Search Menu
DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information
Search Scholarly Publications

Title: Adaptive strong-field control of vibrational population in NO2+

Abstract

An adaptive closed-loop system employing coincidence time-of-flight feedback is used to determine the optimal pulse shapes for manipulating the branching ratio of NO dications following double ionization by an intense laser pulse. Selection between the long-lived NO2+ and the dissociative N+ + O+ final states requires control of the vibrational population distribution in the transient NO2+. The ability to both suppress and enhance NO2+ relative to N+ + O+ is observed, with the effectiveness of shaped pulses surpassing near Fourier transform-limited pulses by about an order of magnitude in each direction, depending on the pulse energy. The control is subsequently investigated using velocity map imaging, identifying plausible dissociation pathways leading to N+ + O+. Combining the information about the N+ + O+ dissociation with a well-defined control objective supports the conclusion that the primary control mechanism involves selectively populating long-lived NO2+ vibrational states.

Authors:
 [1]; ORCiD logo [2]; ORCiD logo [3];  [1];  [1]; ORCiD logo [3]; ORCiD logo [3]; ORCiD logo [1]
+ Show Author Affiliations
  1. Augustana College, Sioux Falls, SD (United States)
  2. Augustana College, Sioux Falls, SD (United States); Kansas State Univ., Manhattan, KS (United States)
  3. Kansas State Univ., Manhattan, KS (United States)
Publication Date:
Research Org.:
Kansas State Univ., Manhattan, KS (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1610039
Alternate Identifier(s):
OSTI ID: 1567725
Grant/Contract Number:  
FG02-86ER13491
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Chemical Physics
Additional Journal Information:
Journal Volume: 151; Journal Issue: 12; Journal ID: ISSN 0021-9606
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Chemistry; Physics; Femtochemistry; Velocity map imaging; Potential energy surfaces; Vibrational states; Molecular dynamics; Coherent control; Ultrafast lasers

Citation Formats

Voznyuk, O., Jochim, Bethany, Zohrabi, M., Broin, Adam, Averin, R., Carnes, K. D., Ben-Itzhak, I., and Wells, E. Adaptive strong-field control of vibrational population in NO2+. United States: N. p., 2019. Web. doi:10.1063/1.5115504.
Copy to clipboard
Voznyuk, O., Jochim, Bethany, Zohrabi, M., Broin, Adam, Averin, R., Carnes, K. D., Ben-Itzhak, I., & Wells, E. Adaptive strong-field control of vibrational population in NO2+. United States. https://doi.org/10.1063/1.5115504
Copy to clipboard
Voznyuk, O., Jochim, Bethany, Zohrabi, M., Broin, Adam, Averin, R., Carnes, K. D., Ben-Itzhak, I., and Wells, E. Sat . "Adaptive strong-field control of vibrational population in NO2+". United States. https://doi.org/10.1063/1.5115504. https://www.osti.gov/servlets/purl/1610039.
Copy to clipboard
@article{osti_1610039,
title = {Adaptive strong-field control of vibrational population in NO2+},
author = {Voznyuk, O. and Jochim, Bethany and Zohrabi, M. and Broin, Adam and Averin, R. and Carnes, K. D. and Ben-Itzhak, I. and Wells, E.},
abstractNote = {An adaptive closed-loop system employing coincidence time-of-flight feedback is used to determine the optimal pulse shapes for manipulating the branching ratio of NO dications following double ionization by an intense laser pulse. Selection between the long-lived NO2+ and the dissociative N+ + O+ final states requires control of the vibrational population distribution in the transient NO2+. The ability to both suppress and enhance NO2+ relative to N+ + O+ is observed, with the effectiveness of shaped pulses surpassing near Fourier transform-limited pulses by about an order of magnitude in each direction, depending on the pulse energy. The control is subsequently investigated using velocity map imaging, identifying plausible dissociation pathways leading to N+ + O+. Combining the information about the N+ + O+ dissociation with a well-defined control objective supports the conclusion that the primary control mechanism involves selectively populating long-lived NO2+ vibrational states.},
doi = {10.1063/1.5115504},
journal = {Journal of Chemical Physics},
number = 12,
volume = 151,
place = {United States},
year = {Sat Sep 28 00:00:00 EDT 2019},
month = {Sat Sep 28 00:00:00 EDT 2019}
}
Copy to clipboard
Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1063/1.5115504
Copyright Statement
Other availability
Search WorldCat Search WorldCat to find libraries that may hold this journal
Save / Share:
Export Metadata
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.

