How lasing happens in CsPbBr3 perovskite nanowires

Schlaus, Andrew P.; Spencer, Michael S.; Miyata, Kiyoshi; Liu, Fang; Wang, Xiaoxia; Datta, Ipshita; Lipson, Michal; Pan, Anlian; Zhu, X. -Y.

doi:10.1038/s41467-018-07972-7

Title: How lasing happens in CsPbBr₃ perovskite nanowires

Journal Article · 15 January 2019 · Nature Communications

DOI: https://doi.org/10.1038/s41467-018-07972-7 · OSTI ID:1566607

Schlaus, Andrew P. ^[1]; Spencer, Michael S. ^[1];

^[1]; Liu, Fang ^[1]; Wang, Xiaoxia ^[2];

^[1]; Lipson, Michal ^[1]; Pan, Anlian ^[2]; Zhu, X. -Y. ^[1]

Columbia Univ., New York, NY (United States)
Hunan Univ., Changsha (China)

Lead halide perovskites are emerging as an excellent material platform for optoelectronic processes. There have been extensive discussions on lasing, polariton formation, and nonlinear processes in this material system, but the underlying mechanism remains unknown. Here we probe lasing from CsPbBr₃ perovskite nanowires with picosecond (ps) time resolution and show that lasing originates from stimulated emission of an electron-hole plasma. We observe an anomalous blue-shifting of the lasing gain profile with time up to 25 ps, and assign this as a signature for lasing involving plasmon emission. The time domain view provides an ultra-sensitive probe of many-body physics which was obscured in previous time-integrated measurements of lasing from lead halide perovskite nanowires.

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Research Organization:: Columbia Univ., New York, NY (United States); Energy Frontier Research Centers (EFRC) (United States). Programmable Quantum Materials (Pro-QM)

Sponsoring Organization:: National Natural Science Foundation of China (NNSFC); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: SC0010692; SC0019443

OSTI ID:: 1566607

Journal Information:: Nature Communications, Journal Name: Nature Communications Journal Issue: 1 Vol. 10; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Title: How lasing happens in CsPbBr3 perovskite nanowires

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Title: How lasing happens in CsPbBr₃ perovskite nanowires