Magnetic properties of the lowdimensional $\mathrm{Ba}{M}_{2}{\mathrm{Si}}_{2}{\mathrm{O}}_{7}$ system $(M=\mathrm{Cu},\mathrm{Co},\mathrm{Mn})$
Abstract
Here, we explored the magnetic properties of the lowdimensional $\mathrm{Ba}{M}_{2}{\mathrm{Si}}_{2}{\mathrm{O}}_{7}$ (M = Cu, Co, and Mn) system using both experimental measurements and theoretical calculations. Magnetization, specific heat, and single crystal neutron diffraction measurements have been performed on single crystal $\mathrm{Ba}{M}_{2}{\mathrm{Si}}_{2}{\mathrm{O}}_{7}$. The spin structure was determined and a magnetic phase diagram with applied field along the b axis was constructed, which contains a spin flop transition around 6 T. Magnetization and specific heat measurements confirmed the presence of weak ferromagnetism in $\mathrm{Ba}{M}_{2}{\mathrm{Si}}_{2}{\mathrm{O}}_{7}$. Furthermore, we performed localspin density approximation with onsite Coulomb energy (LSDA+U) calculations for the $\mathrm{Ba}{M}_{2}{\mathrm{Si}}_{2}{\mathrm{O}}_{7}$ (M = Cu, Co, and Mn) system. Due to the firstprinciples calculations, the origin of the magnetic differences of the three materials is discussed.
 Authors:

 Shanghai Jiao Tong Univ. (China)
 Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
 Univ. of Tennessee, Knoxville, TN (United States)
 Shanghai Jiao Tong Univ. (China); Univ. of Tennessee, Knoxville, TN (United States)
 Shanghai Jiao Tong Univ. (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China)
 Publication Date:
 Research Org.:
 Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
 Sponsoring Org.:
 USDOE; National Natural Science Foundation of China (NSFC)
 OSTI Identifier:
 1566966
 Alternate Identifier(s):
 OSTI ID: 1545457
 Grant/Contract Number:
 AC0500OR22725
 Resource Type:
 Accepted Manuscript
 Journal Name:
 Physical Review B
 Additional Journal Information:
 Journal Volume: 100; Journal Issue: 3; Journal ID: ISSN 24699950
 Publisher:
 American Physical Society (APS)
 Country of Publication:
 United States
 Language:
 English
 Subject:
 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Wang, G. H., Xu, C. Y., Cao, Huibo, Hong, Tao, Huang, Q., Ren, Q. Y., Xu, J. Q., Zhou, Haidong, Luo, W., Qian, D., and Ma, J. Magnetic properties of the lowdimensional BaM2Si2O7 system (M=Cu, Co, Mn). United States: N. p., 2019.
Web. doi:10.1103/PhysRevB.100.035131.
Wang, G. H., Xu, C. Y., Cao, Huibo, Hong, Tao, Huang, Q., Ren, Q. Y., Xu, J. Q., Zhou, Haidong, Luo, W., Qian, D., & Ma, J. Magnetic properties of the lowdimensional BaM2Si2O7 system (M=Cu, Co, Mn). United States. https://doi.org/10.1103/PhysRevB.100.035131
Wang, G. H., Xu, C. Y., Cao, Huibo, Hong, Tao, Huang, Q., Ren, Q. Y., Xu, J. Q., Zhou, Haidong, Luo, W., Qian, D., and Ma, J. Fri .
"Magnetic properties of the lowdimensional BaM2Si2O7 system (M=Cu, Co, Mn)". United States. https://doi.org/10.1103/PhysRevB.100.035131. https://www.osti.gov/servlets/purl/1566966.
@article{osti_1566966,
title = {Magnetic properties of the lowdimensional BaM2Si2O7 system (M=Cu, Co, Mn)},
author = {Wang, G. H. and Xu, C. Y. and Cao, Huibo and Hong, Tao and Huang, Q. and Ren, Q. Y. and Xu, J. Q. and Zhou, Haidong and Luo, W. and Qian, D. and Ma, J.},
abstractNote = {Here, we explored the magnetic properties of the lowdimensional BaM2Si2O7 (M = Cu, Co, and Mn) system using both experimental measurements and theoretical calculations. Magnetization, specific heat, and single crystal neutron diffraction measurements have been performed on single crystal BaM2Si2O7. The spin structure was determined and a magnetic phase diagram with applied field along the b axis was constructed, which contains a spin flop transition around 6 T. Magnetization and specific heat measurements confirmed the presence of weak ferromagnetism in BaM2Si2O7. Furthermore, we performed localspin density approximation with onsite Coulomb energy (LSDA+U) calculations for the BaM2Si2O7 (M = Cu, Co, and Mn) system. Due to the firstprinciples calculations, the origin of the magnetic differences of the three materials is discussed.},
doi = {10.1103/PhysRevB.100.035131},
journal = {Physical Review B},
number = 3,
volume = 100,
place = {United States},
year = {2019},
month = {7}
}
Web of Science
Figures / Tables:
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