Works referenced in this record:

Non-sequential double ionization in slow charge fragmentation of doubly ionized NO
journal, September 2006

  • Wu, Jian; Zeng, H.; Guo, Chunlei
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 39, Issue 18
  • DOI: 10.1088/0953-4075/39/18/014

Femtosecond time-resolved molecular multiphoton ionization: The Na 2 system
journal, December 1991

Coherent control of molecular dynamics
journal, May 2003

Multicomponent control via shaped, strong laser fields mass spectrometry
journal, January 2008

  • Palliyaguru, Lalinda; Sloss, Joseph; Rabitz, Herschel
  • Journal of Modern Optics, Vol. 55, Issue 1
  • DOI: 10.1080/09500340701350239

Field ionization and Coulomb explosion of CO in an intense femtosecond laser field
journal, May 2003

  • Ren, Haizhen; Ma, Ri; Chen, Jianxin
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 36, Issue 11
  • DOI: 10.1088/0953-4075/36/11/304

Control of wavepacket dynamics in mixed alkali metal clusters by optimally shaped fs pulses
journal, October 2001

  • Bartelt, A.; Minemoto, S.; Lupulescu, C.
  • The European Physical Journal D, Vol. 16, Issue 1
  • DOI: 10.1007/s100530170076

Coherent control of the ultrafast dissociative ionization dynamics of bromochloroalkanes
journal, January 2011

  • Plenge, J.; Wirsing, A.; Wagner-Drebenstedt, I.
  • Physical Chemistry Chemical Physics, Vol. 13, Issue 19
  • DOI: 10.1039/c0cp02742a

Photoelectron and photofragment velocity map imaging of state-selected molecular oxygen dissociation/ionization dynamics
journal, August 1997

  • Parker, D. H.; Eppink, A. T. J. B.
  • The Journal of Chemical Physics, Vol. 107, Issue 7
  • DOI: 10.1063/1.474624

Selective Bond Dissociation and Rearrangement with Optimally Tailored, Strong-Field Laser Pulses
journal, March 2001

  • Levis, Robert J.; Menkir, Getahun M.; Rabitz, Herschel
  • Science, Vol. 292, Issue 5517, p. 709-713
  • DOI: 10.1126/science.1059133

Dynamic Stark Control of Photochemical Processes
journal, October 2006

Coulomb explosion of simple molecules in intense laser fields
journal, July 1994

Channel competition between metastable and dissociated states of doubly ionized NO in strong laser fields
journal, February 2005

Potential energy curves for NO +
journal, October 1979

  • Albritton, D. L.; Schmeltekopf, A. L.; Zare, R. N.
  • The Journal of Chemical Physics, Vol. 71, Issue 8
  • DOI: 10.1063/1.438757

Whither the Future of Controlling Quantum Phenomena?
journal, May 2000

Electron-ion correlations in strong-field molecular ionization with shaped ultrafast laser pulses
journal, January 2014

Two-dimensional charged particle image inversion using a polar basis function expansion
journal, November 2004

  • Garcia, Gustavo A.; Nahon, Laurent; Powis, Ivan
  • Review of Scientific Instruments, Vol. 75, Issue 11
  • DOI: 10.1063/1.1807578

Time‐of‐Flight Mass Spectrometer with Improved Resolution
journal, December 1955

  • Wiley, W. C.; McLaren, I. H.
  • Review of Scientific Instruments, Vol. 26, Issue 12
  • DOI: 10.1063/1.1715212

Control of Nuclear Dynamics with Strong Ultrashort Laser Pulses
journal, August 2012

  • Geißler, Dominik; Marquetand, Philipp; González-Vázquez, Jesús
  • The Journal of Physical Chemistry A, Vol. 116, Issue 46
  • DOI: 10.1021/jp306686n

Coincidence velocity map imaging using Tpx3Cam, a time stamping optical camera with 1.5 ns timing resolution
journal, November 2017

  • Zhao, Arthur; van Beuzekom, Martin; Bouwens, Bram
  • Review of Scientific Instruments, Vol. 88, Issue 11
  • DOI: 10.1063/1.4996888

Quantum control of energy flow in light harvesting
journal, May 2002

  • Herek, Jennifer L.; Wohlleben, Wendel; Cogdell, Richard J.
  • Nature, Vol. 417, Issue 6888, p. 533-535
  • DOI: 10.1038/417533a

Femtosecond-laser-induced alignment in Coulomb explosion of N 2
journal, January 2004

