Spatial control of heavy-fermion superconductivity in CeIrIn5

Bachmann, Maja D.; Ferguson, G. M.; Theuss, Florian; Meng, Tobias; Putzke, Carsten; Helm, Toni; Shirer, K. R.; Li, You-Sheng; Modic, K. A.; Nicklas, Michael; König, Markus; Low, D.; Ghosh, Sayak; Mackenzie, Andrew P.; Arnold, Frank; Hassinger, Elena; McDonald, Ross D.; Winter, Laurel E.; Bauer, Eric D.; Ronning, Filip; Ramshaw, B. J.; Nowack, Katja C.; Moll, Philip J. W.

doi:10.1126/science.aao6640

Title: Spatial control of heavy-fermion superconductivity in CeIrIn₅

Abstract

While crystals of strongly correlated metals exhibit a diverse set of electronic ground states, few approaches exist for spatially modulating their properties. In this study, we demonstrate disorder-free control, on the micrometer scale, over the superconducting state in samples of the heavy-fermion superconductor CeIrIn₅. We pattern crystals by focused ion beam milling to tailor the boundary conditions for the elastic deformation upon thermal contraction during cooling. The resulting nonuniform strain fields induce complex patterns of superconductivity, owing to the strong dependence of the transition temperature on the strength and direction of strain. These findings showcase a generic approach to manipulating electronic order on micrometer length scales in strongly correlated matter without compromising the cleanliness, stoichiometry, or mean free path.

Authors:

^[1];

^[2];

^[2]; Meng, Tobias ^[3];

^[4];

^[5];

^[5]; Li, You-Sheng ^[1];

^[5];

^[5]; König, Markus ^[5]; Low, D. ^[2];

^[2]; Mackenzie, Andrew P. ^[1]; Arnold, Frank ^[5];

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^[7] more »

Max Planck Institute for Chemical Physics of Solids, D-01187 Dresden, Germany., School of Physics and Astronomy, University of St. Andrews, St. Andrews KY16 9SS, UK.
Laboratory of Atomic and Solid State Physics, Cornell University, Ithaca, NY 14853, USA.
Institute for Theoretical Physics, Technical University Dresden, D-01062 Dresden, Germany.
Max Planck Institute for Chemical Physics of Solids, D-01187 Dresden, Germany., Institute of Material Science and Engineering, École Polytechnique Fédéral de Lausanne (EPFL), 1015 Lausanne, Switzerland.
Max Planck Institute for Chemical Physics of Solids, D-01187 Dresden, Germany.
Max Planck Institute for Chemical Physics of Solids, D-01187 Dresden, Germany., Physik-Department, Technische Universität München, Garching, D-85748 Germany.
Los Alamos National Laboratory, Los Alamos, NM 87545, USA.
Laboratory of Atomic and Solid State Physics, Cornell University, Ithaca, NY 14853, USA., Kavli Institute at Cornell for Nanoscale Science, Cornell University, Ithaca, NY 14853, USA.

Publication Date:: 2019-10-10

Research Org.:: Cornell Univ., Ithaca, NY (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; German Research Foundation (DFG); National Science Foundation (NSF); European Research Council (ERC)

OSTI Identifier:: 1570501

Alternate Identifier(s):: OSTI ID: 1617015

Grant/Contract Number:: SC0015947; DMR-1719875; DMR-1157490; DMR-1644779

Resource Type:: Published Article

Journal Name:: Science

Additional Journal Information:: Journal Name: Science Journal Volume: 366 Journal Issue: 6462; Journal ID: ISSN 0036-8075

Publisher:: AAAS

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 77 NANOSCIENCE AND NANOTECHNOLOGY; Strain tuning; Strain engineering; Spatial control; Scanning SQUID microscopy; Unconventional superconductivity

Citation Formats


                    Bachmann, Maja D., Ferguson, G. M., Theuss, Florian, Meng, Tobias, Putzke, Carsten, Helm, Toni, Shirer, K. R., Li, You-Sheng, Modic, K. A., Nicklas, Michael, König, Markus, Low, D., Ghosh, Sayak, Mackenzie, Andrew P., Arnold, Frank, Hassinger, Elena, McDonald, Ross D., Winter, Laurel E., Bauer, Eric D., Ronning, Filip, Ramshaw, B. J., Nowack, Katja C., and Moll, Philip J. W. Spatial control of heavy-fermion superconductivity in CeIrIn5.  United States: N. p., 2019. 
Web.  doi:10.1126/science.aao6640.

