal, November 1996


Neutron-diffraction study of the antiferromagnetic form factor of La 2 NiO 4
journal, March 1992


Freezing electronic correlations by polaronic instabilities in doped La 2 NiO 4
journal, September 1994


Orbital Ordering, New Phases, and Stripe Formation in Doped Layered Nickelates
journal, June 2004


Microscopic origin of diagonal stripe phases in doped nickelates
journal, March 2006


Electronic structure of charge and spin stripe order in La 2 x Sr x Ni O 4 ( x = 1 3 , 1 2 )
journal, October 2007


Magnetic ordering in the striped nickelate La 5/3 Sr 1/3 NiO 4 : A band structure point of view
journal, December 2007


First Time Determination of the Microscopic Structure of a Stripe Phase: Low Temperature NMR in La 2 NiO 4.17
journal, November 2001


The geometric order of stripes and Luttinger liquids
journal, October 2001


Magnetization of La 2 x Sr x Ni O 4 + δ ( 0 x 0.5 ) : Spin-glass and memory effects
journal, January 2006