  • Miyazaki, Kenzo; Shimizu, Takayuki; Normand, Didier
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 37, Issue 4
  • DOI: 10.1088/0953-4075/37/4/003

Spatial alignment of diatomic molecules in intense laser fields: I. Experimental results
journal, November 2001

  • Rosca-Pruna, F.; Springate, E.; Offerhaus, H. L.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 34, Issue 23
  • DOI: 10.1088/0953-4075/34/23/332

Time-resolved organometallic photochemistry: Femtosecond fragmentation and adaptive control of CpFe(CO)2X (X=Cl, Br, I)
journal, November 2002

Frequency domain quantum optimal control under multiple constraints
journal, March 2016

Assessment of optimal control mechanism complexity by experimental landscape Hessian analysis: fragmentation of CH 2 BrI
journal, December 2014

Observation of selective charge separation following strong-field single ionization
journal, February 2005

Ion-ion coincidence imaging at high event rate using an in-vacuum pixel detector
journal, July 2017

  • Furch, Federico J.; Durá, Judith; Tremsin, Anton S.
  • The Journal of Chemical Physics, Vol. 147, Issue 1
  • DOI: 10.1063/1.4981126

Control of Chemical Reactions by Feedback-Optimized Phase-Shaped Femtosecond Laser Pulses
journal, October 1998

Closing the Loop on Bond Selective Chemistry Using Tailored Strong Field Laser Pulses
journal, July 2002

  • Levis, R. J.; Rabitz, H. A.
  • The Journal of Physical Chemistry A, Vol. 106, Issue 27, p. 6427-6444
  • DOI: 10.1021/jp0134906

Closed Loop Coherent Control of Electronic Transitions in Gallium Arsenide
journal, June 2011

  • Singha, Sima; Hu, Zhan; Gordon, Robert J.
  • The Journal of Physical Chemistry A, Vol. 115, Issue 23
  • DOI: 10.1021/jp110869f

Mapping Excited-State Dynamics by Coherent Control of a Dendrimer's Photoemission Efficiency
journal, October 2009

Adaptive strong-field control of chemical dynamics guided by three-dimensional momentum imaging
journal, December 2013

  • Wells, E.; Rallis, C. E.; Zohrabi, M.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3895

The effect of control field and measurement imprecision on laboratory feedback control of quantum systems
journal, September 1994

  • Tóth, Gábor J.; Lőrincz, András; Rabitz, Herschel
  • The Journal of Chemical Physics, Vol. 101, Issue 5
  • DOI: 10.1063/1.467555

Post ionization alignment of the fragmentation of molecules in an ultrashort intense laser field
journal, February 2005

  • Tong, X. M.; Zhao, Z. X.; Alnaser, A. S.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 38, Issue 4
  • DOI: 10.1088/0953-4075/38/4/002

Sub-laser-cycle electron pulses for probing molecular dynamics
journal, June 2002

  • Niikura, Hiromichi; Légaré, F.; Hasbani, R.
  • Nature, Vol. 417, Issue 6892
  • DOI: 10.1038/nature00787

Multiphoton ionisation of H 2 and D 2 using an intense sub-picosecond laser
journal, August 1988

  • Codling, K.; Frasinski, L. J.; Hatherly, P. A.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 21, Issue 15
  • DOI: 10.1088/0953-4075/21/15/003

Velocity map imaging as a tool for gaining mechanistic insight from closed-loop control studies of molecular fragmentation
journal, April 2011

Two‐dimensional imaging of state‐selected photodissociation products detected by multiphoton ionization
journal, July 1987

  • Chandler, David W.; Houston, Paul L.
  • The Journal of Chemical Physics, Vol. 87, Issue 2
  • DOI: 10.1063/1.453276

Ab initio potential energy curves of Rydberg, valence and continuum states of NO
journal, April 1997

  • Rabadán, Ismanuel; Tennyson, Jonathan
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 30, Issue 8
  • DOI: 10.1088/0953-4075/30/8/014

Dissociative ionization of NO in an intense laser field: a route towards enhanced ionization
journal, April 1997

  • Talebpour, A.; Larochelle, S.; Chin, S. L.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 30, Issue 8
  • DOI: 10.1088/0953-4075/30/8/010

Why is chemical synthesis and property optimization easier than expected?
journal, January 2011

  • Moore, Katharine W.; Pechen, Alexander; Feng, Xiao-Jiang
  • Physical Chemistry Chemical Physics, Vol. 13, Issue 21
  • DOI: 10.1039/c1cp20353c

