Electrolyte Gated Oxides

Bollinger, Anthony T.; Dubuis, Guy; Leng, Xiang; He, Xi; Božović, Ivan

doi:10.1007/s10948-019-05313-3

Title: Electrolyte Gated Oxides

Abstract

Electrolyte gating has the potential to generate electric fields at the surface of materials in the 10⁷-10⁸ V/cm range and induce charge carriers in these materials up to 10¹⁴-10¹⁵ cm^-2, making this technique very attractive for studying complex and functional oxides. Several types of processes — notably including proton diffusion and intake — can occur during charging, which makes it crucially important to consider and understand exactly how a given material is interacting with an electrolyte. We report on several of these mechanisms and how to distinguish between them.

Authors:

^[1]; Dubuis, Guy ^[2]; Leng, Xiang ^[3]; He, Xi ^[4]; Božović, Ivan ^[4]

Brookhaven National Lab. (BNL), Upton, NY (United States)
Victoria Univ. of Wellington (New Zealand)
Brookhaven National Lab. (BNL), Upton, NY (United States); Lumentum Operations LLC, Milpitas, CA (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States); Yale Univ., New Haven, CT (United States)

Publication Date:: Mon Nov 04 00:00:00 EST 2019

Research Org.:: Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; Gordon and Betty Moore Foundation’s EPiQS Initiative; USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1571430

Alternate Identifier(s):: OSTI ID: 1566291

Report Number(s):: BNL-212203-2019-JAAM; BNL-212111-2019-JAAM
Journal ID: ISSN 1557-1939; TRN: US2001343

Grant/Contract Number:: SC0012704

Resource Type:: Accepted Manuscript

Journal Name:: Journal of Superconductivity and Novel Magnetism

Additional Journal Information:: Journal Volume: 33; Journal Issue: 1; Journal ID: ISSN 1557-1939

Publisher:: Springer

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Electrolyte Gating; Oxides; Electrical transport

Citation Formats


                    Bollinger, Anthony T., Dubuis, Guy, Leng, Xiang, He, Xi, and Božović, Ivan. Electrolyte Gated Oxides.  United States: N. p., 2019. 
Web.  doi:10.1007/s10948-019-05313-3.

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                    Bollinger, Anthony T., Dubuis, Guy, Leng, Xiang, He, Xi, & Božović, Ivan. Electrolyte Gated Oxides.  United States.  https://doi.org/10.1007/s10948-019-05313-3

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                    Bollinger, Anthony T., Dubuis, Guy, Leng, Xiang, He, Xi, and Božović, Ivan. Mon .  
"Electrolyte Gated Oxides".  United States.  https://doi.org/10.1007/s10948-019-05313-3.  https://www.osti.gov/servlets/purl/1571430.

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@article{osti_1571430,

  title        = {Electrolyte Gated Oxides},

  author       = {Bollinger, Anthony T. and Dubuis, Guy and Leng, Xiang and He, Xi and Božović, Ivan},

  abstractNote = {Electrolyte gating has the potential to generate electric fields at the surface of materials in the 107-108 V/cm range and induce charge carriers in these materials up to 1014-1015 cm-2, making this technique very attractive for studying complex and functional oxides. Several types of processes — notably including proton diffusion and intake — can occur during charging, which makes it crucially important to consider and understand exactly how a given material is interacting with an electrolyte. We report on several of these mechanisms and how to distinguish between them.},

  doi          = {10.1007/s10948-019-05313-3},

  journal      = {Journal of Superconductivity and Novel Magnetism},

  number       = 1,

  volume       = 33,

  place        = {United States},

  year         = {Mon Nov 04 00:00:00 EST 2019},

  month        = {Mon Nov 04 00:00:00 EST 2019}

}

Copy to clipboard

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Title: Electrolyte Gated Oxides

Abstract

Citation Formats

Electrostatic Tuning of the Hole Density in NdBa 2 Cu 3 O 7 − δ Films and its Effect on the Hall Response journal, January 2002

Protonation induced high- T c phases in iron-based superconductors evidenced by NMR and magnetization measurements journal, January 2018

New Method for High-Accuracy Determination of the Fine-Structure Constant Based on Quantized Hall Resistance journal, August 1980

Antiferromagnetic order of Cu in Sm 2 CuO 4 journal, April 1991

Electric field effect on superconducting YBa2Cu3O7?? films journal, October 1991

Electrolyte-Gated SmCoO 3 Thin-Film Transistors Exhibiting Thickness-Dependent Large Switching Ratio at Room Temperature journal, February 2013

Insulator to metal transition in WO3 induced by electrolyte gating journal, July 2017

Collective bulk carrier delocalization driven by electrostatic surface charge accumulation journal, July 2012

Suppression of Metal-Insulator Transition in VO2 by Electric Field-Induced Oxygen Vacancy Formation journal, March 2013

