How lasing happens in CsPbBr3 perovskite nanowires

Schlaus, Andrew P.; Spencer, Michael S.; Miyata, Kiyoshi; Liu, Fang; Wang, Xiaoxia; Datta, Ipshita; Lipson, Michal; Pan, Anlian; Zhu, X. -Y.

doi:10.1038/s41467-018-07972-7

Title: How lasing happens in CsPbBr₃ perovskite nanowires

Abstract

Lead halide perovskites are emerging as an excellent material platform for optoelectronic processes. There have been extensive discussions on lasing, polariton formation, and nonlinear processes in this material system, but the underlying mechanism remains unknown. Here we probe lasing from CsPbBr₃ perovskite nanowires with picosecond (ps) time resolution and show that lasing originates from stimulated emission of an electron-hole plasma. We observe an anomalous blue-shifting of the lasing gain profile with time up to 25 ps, and assign this as a signature for lasing involving plasmon emission. The time domain view provides an ultra-sensitive probe of many-body physics which was obscured in previous time-integrated measurements of lasing from lead halide perovskite nanowires.

Authors:

Schlaus, Andrew P. ^[1]; Spencer, Michael S. ^[1];

^[1]; Liu, Fang ^[1]; Wang, Xiaoxia ^[2];

^[1]; Lipson, Michal ^[1]; Pan, Anlian ^[2]; Zhu, X. -Y. ^[1]

Columbia Univ., New York, NY (United States)
Hunan Univ., Changsha (China)

Publication Date:: 2019-01-16

Research Org.:: Energy Frontier Research Centers (EFRC) (United States). Programmable Quantum Materials (Pro-QM); Columbia Univ., New York, NY (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Natural Science Foundation of China (NSFC)

OSTI Identifier:: 1566607

Grant/Contract Number:: SC0010692; SC0019443

Resource Type:: Accepted Manuscript

Journal Name:: Nature Communications

Additional Journal Information:: Journal Volume: 10; Journal Issue: 1; Journal ID: ISSN 2041-1723

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; optics; defects; charge transport; superconductivity; magnetism and spin physics; mesoscale science; materials and chemistry by design; mesostructured materials; synthesis (novel materials); synthesis (self-assembly)

Citation Formats


                    Schlaus, Andrew P., Spencer, Michael S., Miyata, Kiyoshi, Liu, Fang, Wang, Xiaoxia, Datta, Ipshita, Lipson, Michal, Pan, Anlian, and Zhu, X. -Y. How lasing happens in CsPbBr3 perovskite nanowires.  United States: N. p., 2019. 
Web.  doi:10.1038/s41467-018-07972-7.

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                    Schlaus, Andrew P., Spencer, Michael S., Miyata, Kiyoshi, Liu, Fang, Wang, Xiaoxia, Datta, Ipshita, Lipson, Michal, Pan, Anlian, & Zhu, X. -Y. How lasing happens in CsPbBr3 perovskite nanowires.  United States.  https://doi.org/10.1038/s41467-018-07972-7

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                    Schlaus, Andrew P., Spencer, Michael S., Miyata, Kiyoshi, Liu, Fang, Wang, Xiaoxia, Datta, Ipshita, Lipson, Michal, Pan, Anlian, and Zhu, X. -Y. Wed .  
"How lasing happens in CsPbBr3 perovskite nanowires".  United States.  https://doi.org/10.1038/s41467-018-07972-7.  https://www.osti.gov/servlets/purl/1566607.

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@article{osti_1566607,

  title        = {How lasing happens in CsPbBr3 perovskite nanowires},

  author       = {Schlaus, Andrew P. and Spencer, Michael S. and Miyata, Kiyoshi and Liu, Fang and Wang, Xiaoxia and Datta, Ipshita and Lipson, Michal and Pan, Anlian and Zhu, X. -Y.},

  abstractNote = {Lead halide perovskites are emerging as an excellent material platform for optoelectronic processes. There have been extensive discussions on lasing, polariton formation, and nonlinear processes in this material system, but the underlying mechanism remains unknown. Here we probe lasing from CsPbBr3 perovskite nanowires with picosecond (ps) time resolution and show that lasing originates from stimulated emission of an electron-hole plasma. We observe an anomalous blue-shifting of the lasing gain profile with time up to 25 ps, and assign this as a signature for lasing involving plasmon emission. The time domain view provides an ultra-sensitive probe of many-body physics which was obscured in previous time-integrated measurements of lasing from lead halide perovskite nanowires.},

  doi          = {10.1038/s41467-018-07972-7},

  journal      = {Nature Communications},

  number       = 1,

  volume       = 10,

  place        = {United States},

  year         = {2019},

  month        = {1}

}

Copy to clipboard

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Title: How lasing happens in CsPbBr3 perovskite nanowires