Triple-ionization-induced dissociation of NO in strong laser fields
journal, September 2006

Closed-loop control of intense-laser fragmentation of S 8
journal, December 2005

Sur les équations différentielles linéaires à coefficients périodiques
journal, January 1883

  • Floquet, G.
  • Annales scientifiques de l'École normale supérieure, Vol. 12
  • DOI: 10.24033/asens.220

Dynamic and geometric laser-induced alignment of molecules in intense laser fields
journal, July 1998

  • Posthumus, J. H.; Plumridge, J.; Thomas, M. K.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 31, Issue 13
  • DOI: 10.1088/0953-4075/31/13/002

Light-induced multiple electronic-state coupling of O2+ in intense laser fields
journal, June 2001

  • Hishikawa, Akiyoshi; Liu, Shilin; Iwasaki, Atsushi
  • The Journal of Chemical Physics, Vol. 114, Issue 22
  • DOI: 10.1063/1.1368383

Multimass Velocity-Map Imaging with the Pixel Imaging Mass Spectrometry (PImMS) Sensor: An Ultra-Fast Event-Triggered Camera for Particle Imaging
journal, November 2012

  • Clark, Andrew T.; Crooks, Jamie P.; Sedgwick, Iain
  • The Journal of Physical Chemistry A, Vol. 116, Issue 45
  • DOI: 10.1021/jp309860t

Coherent strong-field control of multiple states by a single chirped femtosecond laser pulse
journal, October 2009

Enhanced ionization of the molecular ion H 2 + in intense laser and static magnetic fields
journal, October 2000

On the field ionisation of diatomic molecules by intense laser fields
journal, June 1989

  • Codling, K.; Frasinski, L. J.; Hatherly, P. A.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 22, Issue 12
  • DOI: 10.1088/0953-4075/22/12/004

Control of quantum phenomena: past, present and future
journal, July 2010

An iterative procedure for the inversion of two-dimensional ion/photoelectron imaging experiments
journal, November 2001

  • Vrakking, Marc J. J.
  • Review of Scientific Instruments, Vol. 72, Issue 11
  • DOI: 10.1063/1.1406923

Strong field molecular ionization to multiple ionic states: direct versus indirect pathways
journal, June 2014

  • Sándor, Péter; Zhao, Arthur; Rozgonyi, Tamás
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 47, Issue 12
  • DOI: 10.1088/0953-4075/47/12/124021

Closed-loop control of vibrational population in CO 2+
journal, December 2009

  • Wells, E.; McKenna, J.; Sayler, A. M.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 43, Issue 1
  • DOI: 10.1088/0953-4075/43/1/015101

Field-assisted bond stretching of CO in intense laser fields
journal, April 2009

Ellipticity effects on nonsequential double ionization of diatomic molecules in strong laser fields
journal, September 2005

Active control of product selection in a chemical reaction a view of the current scene
journal, April 2002

  • Rice, Stuart A.; Shah, Suhail P.
  • Physical Chemistry Chemical Physics, Vol. 4, Issue 10, p. 1683-1700
  • DOI: 10.1039/b109911f

Molecular fragmentation driven by ultrafast dynamic ionic resonances
journal, October 2007

  • Pearson, Brett J.; Nichols, Sarah R.; Weinacht, Thomas
  • The Journal of Chemical Physics, Vol. 127, Issue 13
  • DOI: 10.1063/1.2790419

Photoionization and photodissociation dynamics of H2 after (3+1) resonance-enhanced multiphoton ionization via the B 1Σu+ state
journal, November 1998

  • Scheper, C. R.; Buma, W. J.; de Lange, C. A.
  • The Journal of Chemical Physics, Vol. 109, Issue 19
  • DOI: 10.1063/1.477495

Femtosecond pulse shaping using spatial light modulators
journal, May 2000

  • Weiner, A. M.
  • Review of Scientific Instruments, Vol. 71, Issue 5, p. 1929-1960
  • DOI: 10.1063/1.1150614

Transition from weak- to strong-field coherent control
journal, June 2007

Adaptive control of the C O 2 bending vibration: Deciphering field-system dynamics
journal, January 2009

Thick-lens velocity-map imaging spectrometer with high resolution for high-energy charged particles
journal, May 2014

Routes to Control of H 2 Coulomb Explosion in Few-Cycle Laser Pulses
journal, October 2004

Phase control of molecular ionization: H 2 + and H 3 2 + in intense two-color laser fields
journal, October 1996

Incorporating real time velocity map image reconstruction into closed-loop coherent control
journal, November 2014

