Low-Temperature Thermopower in CoSbS

Du, Qianheng; Abeykoon, Milinda; Liu, Yu; Kotliar, G.; Petrovic, C.

doi:10.1103/PhysRevLett.123.076602

Title: Low-Temperature Thermopower in CoSbS

Abstract

Here, we report on giant thermopower of S = 2.5 mV/K in CoSbS single crystals: a material that shows strong high-temperature thermoelectric performance when doped with Ni or Se. Changes of low-temperature thermopower induced by a magnetic field point to the mechanism of electronic diffusion of carriers in the heavy valence band. Intrinsic magnetic susceptibility is consistent with the Kondo-insulatorlike accumulation of electronic states around the gap edges. This suggests that giant thermopower stems from temperature-dependent renormalization of the noninteracting bands and buildup of the electronic correlations on cooling.

Authors:

^[1]; Abeykoon, Milinda ^[2]; Liu, Yu ^[3]; Kotliar, G. ^[4]; Petrovic, C. ^[1]

Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.; Stony Brook Univ., NY (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States). National Synchrotron Light Source II (NSLS-II)
Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.; Rutgers Univ., Piscataway, NJ (United States)

Publication Date:: 2019-08-16

Research Org.:: Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1570672

Alternate Identifier(s):: OSTI ID: 1567981

Report Number(s):: BNL-212195-2019-JAAM
Journal ID: ISSN 0031-9007; PRLTAO; TRN: US2100167

Grant/Contract Number:: SC0012704

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review Letters

Additional Journal Information:: Journal Volume: 123; Journal Issue: 7; Journal ID: ISSN 0031-9007

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Du, Qianheng, Abeykoon, Milinda, Liu, Yu, Kotliar, G., and Petrovic, C. Low-Temperature Thermopower in CoSbS.  United States: N. p., 2019. 
Web.  doi:10.1103/PhysRevLett.123.076602.

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                    Du, Qianheng, Abeykoon, Milinda, Liu, Yu, Kotliar, G., & Petrovic, C. Low-Temperature Thermopower in CoSbS.  United States.  https://doi.org/10.1103/PhysRevLett.123.076602

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                    Du, Qianheng, Abeykoon, Milinda, Liu, Yu, Kotliar, G., and Petrovic, C. Fri .  
"Low-Temperature Thermopower in CoSbS".  United States.  https://doi.org/10.1103/PhysRevLett.123.076602.  https://www.osti.gov/servlets/purl/1570672.

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@article{osti_1570672,

  title        = {Low-Temperature Thermopower in CoSbS},

  author       = {Du, Qianheng and Abeykoon, Milinda and Liu, Yu and Kotliar, G. and Petrovic, C.},

  abstractNote = {Here, we report on giant thermopower of S = 2.5 mV/K in CoSbS single crystals: a material that shows strong high-temperature thermoelectric performance when doped with Ni or Se. Changes of low-temperature thermopower induced by a magnetic field point to the mechanism of electronic diffusion of carriers in the heavy valence band. Intrinsic magnetic susceptibility is consistent with the Kondo-insulatorlike accumulation of electronic states around the gap edges. This suggests that giant thermopower stems from temperature-dependent renormalization of the noninteracting bands and buildup of the electronic correlations on cooling.},

  doi          = {10.1103/PhysRevLett.123.076602},

  journal      = {Physical Review Letters},

  number       = 7,

  volume       = 123,

  place        = {United States},

  year         = {2019},

  month        = {8}

}

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Title: Low-Temperature Thermopower in CoSbS

Abstract

Citation Formats

A matrix formalism for the Hall effect in multicarrier semiconductor systems journal, September 1999

High performance bulk thermoelectrics via a panoscopic approach journal, May 2013

The effect of nickel doping on electron and phonon transport in the n-type nanostructured thermoelectric material CoSbS journal, January 2015

Electronic thermoelectric power factor and metal-insulator transition in FeSb 2 journal, September 2012

Preparation and characterization of some cobalt phosphorus, cobalt arsenic, cobalt antimony sulfide or selenide compounds journal, June 1974