Abstract

Citation Formats

Hot-carrier cooling and photoinduced refractive index changes in organic–inorganic lead halide perovskites journal, September 2015

Tunable polariton absorption of distributed feedback microcavities at room temperature journal, May 1998

Light–Matter Interactions in Cesium Lead Halide Perovskite Nanowire Lasers journal, September 2016

Experimental Demonstration of Correlated Flux Scaling in Photoconductivity and Photoluminescence of Lead-Halide Perovskites journal, November 2018

Continuous-Wave Lasing in Cesium Lead Bromide Perovskite Nanowires journal, December 2017

Semiconductor excitons in new light journal, July 2006

Room-Temperature Polariton Lasing in All-Inorganic Perovskite Nanoplatelets journal, May 2017

Metal halide perovskites for energy applications journal, May 2016

Review on the dynamics of semiconductor nanowire lasers journal, February 2018

Ultrafast carrier thermalization in lead iodide perovskite probed with two-dimensional electronic spectroscopy journal, August 2017

UV polaritonic emission from a perovskite-based microcavity journal, August 2008

65 years of ZnO research - old and very recent results journal, April 2010

Correlated electron–hole plasma in organometal perovskites journal, September 2014

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Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors journal, April 2015

Entropy in halide perovskites journal, April 2018

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Dispersion and line shape of plasmon satellites in one, two, and three dimensions journal, June 2016

Low surface recombination velocity in solution-grown CH3NH3PbBr3 perovskite single crystal journal, August 2015

Nanowire Lasers of Formamidinium Lead Halide Perovskites and Their Stabilized Alloys with Improved Stability journal, January 2016

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Lead halide perovskites: Crystal-liquid duality, phonon glass electron crystals, and large polaron formation journal, October 2017

Quantum confinement of zero-dimensional hybrid organic-inorganic polaritons at room temperature journal, February 2014

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Room-temperature stimulated emission of ZnO: Alternatives to excitonic lasing journal, March 2007

Perovskite photonic sources journal, April 2016

Ultrafast screening and carrier dynamics in ZnO: Theory and experiment journal, July 2011

Ferroelectric large polarons journal, April 2018

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ZnO: Material, Physics and Applications journal, April 2007

Determination of the exciton binding energy and effective masses for methylammonium and formamidinium lead tri-halide perovskite semiconductors journal, January 2016

Carrier density driven lasing dynamics in ZnO nanowires journal, April 2016

Perovskite Materials for Light-Emitting Diodes and Lasers journal, May 2016

Hot carrier cooling mechanisms in halide perovskites journal, November 2017

Observation of a hot-phonon bottleneck in lead-iodide perovskites journal, October 2015

Directional Growth of Ultralong CsPbBr 3 Perovskite Nanowires for High-Performance Photodetectors journal, October 2017

Lead halide perovskites: Crystal-liquid duality, phonon glass electron crystals, and large polaron formation text, January 2017

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Ultrafast screening and carrier dynamics in ZnO: Theory and experiment text, January 2010

Quantum confinement of zero-dimensional hybrid organic-inorganic polaritons at room temperature text, January 2014

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Dispersion and lineshape of plasmon satellites in one, two and three dimensions text, January 2016

High‐Order Shift Current Induced Terahertz Emission from Inorganic Cesium Bromine Lead Perovskite Engendered by Two‐Photon Absorption journal, August 2019

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Title: How lasing happens in CsPbBr₃ perovskite nanowires

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journal, September 2015

Tunable polariton absorption of distributed feedback microcavities at room temperature
journal, May 1998

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journal, July 2006

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Review on the dynamics of semiconductor nanowire lasers
journal, February 2018

Ultrafast carrier thermalization in lead iodide perovskite probed with two-dimensional electronic spectroscopy
journal, August 2017

