Modulation versus Templating: Fine‐Tuning of Hierarchally Porous PCN‐250 Using Fatty Acids To Engineer Guest Adsorption

Kirchon, Angelo; Li, Jialuo; Xia, Fangqing; Day, Gregory S.; Becker, Benjamin; Chen, Wenmiao; Sue, Hung‐Jue; Fang, Yu; Zhou, Hong‐Cai

doi:10.1002/anie.201905006

Title: Modulation versus Templating: Fine‐Tuning of Hierarchally Porous PCN‐250 Using Fatty Acids To Engineer Guest Adsorption

Authors:

Kirchon, Angelo ^[1]; Li, Jialuo ^[1]; Xia, Fangqing ^[2]; Day, Gregory S. ^[1]; Becker, Benjamin ^[1]; Chen, Wenmiao ^[1]; Sue, Hung‐Jue ^[2]; Fang, Yu ^[1];

^[1]

Department of Chemistry Texas A&,M University College Station TX 77843-3255 USA
Department of Materials Science and Engineering Texas A&,M University College Station TX 77843-3255 USA

Publication Date:: 2019-09-02

Sponsoring Org.:: USDOE

OSTI Identifier:: 1572120

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Angewandte Chemie (International Edition)

Additional Journal Information:: Journal Name: Angewandte Chemie (International Edition) Journal Volume: 58 Journal Issue: 36; Journal ID: ISSN 1433-7851

Publisher:: Wiley Blackwell (John Wiley & Sons)

Country of Publication:: Germany

Language:: English

Citation Formats


                    Kirchon, Angelo, Li, Jialuo, Xia, Fangqing, Day, Gregory S., Becker, Benjamin, Chen, Wenmiao, Sue, Hung‐Jue, Fang, Yu, and Zhou, Hong‐Cai. Modulation versus Templating: Fine‐Tuning of Hierarchally Porous PCN‐250 Using Fatty Acids To Engineer Guest Adsorption.  Germany: N. p., 2019. 
Web.  doi:10.1002/anie.201905006.

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                    Kirchon, Angelo, Li, Jialuo, Xia, Fangqing, Day, Gregory S., Becker, Benjamin, Chen, Wenmiao, Sue, Hung‐Jue, Fang, Yu, & Zhou, Hong‐Cai. Modulation versus Templating: Fine‐Tuning of Hierarchally Porous PCN‐250 Using Fatty Acids To Engineer Guest Adsorption.  Germany.  https://doi.org/10.1002/anie.201905006

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                    Kirchon, Angelo, Li, Jialuo, Xia, Fangqing, Day, Gregory S., Becker, Benjamin, Chen, Wenmiao, Sue, Hung‐Jue, Fang, Yu, and Zhou, Hong‐Cai. Mon .  
"Modulation versus Templating: Fine‐Tuning of Hierarchally Porous PCN‐250 Using Fatty Acids To Engineer Guest Adsorption".  Germany.  https://doi.org/10.1002/anie.201905006.

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@article{osti_1572120,

  title        = {Modulation versus Templating: Fine‐Tuning of Hierarchally Porous PCN‐250 Using Fatty Acids To Engineer Guest Adsorption},

  author       = {Kirchon, Angelo and Li, Jialuo and Xia, Fangqing and Day, Gregory S. and Becker, Benjamin and Chen, Wenmiao and Sue, Hung‐Jue and Fang, Yu and Zhou, Hong‐Cai},

  abstractNote = {},

  doi          = {10.1002/anie.201905006},

  journal      = {Angewandte Chemie (International Edition)},

  number       = 36,

  volume       = 58,

  place        = {Germany},

  year         = {2019},

  month        = {9}

}

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Title: Modulation versus Templating: Fine‐Tuning of Hierarchally Porous PCN‐250 Using Fatty Acids To Engineer Guest Adsorption

Citation Formats

Physisorption of gases, with special reference to the evaluation of surface area and pore size distribution (IUPAC Technical Report) journal, October 2015

