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Title: Strain tuning of excitons in monolayer WSe 2

Journal Article · · Physical Review B
 [1];  [1];  [1]
  1. Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)

We investigate excitonic absorption and emission in monolayer (1L) WSe2 under tensile strain. We observe a redshift of 100 meV in the A exciton energy and a decrease of 25 meV in its estimated binding energy under 2.1% strain. Surprisingly, the linewidth of the A exciton decreases by almost a factor of two under strain, from 42 to 24 meV at room temperature. We explain this effect as the result of suppression of phonon-mediated exciton scattering channels. Here, we show that such a suppression results from the relative shift under strain of a secondary valley in the conduction band that is nearly degenerate with the K valley where the A exciton is formed.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Stanford Univ., CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
DMR-1420634; AC02-76SF00515
OSTI ID:
1562880
Alternate ID(s):
OSTI ID: 1474105; OSTI ID: 1474195
Journal Information:
Physical Review B, Vol. 98, Issue 11; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 114 works
Citation information provided by
Web of Science

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Cited By (6)

Dielectric disorder in two-dimensional materials journal August 2019
Intrinsic lifetime of higher excitonic states in tungsten diselenide monolayers journal January 2019
Strain-tunable orbital, spin-orbit, and optical properties of monolayer transition-metal dichalcogenides journal November 2019
Exciton control in a room temperature bulk semiconductor with coherent strain pulses journal November 2019
Strain-tunable orbital, spin-orbit, and optical properties of monolayer transition-metal dichalcogenides text January 2019
Intrinsic Lifetime of Higher Excitonic States in Tungsten Diselenide Monolayers text January 2019

Figures / Tables (3)