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                    Bachmann, Maja D., Ferguson, G. M., Theuss, Florian, Meng, Tobias, Putzke, Carsten, Helm, Toni, Shirer, K. R., Li, You-Sheng, Modic, K. A., Nicklas, Michael, König, Markus, Low, D., Ghosh, Sayak, Mackenzie, Andrew P., Arnold, Frank, Hassinger, Elena, McDonald, Ross D., Winter, Laurel E., Bauer, Eric D., Ronning, Filip, Ramshaw, B. J., Nowack, Katja C., & Moll, Philip J. W. Spatial control of heavy-fermion superconductivity in CeIrIn5.  United States.  https://doi.org/10.1126/science.aao6640

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                    Bachmann, Maja D., Ferguson, G. M., Theuss, Florian, Meng, Tobias, Putzke, Carsten, Helm, Toni, Shirer, K. R., Li, You-Sheng, Modic, K. A., Nicklas, Michael, König, Markus, Low, D., Ghosh, Sayak, Mackenzie, Andrew P., Arnold, Frank, Hassinger, Elena, McDonald, Ross D., Winter, Laurel E., Bauer, Eric D., Ronning, Filip, Ramshaw, B. J., Nowack, Katja C., and Moll, Philip J. W. Thu .  
"Spatial control of heavy-fermion superconductivity in CeIrIn5".  United States.  https://doi.org/10.1126/science.aao6640.

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@article{osti_1570501,

  title        = {Spatial control of heavy-fermion superconductivity in CeIrIn5},

  author       = {Bachmann, Maja D. and Ferguson, G. M. and Theuss, Florian and Meng, Tobias and Putzke, Carsten and Helm, Toni and Shirer, K. R. and Li, You-Sheng and Modic, K. A. and Nicklas, Michael and König, Markus and Low, D. and Ghosh, Sayak and Mackenzie, Andrew P. and Arnold, Frank and Hassinger, Elena and McDonald, Ross D. and Winter, Laurel E. and Bauer, Eric D. and Ronning, Filip and Ramshaw, B. J. and Nowack, Katja C. and Moll, Philip J. W.},

  abstractNote = {While crystals of strongly correlated metals exhibit a diverse set of electronic ground states, few approaches exist for spatially modulating their properties. In this study, we demonstrate disorder-free control, on the micrometer scale, over the superconducting state in samples of the heavy-fermion superconductor CeIrIn5. We pattern crystals by focused ion beam milling to tailor the boundary conditions for the elastic deformation upon thermal contraction during cooling. The resulting nonuniform strain fields induce complex patterns of superconductivity, owing to the strong dependence of the transition temperature on the strength and direction of strain. These findings showcase a generic approach to manipulating electronic order on micrometer length scales in strongly correlated matter without compromising the cleanliness, stoichiometry, or mean free path.},

  doi          = {10.1126/science.aao6640},

  journal      = {Science},

  number       = 6462,

  volume       = 366,

  place        = {United States},

  year         = {2019},

  month        = {10}

}

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Cited by: 21 works

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Figure 1: The superconducting transition in a slab under biaxial strain (A) Sketch of the distortion of a thin slab of CeIrIn₅ coupled to sapphire at low temperatures. (B) Optical image of a slab 2 μm in thickness cut by FIB machining in the (a,c) plane. (C)T_c-map across the samplemore »

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Works referenced in this record:

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Title: Spatial control of heavy-fermion superconductivity in CeIrIn5

Abstract

Citation Formats

Figures / Tables:

A Drastic Change of the Fermi Surface at a Critical Pressure in CeRhIn 5 : dHvA Study under Pressure journal, April 2005

Thermal Conductivity Evidence for a d x 2 − y 2 Pairing Symmetry in the Heavy-Fermion CeIrIn 5 Superconductor journal, May 2008

Interface superconductivity in the eutectic Sr 2 RuO 4 − Ru : 3-K phase of Sr 2 RuO 4 journal, June 2003

Sign Reversal of Field-Angle Resolved Heat Capacity Oscillations in a Heavy Fermion Superconductor CeCoIn 5 and d x 2 − y 2 Pairing Symmetry journal, January 2010

Structural Investigations of CeIrIn 5 and CeCoIn 5 on Macroscopic and Atomic Length Scales journal, June 2014

Strong Increase of Tc of Sr2RuO4 Under Both Tensile and Compressive Strain journal, April 2014

Heat capacity of the heavy fermion superconductor CeIrIn5 under hydrostatic pressure journal, March 2002

CeIrIn 5 : Superconductivity on a magnetic instability journal, January 2014

Flux dynamics and low-field magnetic properties of the heavy-fermion superconductor CeCu2Si2 journal, January 1993

Anisotropic elastic properties of CeRhIn 5 journal, January 2004

Perspective: Extremely fine tuning of doping enabled by combinatorial molecular-beam epitaxy journal, June 2015

Origin of the zero-resistance anomaly in heavy fermion superconducting CeIrIn 5 : A clue from magnetic-field and Rh-doping studies journal, November 2001

On the normal modes of free vibration of inhomogeneous and anisotropic elastic objects journal, October 1991

Uniaxial Pressure Effects on C e I r I n 5 and C e C o I n 5 Studied by Low-Temperature Thermal Expansion journal, August 2003

Analysis of the Normal-State Magnetotransport in CeIrIn5 journal, October 2008

Quasi-two-dimensional Fermi surfaces of the heavy fermion superconductor CeIrIn 5 journal, January 2001

Method for Measuring Electrical Resistivity of Anisotropic Materials journal, June 1971

Evidence of d -wave pairing symmetry of the gap of the heavy-fermion superconductor CeIrIn 5 from magnetic-penetration-depth measurements journal, June 2009

Avoided valence transition in a plutonium superconductor journal, March 2015

Magnetic properties of the heavy-fermion superconductors UPt3 and URu2Si2 journal, January 1993

Precursor state to superconductivity in CeIrIn 5 : Unusual scaling of magnetotransport journal, March 2009

Electronic in-plane symmetry breaking at field-tuned quantum criticality in CeRhIn5 journal, August 2017

Field-induced density wave in the heavy-fermion compound CeRhIn5 journal, March 2015

Anisotropic Dependence of Superconductivity on Uniaxial Pressure in CeIrIn 5 journal, May 2009

A new heavy-fermion superconductor CeIrIn 5 : A relative of the cuprates? journal, February 2001

Fermi Surface, Magnetic and Superconducting Properties of LaRhIn 5 and CeTIn 5 (T: Co, Rh and Ir) journal, January 2002

Title: Spatial control of heavy-fermion superconductivity in CeIrIn₅

A Drastic Change of the Fermi Surface at a Critical Pressure in CeRhIn ₅ : dHvA Study under Pressure
journal, April 2005

Thermal Conductivity Evidence for a $d_{x^{2} - y^{2}}$ Pairing Symmetry in the Heavy-Fermion ${CeIrIn}_{5}$ Superconductor
journal, May 2008

Interface superconductivity in the eutectic ${Sr}_{2} {RuO}_{4} - Ru :$ 3-K phase of ${Sr}_{2} {RuO}_{4}$
journal, June 2003

Sign Reversal of Field-Angle Resolved Heat Capacity Oscillations in a Heavy Fermion Superconductor ${CeCoIn}_{5}$ and $d_{x^{2} - y^{2}}$ Pairing Symmetry
journal, January 2010

Structural Investigations of CeIrIn ₅ and CeCoIn ₅ on Macroscopic and Atomic Length Scales
journal, June 2014

Strong Increase of Tc of Sr2RuO4 Under Both Tensile and Compressive Strain
journal, April 2014

Heat capacity of the heavy fermion superconductor CeIrIn5 under hydrostatic pressure
journal, March 2002

CeIrIn $_{5}$ : Superconductivity on a magnetic instability
journal, January 2014

Flux dynamics and low-field magnetic properties of the heavy-fermion superconductor CeCu2Si2
journal, January 1993

Anisotropic elastic properties of ${CeRhIn}_{5}$
journal, January 2004

Perspective: Extremely fine tuning of doping enabled by combinatorial molecular-beam epitaxy
journal, June 2015

Origin of the zero-resistance anomaly in heavy fermion superconducting ${CeIrIn}_{5} :$ A clue from magnetic-field and Rh-doping studies
journal, November 2001

On the normal modes of free vibration of inhomogeneous and anisotropic elastic objects
journal, October 1991

Uniaxial Pressure Effects on ${C e I r I n}_{5}$ and ${C e C o I n}_{5}$ Studied by Low-Temperature Thermal Expansion
journal, August 2003

Analysis of the Normal-State Magnetotransport in CeIrIn5
journal, October 2008

Quasi-two-dimensional Fermi surfaces of the heavy fermion superconductor ${CeIrIn}_{5}$
journal, January 2001

Method for Measuring Electrical Resistivity of Anisotropic Materials
journal, June 1971

Evidence of $d$ -wave pairing symmetry of the gap of the heavy-fermion superconductor ${CeIrIn}_{5}$ from magnetic-penetration-depth measurements
journal, June 2009

Avoided valence transition in a plutonium superconductor
journal, March 2015

Magnetic properties of the heavy-fermion superconductors UPt3 and URu2Si2
journal, January 1993

Precursor state to superconductivity in ${CeIrIn}_{5}$ : Unusual scaling of magnetotransport
journal, March 2009

Electronic in-plane symmetry breaking at field-tuned quantum criticality in CeRhIn5
journal, August 2017

Field-induced density wave in the heavy-fermion compound CeRhIn5
journal, March 2015

Anisotropic Dependence of Superconductivity on Uniaxial Pressure in ${CeIrIn}_{5}$
journal, May 2009

A new heavy-fermion superconductor CeIrIn ₅ : A relative of the cuprates?
journal, February 2001

Fermi Surface, Magnetic and Superconducting Properties of LaRhIn ₅ and CeTIn ₅ (T: Co, Rh and Ir)
journal, January 2002