Amino acid assisted templating synthesis of hierarchical zeolitic imidazolate framework-8 for efficient arsenate removal journal, January 2014

A Kinetic Study of the Growth of Fatty Acid Vesicles journal, August 2004

Nanoscale metal–organic frameworks for drug delivery: a conventional platform with new promise journal, January 2018

Ultrafast room-temperature synthesis of hierarchically porous metal–organic frameworks by a versatile cooperative template strategy journal, August 2018

Gas storage in porous metal–organic frameworks for clean energy applications journal, January 2010

Creating Hierarchical Pores by Controlled Linker Thermolysis in Multivariate Metal–Organic Frameworks journal, January 2018

Hierarchically structured metal–organic frameworks assembled by hydroxy double salt–template synergy with high space–time yields journal, January 2018

Aqueous-Phase Synthesis of Mesoporous Zr-Based MOFs Templated by Amphoteric Surfactants journal, February 2018

A Modulator-Induced Defect-Formation Strategy to Hierarchically Porous Metal-Organic Frameworks with High Stability journal, December 2016

Micelle Formation and the Hydrophobic Effect † journal, May 2004

Metal–organic frameworks for energy storage: Batteries and supercapacitors journal, January 2016

Implicit-Solvent Models for Micellization: Nonionic Surfactants and Temperature-Dependent Properties journal, February 2011

Solvophobic Interactions and Micelle Formation in Structure Forming Nonaqueous Solvents journal, June 1971

Aqueous-Phase Synthesis of Mesoporous Zr-Based MOFs Templated by Amphoteric Surfactants journal, February 2018

Kinetically tuned dimensional augmentation as a versatile synthetic route towards robust metal–organic frameworks journal, December 2014

Characterization of micro- and mesoporous solids by physisorption methods and pore-size analysis journal, November 1998

PCN-250 under Pressure: Sequential Phase Transformation and the Implications for MOF Densification journal, December 2017

Effect of temperature on micelle formation in aqueous solutions of alkyltrimethylammonium bromides journal, April 1989

A comparison of micelle formation of ionic surfactants in formamide, in N-methylformamide and in N,N-dimethylformamide journal, June 2003

Pore size determination in modified micro- and mesoporous materials. Pitfalls and limitations in gas adsorption data analysis journal, June 2003

A Modulator-Induced Defect-Formation Strategy to Hierarchically Porous Metal-Organic Frameworks with High Stability journal, December 2016

Template-directed synthesis of metal–organic materials journal, January 2014

Hierarchically mesostructured MIL-101 metal–organic frameworks: supramolecular template-directed synthesis and accelerated adsorption kinetics for dye removal journal, January 2012

Introduction to Metal–Organic Frameworks journal, September 2011

Template synthesis of hierarchical porous metal–organic frameworks with tunable porosity journal, January 2017

Effect of Benzoic Acid as a Modulator in the Structure of UiO-66: An Experimental and Computational Study journal, April 2017

Construction of hierarchically porous metal–organic frameworks through linker labilization journal, May 2017

Applications of hierarchically structured porous materials from energy storage and conversion, catalysis, photocatalysis, adsorption, separation, and sensing to biomedicine journal, January 2016

Determination of pore size and pore size distribution journal, November 1994

Modulator Effects on the Water-Based Synthesis of Zr/Hf Metal–Organic Frameworks: Quantitative Relationship Studies between Modulator, Synthetic Condition, and Performance journal, March 2016

Incorporating Heavy Alkanes in Metal–Organic Frameworks for Optimizing Adsorbed Natural Gas Capacity journal, July 2018

Micelles in Non‐Aqueous Media journal, May 1949

Supramolecular templating of hierarchically porous metal–organic frameworks journal, January 2014

Temperature Effect on Micelle Formation: Molecular Thermodynamic Model Revisited journal, February 2016

Suspension Processing of Microporous Metal-Organic Frameworks: A Scalable Route to High-Quality Adsorbents journal, July 2018

Physisorption of gases, with special reference to the evaluation of surface area and pore size distribution (IUPAC Technical Report)
journal, October 2015

Amino acid assisted templating synthesis of hierarchical zeolitic imidazolate framework-8 for efficient arsenate removal
journal, January 2014

A Kinetic Study of the Growth of Fatty Acid Vesicles
journal, August 2004

Nanoscale metal–organic frameworks for drug delivery: a conventional platform with new promise
journal, January 2018

Ultrafast room-temperature synthesis of hierarchically porous metal–organic frameworks by a versatile cooperative template strategy
journal, August 2018

Gas storage in porous metal–organic frameworks for clean energy applications
journal, January 2010

Creating Hierarchical Pores by Controlled Linker Thermolysis in Multivariate Metal–Organic Frameworks
journal, January 2018

Hierarchically structured metal–organic frameworks assembled by hydroxy double salt–template synergy with high space–time yields
journal, January 2018

Aqueous-Phase Synthesis of Mesoporous Zr-Based MOFs Templated by Amphoteric Surfactants
journal, February 2018

A Modulator-Induced Defect-Formation Strategy to Hierarchically Porous Metal-Organic Frameworks with High Stability
journal, December 2016

Micelle Formation and the Hydrophobic Effect ^†
journal, May 2004

Metal–organic frameworks for energy storage: Batteries and supercapacitors
journal, January 2016

Implicit-Solvent Models for Micellization: Nonionic Surfactants and Temperature-Dependent Properties
journal, February 2011

Solvophobic Interactions and Micelle Formation in Structure Forming Nonaqueous Solvents
journal, June 1971

Aqueous-Phase Synthesis of Mesoporous Zr-Based MOFs Templated by Amphoteric Surfactants
journal, February 2018

Kinetically tuned dimensional augmentation as a versatile synthetic route towards robust metal–organic frameworks
journal, December 2014

Characterization of micro- and mesoporous solids by physisorption methods and pore-size analysis
journal, November 1998

PCN-250 under Pressure: Sequential Phase Transformation and the Implications for MOF Densification
journal, December 2017

Effect of temperature on micelle formation in aqueous solutions of alkyltrimethylammonium bromides
journal, April 1989

A comparison of micelle formation of ionic surfactants in formamide, in N-methylformamide and in N,N-dimethylformamide
journal, June 2003

Pore size determination in modified micro- and mesoporous materials. Pitfalls and limitations in gas adsorption data analysis
journal, June 2003

A Modulator-Induced Defect-Formation Strategy to Hierarchically Porous Metal-Organic Frameworks with High Stability
journal, December 2016

Template-directed synthesis of metal–organic materials
journal, January 2014

Hierarchically mesostructured MIL-101 metal–organic frameworks: supramolecular template-directed synthesis and accelerated adsorption kinetics for dye removal
journal, January 2012

Introduction to Metal–Organic Frameworks
journal, September 2011

Template synthesis of hierarchical porous metal–organic frameworks with tunable porosity
journal, January 2017

Effect of Benzoic Acid as a Modulator in the Structure of UiO-66: An Experimental and Computational Study
journal, April 2017

Construction of hierarchically porous metal–organic frameworks through linker labilization
journal, May 2017

Applications of hierarchically structured porous materials from energy storage and conversion, catalysis, photocatalysis, adsorption, separation, and sensing to biomedicine
journal, January 2016

Determination of pore size and pore size distribution
journal, November 1994

Modulator Effects on the Water-Based Synthesis of Zr/Hf Metal–Organic Frameworks: Quantitative Relationship Studies between Modulator, Synthetic Condition, and Performance
journal, March 2016

Incorporating Heavy Alkanes in Metal–Organic Frameworks for Optimizing Adsorbed Natural Gas Capacity
journal, July 2018

Micelles in Non‐Aqueous Media
journal, May 1949

Supramolecular templating of hierarchically porous metal–organic frameworks
journal, January 2014

Temperature Effect on Micelle Formation: Molecular Thermodynamic Model Revisited
journal, February 2016

Suspension Processing of Microporous Metal-Organic Frameworks: A Scalable Route to High-Quality Adsorbents
journal, July 2018