  • Rallis, C. E.; Burwitz, T. G.; Andrews, P. R.
  • Review of Scientific Instruments, Vol. 85, Issue 11
  • DOI: 10.1063/1.4899267

Fast closed-loop optimal control of ultracold atoms in an optical lattice
journal, August 2013

Quantum Optimally Controlled Transition Landscapes
journal, March 2004

Closed-loop learning control of isomerization using shaped ultrafast laser pulses in the deep ultraviolet
journal, April 2009

  • Kotur, Marija; Weinacht, Thomas; Pearson, Brett J.
  • The Journal of Chemical Physics, Vol. 130, Issue 13
  • DOI: 10.1063/1.3103486

Examining the feedback signals used in closed-loop control of intense laser fragmentation of CO +
journal, December 2009

Ab initio potential energy curves of Rydberg, valence and continuum states of NO
journal, October 1998

  • Rabadán, I.; Tennyson, J.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 31, Issue 19
  • DOI: 10.1088/0953-4075/31/19/031

Coherent control of bond breaking in amino acid complexes with tailored femtosecond pulses
journal, November 2007

  • Laarmann, T.; Shchatsinin, I.; Singh, P.
  • The Journal of Chemical Physics, Vol. 127, Issue 20
  • DOI: 10.1063/1.2806029

High resolution kinetic energy release spectra and angular distributions from double ionization of nitrogen and oxygen by short laser pulses
journal, October 2004

  • Voss, S.; Alnaser, A. S.; Tong, X-M
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 37, Issue 21
  • DOI: 10.1088/0953-4075/37/21/002

Control of bond-selective photochemistry in CH $\scriptstyle \mathsf {2}$ BrCl using adaptive femtosecond pulse shaping
journal, July 2002

  • Damrauer, N. H.; Dietl, C.; Krampert, G.
  • The European Physical Journal D - Atomic, Molecular and Optical Physics, Vol. 20, Issue 1
  • DOI: 10.1140/epjd/e2002-00101-8

Isotope Selective Ionization by Optimal Control Using Shaped Femtosecond Laser Pulses
journal, July 2004

Coherent Control of the Photoionization of Pyrazine
journal, September 2012

  • Hu, Zhan; Singha, Sima; Zhao, Youbo
  • The Journal of Physical Chemistry Letters, Vol. 3, Issue 19
  • DOI: 10.1021/jz301144q

General Method for the Dimension Reduction of Adaptive Control Experiments
journal, May 2006

  • Montgomery, Matthew A.; Meglen, Robert R.; Damrauer, Niels H.
  • The Journal of Physical Chemistry A, Vol. 110, Issue 20
  • DOI: 10.1021/jp061160l

Phase Dependence of Enhanced Ionization in Asymmetric Molecules
journal, May 2005

Ultrafast ionization study of N 2 in intense linearly and circularly polarized laser fields
journal, April 2006

Coincidence velocity map imaging using a single detector
journal, July 2017

  • Zhao, Arthur; Sándor, Péter; Weinacht, Thomas
  • The Journal of Chemical Physics, Vol. 147, Issue 1
  • DOI: 10.1063/1.4981917

Gaining Mechanistic Insight with Control Pulse Slicing: Application to the Dissociative Ionization of CH 2 BrI
journal, November 2017

  • Xing, Xi; Rey-de-Castro, Roberto; Rabitz, Herschel
  • The Journal of Physical Chemistry A, Vol. 121, Issue 45
  • DOI: 10.1021/acs.jpca.7b08835

Controlling the Femtochemistry of Fe(CO)5
journal, December 1999

  • Bergt, M.; Brixner, T.; Kiefer, B.
  • The Journal of Physical Chemistry A, Vol. 103, Issue 49, p. 10381-10387
  • DOI: 10.1021/jp992541k

Transformations to diagonal bases in closed-loop quantum learning control experiments
journal, March 2005

  • Cardoza, David; Trallero-Herrero, Carlos; Langhojer, Florian
  • The Journal of Chemical Physics, Vol. 122, Issue 12
  • DOI: 10.1063/1.1867334

Nonsymmetric molecules driven by intense few-cycle laser pulses: Phase and orientation dependence of enhanced ionization
journal, November 2007

The dissociation dynamics of diatomic molecules in intense laser fields
journal, July 1996

  • Posthumus, J. H.; Giles, A. J.; Thompson, M. R.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 29, Issue 14
  • DOI: 10.1088/0953-4075/29/14/004