Room-Temperature-Protonation-Driven On-Demand Metal-Insulator Conversion of a Transition Metal Oxide journal, June 2015

BiFeO 3 /YBa 2 Cu 3 O 7−δ heterostructures for strong ferroelectric modulation of superconductivity journal, January 2013

Purely electronic mechanism of electrolyte gating of indium tin oxide thin films journal, August 2016

Transient Characteristics for Proton Gating in Laterally Coupled Indium–Zinc-Oxide Transistors journal, March 2015

Electric field effect in correlated oxide systems journal, August 2003

Electric-field-induced superconductivity in electrochemically etched ultrathin FeSe films on SrTiO3 and MgO journal, November 2015

Electric-Field Control of the Metal-Insulator Transition in Ultrathin NdNiO3 Films journal, October 2010

Effect of gate voltage polarity on the ionic liquid gating behavior of NdNiO 3 /NdGaO 3 heterostructures journal, May 2017

Superconductor–insulator transition in La2 − xSr x CuO4 at the pair quantum resistance journal, April 2011

Field-effect tuning of carrier density in Nd1.2Ba1.8Cu3Oy thin films journal, May 2004

Studies of superconducting field effect transistors with sheet resistances close to the quantum resistance journal, May 2005

Electric-field-induced superconductivity in an insulator journal, October 2008

Highly conductive nanolayers on strontium titanate produced by preferential ion-beam etching journal, July 2005

“Cut and Stick” Rubbery Ion Gels as High Capacitance Gate Dielectrics journal, July 2012

Origin of Charge Density at LaAlO3 on SrTiO3 Heterointerfaces: Possibility of Intrinsic Doping journal, May 2007

Watch out for the lack of oxygen journal, July 2007

Electron-doped superconductivity at 40 K in the infinite-layer compound Sr1–yNdyCu02 journal, June 1991

Superconducting Interfaces Between Insulating Oxides journal, August 2007

The electrochemical impact on electrostatic modulation of the metal-insulator transition in nickelates journal, March 2015

Dual field effects in electrolyte-gated spinel ferrite: electrostatic carrier doping and redox reactions journal, July 2014

High-Density Carrier Accumulation in ZnO Field-Effect Transistors Gated by Electric Double Layers of Ionic Liquids journal, April 2009

Influence of the doping concentration of Y1−yCayBa2Cu3O7−δ drain-source channels on the properties of superconducting field-effect devices journal, October 2003

Oxygen Displacement in Cuprates under Ionic Liquid Field-Effect Gating journal, August 2016

Suppression of Ionic Liquid Gate-Induced Metallization of SrTiO 3 (001) by Oxygen journal, September 2013

Electric-Field-Effect Modulation of the Transition Temperature, Mobile Carrier Density, and In-Plane Penetration Depth of NdBa 2 Cu 3 O 7 − δ Thin Films journal, January 2007

Electric double layer transistors with ferroelectric BaTiO 3 channels journal, June 2014

Modulation of the Electrical Properties of VO 2 Nanobeams Using an Ionic Liquid as a Gating Medium journal, May 2012

Modulation of Metal-Insulator Transition in VO 2 by Electrolyte Gating-Induced Protonation journal, December 2015

Superconductivity at 110 K in the infinite-layer compound (Sr1-xCax)1-yCuO2 journal, April 1992

Response of the double-layer capacitance of a high-temperature superconductor/fluid electrolyte interface to the onset of superconductivity journal, August 1992

Electrostatic Modulation of Superconductivity in Ultrathin GdBa2Cu3O7-x Films journal, May 1999

Tuning of the metal-insulator transition in electrolyte-gated NdNiO3 thin films journal, October 2010

Electrical conduction on the surface of ferroelectric PbTiO3 thin film induced by electrolyte gating journal, January 2018

Electric field effect on superconducting YBa2Cu3O7−δ films journal, December 1991

Electric-field-induced superconductivity in electrochemically-etched ultrathin FeSe films on SrTiO3 and MgO text, January 2015

Insulator to Metal Transition in WO$_3$ Induced by Electrolyte Gating text, January 2017

Protonation induced high-Tc phases in iron-based superconductors evidenced by NMR and magnetization measurements text, January 2017

Electrostatic Tuning of the Hole Density in ${{NdBa}_{2} {Cu}_{3} O}_{7 - δ}$ Films and its Effect on the Hall Response
journal, January 2002

Protonation induced high- T c phases in iron-based superconductors evidenced by NMR and magnetization measurements
journal, January 2018

New Method for High-Accuracy Determination of the Fine-Structure Constant Based on Quantized Hall Resistance
journal, August 1980

Antiferromagnetic order of Cu in Sm ₂ CuO ₄
journal, April 1991

Electric field effect on superconducting YBa2Cu3O7?? films
journal, October 1991

Electrolyte-Gated SmCoO ₃ Thin-Film Transistors Exhibiting Thickness-Dependent Large Switching Ratio at Room Temperature
journal, February 2013

Insulator to metal transition in WO3 induced by electrolyte gating
journal, July 2017

Collective bulk carrier delocalization driven by electrostatic surface charge accumulation
journal, July 2012

Suppression of Metal-Insulator Transition in VO2 by Electric Field-Induced Oxygen Vacancy Formation
journal, March 2013

Room-Temperature-Protonation-Driven On-Demand Metal-Insulator Conversion of a Transition Metal Oxide
journal, June 2015

BiFeO ₃ /YBa ₂ Cu ₃ O _7−δ heterostructures for strong ferroelectric modulation of superconductivity
journal, January 2013

Purely electronic mechanism of electrolyte gating of indium tin oxide thin films
journal, August 2016

Transient Characteristics for Proton Gating in Laterally Coupled Indium–Zinc-Oxide Transistors
journal, March 2015

Electric field effect in correlated oxide systems
journal, August 2003

Electric-field-induced superconductivity in electrochemically etched ultrathin FeSe films on SrTiO3 and MgO
journal, November 2015

Electric-Field Control of the Metal-Insulator Transition in Ultrathin NdNiO3 Films
journal, October 2010

Effect of gate voltage polarity on the ionic liquid gating behavior of NdNiO ₃ /NdGaO ₃ heterostructures
journal, May 2017

Superconductor–insulator transition in La2 − xSr x CuO4 at the pair quantum resistance
journal, April 2011

Field-effect tuning of carrier density in Nd1.2Ba1.8Cu3Oy thin films
journal, May 2004

Studies of superconducting field effect transistors with sheet resistances close to the quantum resistance
journal, May 2005

Electric-field-induced superconductivity in an insulator
journal, October 2008

Highly conductive nanolayers on strontium titanate produced by preferential ion-beam etching
journal, July 2005

“Cut and Stick” Rubbery Ion Gels as High Capacitance Gate Dielectrics
journal, July 2012

Origin of Charge Density at ${LaAlO}_{3}$ on ${SrTiO}_{3}$ Heterointerfaces: Possibility of Intrinsic Doping
journal, May 2007

Watch out for the lack of oxygen
journal, July 2007

Electron-doped superconductivity at 40 K in the infinite-layer compound Sr1–yNdyCu02
journal, June 1991

Superconducting Interfaces Between Insulating Oxides
journal, August 2007

The electrochemical impact on electrostatic modulation of the metal-insulator transition in nickelates
journal, March 2015

Dual field effects in electrolyte-gated spinel ferrite: electrostatic carrier doping and redox reactions
journal, July 2014

High-Density Carrier Accumulation in ZnO Field-Effect Transistors Gated by Electric Double Layers of Ionic Liquids
journal, April 2009

Influence of the doping concentration of Y1−yCayBa2Cu3O7−δ drain-source channels on the properties of superconducting field-effect devices
journal, October 2003

Oxygen Displacement in Cuprates under Ionic Liquid Field-Effect Gating
journal, August 2016

Suppression of Ionic Liquid Gate-Induced Metallization of SrTiO ₃ (001) by Oxygen
journal, September 2013

Electric-Field-Effect Modulation of the Transition Temperature, Mobile Carrier Density, and In-Plane Penetration Depth of ${NdBa}_{2} {Cu}_{3} O_{7 - δ}$ Thin Films
journal, January 2007

Electric double layer transistors with ferroelectric BaTiO ₃ channels
journal, June 2014

Modulation of the Electrical Properties of VO ₂ Nanobeams Using an Ionic Liquid as a Gating Medium
journal, May 2012

Modulation of Metal-Insulator Transition in VO ₂ by Electrolyte Gating-Induced Protonation
journal, December 2015

Superconductivity at 110 K in the infinite-layer compound (Sr1-xCax)1-yCuO2
journal, April 1992

Response of the double-layer capacitance of a high-temperature superconductor/fluid electrolyte interface to the onset of superconductivity
journal, August 1992

Electrostatic Modulation of Superconductivity in Ultrathin GdBa2Cu3O7-x Films
journal, May 1999

Tuning of the metal-insulator transition in electrolyte-gated NdNiO3 thin films
journal, October 2010

Electrical conduction on the surface of ferroelectric PbTiO3 thin film induced by electrolyte gating
journal, January 2018

Electric field effect on superconducting YBa2Cu3O7−δ films
journal, December 1991

Electric-field-induced superconductivity in electrochemically-etched ultrathin FeSe films on SrTiO3 and MgO
text, January 2015

Insulator to Metal Transition in WO$_3$ Induced by Electrolyte Gating
text, January 2017

Protonation induced high-Tc phases in iron-based superconductors evidenced by NMR and magnetization measurements
text, January 2017