This content will become publicly available on July 9, 2020
Interfacial Octahedral Manipulation Imparts Hysteresis-Free Metal to Insulator Transition in Ultrathin Nickelate Heterostructure
Abstract
Much like epitaxial strain, engineering oxygen octahedral rotations (OORs) in perovskite oxide thin films can be a powerful means of manipulating their physical and chemical properties. Here, it is demonstrated that the fundamental character of the metal-insulator transition (MIT) can be sensitively controlled by the structure of the oxygen sublattice for NdNiO 3 thin films grown epitaxially on NdGaO 3 (110) substrates. The MIT is sharp and hysteretic for a Ni-O-Ni bond angle of 154.0° (6 nm thick film) like the bulk behavior, while it is diffuse and largely nonhysteretic for a bond angle of 149.5° (3 nm thick film), stemming from the smaller bond angle of the NdGaO 3 substrate. Using synchrotron X-ray diffraction to quantify the geometric framework of the oxygen sublattice, it is found that the influence of the substrate OORs propagates and decays after a few nanometers into the ultrathin film. The sublattice structure in the 6 nm thick film is similar to that for bulk NdNiO 3, leading to the sharp and hysteretic MIT.
- Authors:
-
[3];
- Univ. of Science and Technology of China, Hefei (China). National Synchrotron Radiation Lab.; Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
- Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)
- Univ. of Science and Technology of China, Hefei (China). National Synchrotron Radiation Lab.
- Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
- Chinese Academy of Sciences (CAS), Hefei (China). High Magnetic Field Lab.
- Univ. of Science and Technology of China, Hefei (China). National Synchrotron Radiation Lab.; Chinese Academy of Sciences (CAS), Beijing (China). Beijing Advanced Sciences and Innovation Center
- Publication Date:
- Research Org.:
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- National Key Research and Development Program of China; National Natural Science Foundation of China (NNSFC); China Scholarship Council; USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division
- OSTI Identifier:
- 1574391
- Alternate Identifier(s):
- OSTI ID: 1532581
- Grant/Contract Number:
- [AC02-06CH11357]
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials Interfaces
- Additional Journal Information:
- [ Journal Volume: 6; Journal Issue: 17]; Journal ID: ISSN 2196-7350
- Publisher:
- Wiley-VCH
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; NdNiO3 oxide heterostructure; half-order Bragg reflection; oxygen octahedral tilting and rotation; synchrotron X-ray techniques
Citation Formats
Dong, Yongqi, Ma, Zhiyuan, Luo, Zhenlin, Zhou, Hua, Fong, Dillon D., Wu, Wenbin, and Gao, Chen. Interfacial Octahedral Manipulation Imparts Hysteresis-Free Metal to Insulator Transition in Ultrathin Nickelate Heterostructure. United States: N. p., 2019.
Web. doi:10.1002/admi.201900644.
Dong, Yongqi, Ma, Zhiyuan, Luo, Zhenlin, Zhou, Hua, Fong, Dillon D., Wu, Wenbin, & Gao, Chen. Interfacial Octahedral Manipulation Imparts Hysteresis-Free Metal to Insulator Transition in Ultrathin Nickelate Heterostructure. United States. doi:10.1002/admi.201900644.
Dong, Yongqi, Ma, Zhiyuan, Luo, Zhenlin, Zhou, Hua, Fong, Dillon D., Wu, Wenbin, and Gao, Chen. Tue .
"Interfacial Octahedral Manipulation Imparts Hysteresis-Free Metal to Insulator Transition in Ultrathin Nickelate Heterostructure". United States. doi:10.1002/admi.201900644.
@article{osti_1574391,
title = {Interfacial Octahedral Manipulation Imparts Hysteresis-Free Metal to Insulator Transition in Ultrathin Nickelate Heterostructure},
author = {Dong, Yongqi and Ma, Zhiyuan and Luo, Zhenlin and Zhou, Hua and Fong, Dillon D. and Wu, Wenbin and Gao, Chen},
abstractNote = {Much like epitaxial strain, engineering oxygen octahedral rotations (OORs) in perovskite oxide thin films can be a powerful means of manipulating their physical and chemical properties. Here, it is demonstrated that the fundamental character of the metal-insulator transition (MIT) can be sensitively controlled by the structure of the oxygen sublattice for NdNiO3 thin films grown epitaxially on NdGaO3 (110) substrates. The MIT is sharp and hysteretic for a Ni-O-Ni bond angle of 154.0° (6 nm thick film) like the bulk behavior, while it is diffuse and largely nonhysteretic for a bond angle of 149.5° (3 nm thick film), stemming from the smaller bond angle of the NdGaO3 substrate. Using synchrotron X-ray diffraction to quantify the geometric framework of the oxygen sublattice, it is found that the influence of the substrate OORs propagates and decays after a few nanometers into the ultrathin film. The sublattice structure in the 6 nm thick film is similar to that for bulk NdNiO3, leading to the sharp and hysteretic MIT.},
doi = {10.1002/admi.201900644},
journal = {Advanced Materials Interfaces},
number = [17],
volume = [6],
place = {United States},
year = {2019},
month = {7}
}
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Works referencing / citing this record:
Surface X-ray diffraction
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Heterointerface engineered electronic and magnetic phases of NdNiO3 thin films
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Thickness-Dependent Structure-Property Relationships in Strained (110) SrRuO 3 Thin Films
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La 2/3 Sr 1/3 VO 3 Thin Films: A New p-Type Transparent Conducting Oxide with Very High Figure of Merit
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Stable metal–insulator transition in epitaxial SmNiO3 thin films
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Structural refinement of Pbnm -type perovskite films from analysis of half-order diffraction peaks
journal, January 2017
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The photoemission study of NdNiO3/NdGaO3 thin films, through the metal–insulator transition
journal, February 2009
- Galicka, K.; Szade, J.; Ruello, P.