Exploring wavepacket dynamics behind strong-field momentum-dependent photodissociation in CH2BrI+
journal, January 2010

  • González-Vázquez, Jesús; González, Leticia; Nichols, Sarah R.
  • Physical Chemistry Chemical Physics, Vol. 12, Issue 42
  • DOI: 10.1039/c0cp00303d

Strong-field control landscapes of coherent electronic excitation
journal, March 2008

  • Bayer, Tim; Wollenhaupt, Matthias; Baumert, Thomas
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 41, Issue 7
  • DOI: 10.1088/0953-4075/41/7/074007

Charge-transfer as a mechanism for controlling molecular fragmentation
journal, June 2006

  • Cardoza, David; Pearson, Brett J.; Baertschy, Mark
  • Journal of Photochemistry and Photobiology A: Chemistry, Vol. 180, Issue 3
  • DOI: 10.1016/j.jphotochem.2006.02.007

Two-step Coulomb explosions of diatoms in intense laser fields
journal, December 1995

  • Chelkowski, S.; Bandrauk, A. D.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 28, Issue 23
  • DOI: 10.1088/0953-4075/28/23/004

Coherent control of strong field multiphoton absorption in the presence of dynamic Stark shifts
journal, January 2005

Extracting quantum dynamics from genetic learning algorithms through principal control analysis
journal, December 2004

  • White, J. L.; Pearson, B. J.; Bucksbaum, P. H.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 37, Issue 24
  • DOI: 10.1088/0953-4075/37/24/l02

Computed lifetimes of metastable states of the NO2+ dication
journal, April 2008

  • Baková, R.; Fišer, J.; Šedivcová-Uhlíková, T.
  • The Journal of Chemical Physics, Vol. 128, Issue 14
  • DOI: 10.1063/1.2898495

Publisher’s Note: Rescattering Double Ionization of D 2 and H 2 by Intense Laser Pulses [Phys. Rev. Lett. 91 , 163002 (2003)]
journal, November 2003

Enhanced ionization of molecular hydrogen in very strong fields
journal, April 2000

Velocity map imaging of ions and electrons using electrostatic lenses: Application in photoelectron and photofragment ion imaging of molecular oxygen
journal, September 1997

  • Eppink, André T. J. B.; Parker, David H.
  • Review of Scientific Instruments, Vol. 68, Issue 9
  • DOI: 10.1063/1.1148310

Deciphering the Reaction Dynamics Underlying Optimal Control Laser Fields
journal, January 2003

  • Daniel, Chantal; Full, Jurgen; Gonzalez, Leticia
  • Science, Vol. 299, Issue 5606, p. 536-539
  • DOI: 10.1126/science.1078517

Gaining mechanistic insight from closed loop learning control: The importance of basis in searching the phase space
journal, January 2005

  • Langhojer, Florian; Cardoza, David; Baertschy, Mark
  • The Journal of Chemical Physics, Vol. 122, Issue 1
  • DOI: 10.1063/1.1826011

Recoil-ion and electron momentum spectroscopy: reaction-microscopes
journal, August 2003

Extracting Information from Adaptive Control Experiments
journal, March 2012

  • White, James L.; Carroll, Elizabeth C.; Spears, Kenneth G.
  • Israel Journal of Chemistry, Vol. 52, Issue 5
  • DOI: 10.1002/ijch.201100106

Rotational dynamics of dissociating H + 2 in a short intense laser pulse
journal, April 2009

  • Anis, Fatima; Cackowski, Ted; Esry, B. D.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 42, Issue 9
  • DOI: 10.1088/0953-4075/42/9/091001

Time-resolved quantum process tomography using Hamiltonian-encoding and observable-decoding
journal, February 2013

A newcomer's guide to ultrashort pulse shaping and characterization
journal, May 2010

  • Monmayrant, Antoine; Weber, Sébastien; Chatel, Béatrice
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 43, Issue 10
  • DOI: 10.1088/0953-4075/43/10/103001

Toward real-time charged-particle image reconstruction using polar onion-peeling
journal, May 2009

  • Roberts, G. M.; Nixon, J. L.; Lecointre, J.
  • Review of Scientific Instruments, Vol. 80, Issue 5
  • DOI: 10.1063/1.3126527

Control of quantum phenomena: Past, present, and future
text, January 2009

Fast closed-loop optimal control of ultracold atoms in an optical lattice
text, January 2013

    Sort by:
    [ × clear filter / sort ]

    Similar Records in DOE PAGES and OSTI.GOV collections: