Molecular Symmetry-Mixed Dichroism in Double Photoionization of $H2$
Abstract
Dichroism in double photoionization of H2 molecules by elliptically polarized extreme ultraviolet pulses is formulated analytically as a sum of atomiclike dichroism (AD) and molecular symmetry-mixed dichroism (MSMD) terms. The MSMD originates from an interplay of 1Σ and 1Π continuum molecular ionization amplitudes. For detection geometries in which the AD vanishes, numerical results for the sixfold differential probabilities for opposite pulse helicities show that the MSMD is significant in the electron momentum and angular distributions and is controllable by the ellipticity.
- Authors:
-
[1];
[1]
- Univ. of Nebraska, Lincoln, NE (United States)
- Voronezh State Univ., Voronezh (Russia). Dept. of Physics
- Aarhus Univ., Aarhus (Denmark). Dept. of Physics and Astronomy
- Univ. of Rochester, Rochester, NY (United States). Lab. for Laser Energetics
- Publication Date:
- Research Org.:
- Univ. of Nebraska-Lincoln, Lincoln, NE (United States); Univ. of Nebraska, Lincoln, NE (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA); Russian Ministry of Education and Science; VKR Center of Excellence; QUSCOPE
- OSTI Identifier:
- 1568769
- Alternate Identifier(s):
- OSTI ID: 1595971
- Grant/Contract Number:
- FG02-96ER14646; PHY-120003; NA0003856
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review Letters
- Additional Journal Information:
- Journal Volume: 123; Journal Issue: 14; Related Information: http://link.aps.org/supplemental/10.1103/PhysRevLett.123.143202; Journal ID: ISSN 0031-9007
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 74 ATOMIC AND MOLECULAR PHYSICS; double photoionization of diatomic molecules; atomic dichroism; molecular dichroism; molecular symmetry-mixed dichroism; achiral molecules; elliptically-polarized laser pulse; angular distributions; momentum distributions
Citation Formats
Djiokap, Jean Marcel Ngoko, Meremianin, Alexei V., Manakov, Nikolai L., Madsen, Lars B., Hu, Su Xing, and Starace, Anthony F. Molecular Symmetry-Mixed Dichroism in Double Photoionization of $H2$. United States: N. p., 2019.
Web. doi:10.1103/PhysRevLett.123.143202.
Djiokap, Jean Marcel Ngoko, Meremianin, Alexei V., Manakov, Nikolai L., Madsen, Lars B., Hu, Su Xing, & Starace, Anthony F. Molecular Symmetry-Mixed Dichroism in Double Photoionization of $H2$. United States. doi:10.1103/PhysRevLett.123.143202.
Djiokap, Jean Marcel Ngoko, Meremianin, Alexei V., Manakov, Nikolai L., Madsen, Lars B., Hu, Su Xing, and Starace, Anthony F. Wed .
"Molecular Symmetry-Mixed Dichroism in Double Photoionization of $H2$". United States. doi:10.1103/PhysRevLett.123.143202. https://www.osti.gov/servlets/purl/1568769.
@article{osti_1568769,
title = {Molecular Symmetry-Mixed Dichroism in Double Photoionization of $H2$},
author = {Djiokap, Jean Marcel Ngoko and Meremianin, Alexei V. and Manakov, Nikolai L. and Madsen, Lars B. and Hu, Su Xing and Starace, Anthony F.},
abstractNote = {Dichroism in double photoionization of H2 molecules by elliptically polarized extreme ultraviolet pulses is formulated analytically as a sum of atomiclike dichroism (AD) and molecular symmetry-mixed dichroism (MSMD) terms. The MSMD originates from an interplay of 1Σ and 1Π continuum molecular ionization amplitudes. For detection geometries in which the AD vanishes, numerical results for the sixfold differential probabilities for opposite pulse helicities show that the MSMD is significant in the electron momentum and angular distributions and is controllable by the ellipticity.},
doi = {10.1103/PhysRevLett.123.143202},
journal = {Physical Review Letters},
number = 14,
volume = 123,
place = {United States},
year = {2019},
month = {10}
}
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