Jenseits von Ladungsausgleich: Gegenkationen in der Polyoxometallat‐Chemie
Abstract
Abstract Polyoxometallate (POMs) sind molekulare Metalloxidanionen, die Anwendung in Energiewandlung und ‐speicherung, biomolekularer Chemie sowie Materialdesign und ‐integration finden. Das Wechselspiel von intrinsisch anionischen POMs mit organischen oder anorganischen Gegenionen wird häufig übersehen, ist jedoch essenziell, um die Aggregation, Stabilisierung, Löslichkeit und Funktion von POMs zu verstehen. Jenseits von einfachen Alkalimetall‐ oder Ammoniumkationen können neuartige Anwendungen durch vielseitige Kationen wie Dendrimere, mehrwertige Metallkationen, Metallkomplexe, Amphiphile oder Alkaloidkationen erzielt werden. Dieser Aufsatz gibt einen Überblick über grundlegende POM‐Kation‐Wechselwirkungen in Lösung, die daraus resultierenden Festkörperstrukturen und bespricht neuartige Reaktivitäten und Eigenschaften, die aus diesen Wechselwrkungen resultieren. Wir untersuchen, wie anwendungsnahe Forschung das Kation‐kontrollierte Design neuartiger POM‐Materialien ermöglicht hat, was wiederum den Wunsch nach der Aufklärung der Grundlagen von POM‐Kation‐Wechselwirkungen angeregt hat.
- Authors:
-
[1];
[2]
- Anorganische Chemie I Universtität Ulm Albert-Einstein-Allee 11 89081 Ulm Deutschland
- Department of Chemistry Oregon State University Corvallis OR 97331 USA
- Publication Date:
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1580769
- Alternate Identifier(s):
- OSTI ID: 1572577
- Grant/Contract Number:
- DE SC0010802
- Resource Type:
- Published Article
- Journal Name:
- Angewandte Chemie
- Additional Journal Information:
- Journal Name: Angewandte Chemie Journal Volume: 132 Journal Issue: 2; Journal ID: ISSN 0044-8249
- Publisher:
- Wiley Blackwell (John Wiley & Sons)
- Country of Publication:
- Germany
- Language:
- English
Citation Formats
Misra, Archismita, Kozma, Karoly, Streb, Carsten, and Nyman, May. Jenseits von Ladungsausgleich: Gegenkationen in der Polyoxometallat‐Chemie. Germany: N. p., 2019.
Web. doi:10.1002/ange.201905600.
Misra, Archismita, Kozma, Karoly, Streb, Carsten, & Nyman, May. Jenseits von Ladungsausgleich: Gegenkationen in der Polyoxometallat‐Chemie. Germany. https://doi.org/10.1002/ange.201905600
Misra, Archismita, Kozma, Karoly, Streb, Carsten, and Nyman, May. Thu .
"Jenseits von Ladungsausgleich: Gegenkationen in der Polyoxometallat‐Chemie". Germany. https://doi.org/10.1002/ange.201905600.
@article{osti_1580769,
title = {Jenseits von Ladungsausgleich: Gegenkationen in der Polyoxometallat‐Chemie},
author = {Misra, Archismita and Kozma, Karoly and Streb, Carsten and Nyman, May},
abstractNote = {Abstract Polyoxometallate (POMs) sind molekulare Metalloxidanionen, die Anwendung in Energiewandlung und ‐speicherung, biomolekularer Chemie sowie Materialdesign und ‐integration finden. Das Wechselspiel von intrinsisch anionischen POMs mit organischen oder anorganischen Gegenionen wird häufig übersehen, ist jedoch essenziell, um die Aggregation, Stabilisierung, Löslichkeit und Funktion von POMs zu verstehen. Jenseits von einfachen Alkalimetall‐ oder Ammoniumkationen können neuartige Anwendungen durch vielseitige Kationen wie Dendrimere, mehrwertige Metallkationen, Metallkomplexe, Amphiphile oder Alkaloidkationen erzielt werden. Dieser Aufsatz gibt einen Überblick über grundlegende POM‐Kation‐Wechselwirkungen in Lösung, die daraus resultierenden Festkörperstrukturen und bespricht neuartige Reaktivitäten und Eigenschaften, die aus diesen Wechselwrkungen resultieren. Wir untersuchen, wie anwendungsnahe Forschung das Kation‐kontrollierte Design neuartiger POM‐Materialien ermöglicht hat, was wiederum den Wunsch nach der Aufklärung der Grundlagen von POM‐Kation‐Wechselwirkungen angeregt hat.},
doi = {10.1002/ange.201905600},
journal = {Angewandte Chemie},
number = 2,
volume = 132,
place = {Germany},
year = {Thu Oct 31 00:00:00 EDT 2019},
month = {Thu Oct 31 00:00:00 EDT 2019}
}
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