UV polaritonic emission from a perovskite-based microcavity
journal, August 2008

65 years of ZnO research - old and very recent results
journal, April 2010

Correlated electron–hole plasma in organometal perovskites
journal, September 2014

Bright triplet excitons in caesium lead halide perovskites
journal, January 2018

Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors
journal, April 2015

Entropy in halide perovskites
journal, April 2018

Lasing in robust cesium lead halide perovskite nanowires
journal, February 2016

Dispersion and line shape of plasmon satellites in one, two, and three dimensions
journal, June 2016

Low surface recombination velocity in solution-grown CH3NH3PbBr3 perovskite single crystal
journal, August 2015

Nanowire Lasers of Formamidinium Lead Halide Perovskites and Their Stabilized Alloys with Improved Stability
journal, January 2016

Slow hot carrier cooling in cesium lead iodide perovskites
journal, October 2017

Screening in crystalline liquids protects energetic carriers in hybrid perovskites
journal, September 2016

Lead halide perovskites: Crystal-liquid duality, phonon glass electron crystals, and large polaron formation
journal, October 2017

Quantum confinement of zero-dimensional hybrid organic-inorganic polaritons at room temperature
journal, February 2014

Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites
journal, January 2017

Broad Wavelength Tunable Robust Lasing from Single-Crystal Nanowires of Cesium Lead Halide Perovskites (CsPbX ₃ , X = Cl, Br, I)
journal, July 2016

Organic Cations Might Not Be Essential to the Remarkable Properties of Band Edge Carriers in Lead Halide Perovskites
journal, October 2016

Room-temperature stimulated emission of ZnO: Alternatives to excitonic lasing
journal, March 2007

Perovskite photonic sources
journal, April 2016

Ultrafast screening and carrier dynamics in ZnO: Theory and experiment
journal, July 2011

Ferroelectric large polarons
journal, April 2018

Impact of the Halide Cage on the Electronic Properties of Fully Inorganic Cesium Lead Halide Perovskites
journal, June 2017

ZnO: Material, Physics and Applications
journal, April 2007

Determination of the exciton binding energy and effective masses for methylammonium and formamidinium lead tri-halide perovskite semiconductors
journal, January 2016

Carrier density driven lasing dynamics in ZnO nanowires
journal, April 2016

Perovskite Materials for Light-Emitting Diodes and Lasers
journal, May 2016

Hot carrier cooling mechanisms in halide perovskites
journal, November 2017

Observation of a hot-phonon bottleneck in lead-iodide perovskites
journal, October 2015

Directional Growth of Ultralong CsPbBr ₃ Perovskite Nanowires for High-Performance Photodetectors
journal, October 2017

Lead halide perovskites: Crystal-liquid duality, phonon glass electron crystals, and large polaron formation
text, January 2017

Ultrafast carrier thermalization in lead iodide perovskite probed with two-dimensional electronic spectroscopy
text, January 2017

Ultrafast screening and carrier dynamics in ZnO: Theory and experiment
text, January 2010

Quantum confinement of zero-dimensional hybrid organic-inorganic polaritons at room temperature
text, January 2014

Carrier density driven lasing dynamics in ZnO nanowires
text, January 2016

Dispersion and lineshape of plasmon satellites in one, two and three dimensions
text, January 2016

High‐Order Shift Current Induced Terahertz Emission from Inorganic Cesium Bromine Lead Perovskite Engendered by Two‐Photon Absorption
journal, August 2019

Single‐Crystalline Perovskite Microlasers for High‐Contrast and Sub‐Diffraction Imaging
journal, July 2019

Continuous‐Wave Pumped Perovskite Lasers
journal, June 2019

Structure and optical properties of perovskite-embedded dual-phase microcrystals synthesized by sonochemistry
journal, February 2020

Amplified spontaneous emission and random lasing using CsPbBr ₃ quantum dot glass through controlling crystallization
journal, January 2020

Active meta-optics and nanophotonics with halide perovskites
journal, September 2019

Lasing from reduced dimensional perovskite microplatelets: Fabry-Pérot or whispering-gallery-mode?
journal, December 2019

Lead-Free Perovskites for Lighting and Lasing Applications: A Minireview
journal, November 2019

Active meta-optics and nanophotonics with halide perovskites
preprint, January 2019