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Title: Lateral charge carrier transport properties of B-10 enriched hexagonal BN thick epilayers

Abstract

Neutron detectors based on B-10 enriched hexagonal boron nitride (h- 10BN or h-BN) epilayers have demonstrated the highest thermal neutron detection efficiency among solid-state neutron detectors at about 58%. However, many fundamental transport parameters of h-BN, including the room temperature carrier mobility, minority carrier lifetime, and surface recombination velocity, which are essential to the performance of detectors, are still unknown. Here, we report here the carrier drift mobilities ( μ) and lifetimes (τ) of both electrons and holes in h- 10BN epilayers measured by using a time-of-flight (TOF) technique. Lateral photoconductive type detectors fabricated from a 65 μm thick freestanding h- 10BN epilayer were utilized to carry out the TOF measurements, which revealed μ e ~34 cm 2/V s for electrons and μ h ~36 cm 2/V s for holes and carrier lifetimes on the order of tens of microseconds. By combining the values of μ measured from TOF with S/μ (the ratio of the surface recombination velocity to mobility) deduced directly from the bias voltage dependence of photocurrent, S for both electrons ( S e ~1.4 × 10 4 cm/s) and holes ( S h ~2.7 × 10 3 cm/s) in h- 10BN has been extracted. The determination ofmore » these important fundamental parameters (μ, τ, and S) not only provides a better understanding of the carrier dynamics and electrical transport properties of h-BN but is also valuable for further advancing the development of h-BN materials and devices.« less

Authors:
 [1];  [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]
  1. Texas Tech Univ., Lubbock, TX (United States). Dept. of Electrical and Computer Engineering
Publication Date:
Research Org.:
Texas Tech Univ., Lubbock, TX (United States)
Sponsoring Org.:
USDOE Advanced Research Projects Agency - Energy (ARPA-E)
OSTI Identifier:
1571782
Alternate Identifier(s):
OSTI ID: 1557337
Grant/Contract Number:  
AR0000964; NA0002927
Resource Type:
Accepted Manuscript
Journal Name:
Applied Physics Letters
Additional Journal Information:
Journal Volume: 115; Journal Issue: 7; Journal ID: ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
15 GEOTHERMAL ENERGY; 36 MATERIALS SCIENCE; 61 RADIATION PROTECTION AND DOSIMETRY

Citation Formats

Grenadier, S., Maity, A., Li, J., Lin, J. Y., and Jiang, H. X. Lateral charge carrier transport properties of B-10 enriched hexagonal BN thick epilayers. United States: N. p., 2019. Web. doi:10.1063/1.5097984.
Grenadier, S., Maity, A., Li, J., Lin, J. Y., & Jiang, H. X. Lateral charge carrier transport properties of B-10 enriched hexagonal BN thick epilayers. United States. doi:10.1063/1.5097984.
Grenadier, S., Maity, A., Li, J., Lin, J. Y., and Jiang, H. X. Wed . "Lateral charge carrier transport properties of B-10 enriched hexagonal BN thick epilayers". United States. doi:10.1063/1.5097984.
@article{osti_1571782,
title = {Lateral charge carrier transport properties of B-10 enriched hexagonal BN thick epilayers},
author = {Grenadier, S. and Maity, A. and Li, J. and Lin, J. Y. and Jiang, H. X.},
abstractNote = {Neutron detectors based on B-10 enriched hexagonal boron nitride (h-10BN or h-BN) epilayers have demonstrated the highest thermal neutron detection efficiency among solid-state neutron detectors at about 58%. However, many fundamental transport parameters of h-BN, including the room temperature carrier mobility, minority carrier lifetime, and surface recombination velocity, which are essential to the performance of detectors, are still unknown. Here, we report here the carrier drift mobilities (μ) and lifetimes (τ) of both electrons and holes in h-10BN epilayers measured by using a time-of-flight (TOF) technique. Lateral photoconductive type detectors fabricated from a 65 μm thick freestanding h-10BN epilayer were utilized to carry out the TOF measurements, which revealed μe ~34 cm2/V s for electrons and μh ~36 cm2/V s for holes and carrier lifetimes on the order of tens of microseconds. By combining the values of μ measured from TOF with S/μ (the ratio of the surface recombination velocity to mobility) deduced directly from the bias voltage dependence of photocurrent, S for both electrons (Se ~1.4 × 104 cm/s) and holes (Sh ~2.7 × 103 cm/s) in h-10BN has been extracted. The determination of these important fundamental parameters (μ, τ, and S) not only provides a better understanding of the carrier dynamics and electrical transport properties of h-BN but is also valuable for further advancing the development of h-BN materials and devices.},
doi = {10.1063/1.5097984},
journal = {Applied Physics Letters},
number = 7,
volume = 115,
place = {United States},
year = {2019},
month = {8}
}

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Works referenced in this record:

Van der Waals heterostructures
journal, July 2013

  • Geim, A. K.; Grigorieva, I. V.
  • Nature, Vol. 499, Issue 7459, p. 419-425
  • DOI: 10.1038/nature12385

Boron nitride substrates for high-quality graphene electronics
journal, August 2010

  • Dean, C. R.; Young, A. F.; Meric, I.
  • Nature Nanotechnology, Vol. 5, Issue 10, p. 722-726
  • DOI: 10.1038/nnano.2010.172

High Carrier Mobility in Single-Crystal Plasma-Deposited Diamond
journal, September 2002

  • Isberg, Jan; Hammersberg, Johan; Johansson, Erik
  • Science, Vol. 297, Issue 5587, p. 1670-1672
  • DOI: 10.1126/science.1074374

Light scattering study of boron nitride microcrystals
journal, June 1981

  • Nemanich, R. J.; Solin, S. A.; Martin, Richard M.
  • Physical Review B, Vol. 23, Issue 12, p. 6348-6356
  • DOI: 10.1103/PhysRevB.23.6348