Electronic and thermoelectric properties of CoSbS and FeSbS journal, January 2013

Paramagnetic Excited State of FeSi journal, August 1967

Observation of enhanced thermopower due to spin fluctuation in weak itinerant ferromagnet journal, February 2019

A simplified method for calculating the debye temperature from elastic constants journal, July 1963

Kondo insulator description of spin state transition in FeSb2 journal, July 2005

Complex thermoelectric materials journal, February 2008

Thermoelectric Response Near the Density Driven Mott Transition journal, May 1998

Semiconductivity in pyrite, marcasite and arsenopyrite phases journal, February 1965

Colossal Seebeck effect enhanced by quasi-ballistic phonons dragging massive electrons in FeSb2 journal, September 2016

Unconventional charge gap formation in FeSi journal, September 1993

Effects of Spin and Orbital Degeneracy on the Thermopower of Strongly Correlated Systems journal, November 2001

Ce3Bi4Pt3 and hybridization Gap physics journal, April 1992

Thermoelectric and Magnetic Properties of a Narrow-Gap Semiconductor FeGa 3 journal, January 2009

Theory of the Thermoelectric Power of Semiconductors journal, December 1954

Magnetic, transport, and structural properties of Fe 1 − x Ir x Si journal, September 1994

Observation of Anderson Localization in an Electron Gas journal, May 1969

FeSb 2 : Prototype of huge electron-diffusion thermoelectricity journal, April 2009

Resonant levels in bulk thermoelectric semiconductors journal, January 2012

Study for material analogs of FeSb 2 : Material design for thermoelectric materials journal, March 2018

Kondo-hole conduction in the La-doped Kondo insulator Ce 3 Bi 4 Pt 3 journal, March 2008

Structural and magnetic transitions in PbV 6 O 11 journal, October 2001

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Highly dispersive electron relaxation and colossal thermoelectricity in the correlated semiconductor FeSb 2 journal, December 2013

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Thermodynamics of FeSi journal, February 1995

On the thermoelectricity of correlated electrons in the zero-temperature limit journal, July 2004

Transport properties of silicon journal, August 1991

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Strong Reduction of Thermal Conductivity and Enhanced Thermoelectric Properties in CoSbS1-xSex Paracostibite journal, April 2017

Low-temperature transport, thermodynamic, and optical properties of FeSi journal, November 1997

Introduction to Thermoelectricity book, January 2010

Semiconductivity in pyrite, marcasite and arsenopyrite phases journal, August 1964

A matrix formalism for the Hall effect in multicarrier semiconductor systems
journal, September 1999

High performance bulk thermoelectrics via a panoscopic approach
journal, May 2013

The effect of nickel doping on electron and phonon transport in the n-type nanostructured thermoelectric material CoSbS
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Electronic thermoelectric power factor and metal-insulator transition in FeSb $_{2}$
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Preparation and characterization of some cobalt phosphorus, cobalt arsenic, cobalt antimony sulfide or selenide compounds
journal, June 1974

Electronic and thermoelectric properties of CoSbS and FeSbS
journal, January 2013

Paramagnetic Excited State of FeSi
journal, August 1967

Observation of enhanced thermopower due to spin fluctuation in weak itinerant ferromagnet
journal, February 2019

A simplified method for calculating the debye temperature from elastic constants
journal, July 1963

Kondo insulator description of spin state transition in FeSb2
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Complex thermoelectric materials
journal, February 2008

Thermoelectric Response Near the Density Driven Mott Transition
journal, May 1998

Semiconductivity in pyrite, marcasite and arsenopyrite phases
journal, February 1965

Colossal Seebeck effect enhanced by quasi-ballistic phonons dragging massive electrons in FeSb2
journal, September 2016

Unconventional charge gap formation in FeSi
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Effects of Spin and Orbital Degeneracy on the Thermopower of Strongly Correlated Systems
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Ce3Bi4Pt3 and hybridization Gap physics
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Thermoelectric and Magnetic Properties of a Narrow-Gap Semiconductor FeGa ₃
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journal, March 2018

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