- Applied Surface Science, Vol. 255, Issue 8
Anisotropic-strain-controlled metal-insulator transition in epitaxial NdNiO 3 films grown on orthorhombic NdGaO 3 substrates
journal, October 2013
- Lian, X. K.; Chen, F.; Tan, X. L.
- Applied Physics Letters, Vol. 103, Issue 17
Transport properties of NdNiO3 thin films made by pulsed-laser deposition
journal, January 2000
- Catalan, G.; Bowman, R. M.; Gregg, J. M.
- Journal of Applied Physics, Vol. 87, Issue 1
Effect of gate voltage polarity on the ionic liquid gating behavior of NdNiO 3 /NdGaO 3 heterostructures
journal, May 2017
- Dong, Yongqi; Xu, Haoran; Luo, Zhenlin
- APL Materials, Vol. 5, Issue 5
Physics of Ultrathin Films and Heterostructures of Rare-Earth Nickelates
journal, July 2016
- Middey, S.; Chakhalian, J.; Mahadevan, P.
- Annual Review of Materials Research, Vol. 46, Issue 1
Strongly correlated perovskite fuel cells
journal, May 2016
- Zhou, You; Guan, Xiaofei; Zhou, Hua
- Nature, Vol. 534, Issue 7606
Oxygen Vacancy Induced Room-Temperature Metal–Insulator Transition in Nickelate Films and Its Potential Application in Photovoltaics
journal, April 2016
- Wang, Le; Dash, Sibashisa; Chang, Lei
- ACS Applied Materials & Interfaces, Vol. 8, Issue 15
Study of the phase transitions in
journal, January 1999
- Pérez-Cacho, J.; Blasco, J.; García, J.
- Journal of Physics: Condensed Matter, Vol. 11, Issue 2
Evidence of strain induced structural change in hetero-epitaxial NdNiO 3 thin films with metal-insulator transition
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Electric-Field Control of the Metal-Insulator Transition in Ultrathin NdNiO3 Films
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Structural, magnetic and electronic properties of perovskites (R = rare earth)
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- Medarde, María Luisa
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Structure and photoemission spectroscopy of strain-controlled metal-insulator transition in NdNiO3 thin films
journal, March 2009
- Eguchi, R.; Okamoto, Y.; Hiroi, Z.
- Journal of Applied Physics, Vol. 105, Issue 5
Control of Structural Distortions in Transition-Metal Oxide Films through Oxygen Displacement at the Heterointerface
journal, April 2014
- Aso, Ryotaro; Kan, Daisuke; Shimakawa, Yuichi
- Advanced Functional Materials, Vol. 24, Issue 33
Strain Engineering of Octahedral Rotations and Physical Properties of SrRuO3 Films
journal, May 2015
- Lu, Wenlai; Song, Wendong; Yang, Ping
- Scientific Reports, Vol. 5, Issue 1
X-ray diffraction from rough, relaxed and reconstructed surfaces
journal, March 1989
- Vlieg, E.; Van Der Veen, J. F.; Gurman, S. J.
- Surface Science, Vol. 210, Issue 3
Dimensionality Controlled Octahedral Symmetry-Mismatch and Functionalities in Epitaxial LaCoO 3 /SrTiO 3 Heterostructures
journal, June 2015
- Qiao, Liang; Jang, Jae Hyuck; Singh, David J.
- Nano Letters, Vol. 15, Issue 7
Tuning bad metal and non-Fermi liquid behavior in a Mott material: Rare-earth nickelate thin films
journal, November 2015
- Mikheev, Evgeny; Hauser, Adam J.; Himmetoglu, Burak
- Science Advances, Vol. 1, Issue 10
Comprehensive studies of interfacial strain and oxygen vacancy on metal–insulator transition of VO 2 film
journal, May 2016
- Fan, L. L.; Chen, S.; Liao, G. M.
- Journal of Physics: Condensed Matter, Vol. 28, Issue 25
Improving of the Thermoelectric Efficiency of LaCoO 3 by Double Substitution with Nickel and Iron
journal, June 2012
- Vulchev, V.; Vassilev, L.; Harizanova, S.
- The Journal of Physical Chemistry C, Vol. 116, Issue 25
Key role of lattice symmetry in the metal-insulator transition of NdNiO3 films
journal, April 2016
- Zhang, Jack Y.; Kim, Honggyu; Mikheev, Evgeny
- Scientific Reports, Vol. 6, Issue 1
Progress in perovskite nickelate research
journal, July 2008
- Catalan, G.
- Phase Transitions, Vol. 81, Issue 7-8
Polarity compensation in ultra-thin films of complex oxides: The case of a perovskite nickelate
journal, October 2014
- Middey, S.; Rivero, P.; Meyers, D.
- Scientific Reports, Vol. 4, Issue 1