Evolution of charge order topology across a magnetic phase transition in cuprate superconductors
Abstract
Charge order is now accepted as an integral constituent of cuprate high-temperature superconductors, one that is intimately related to other electronic instabilities including antiferromagnetism and superconductivity. Unlike conventional Peierls density waves, the charge correlations in cuprates have been predicted to display a rich momentum space topology depending on the underlying fermiology. However, charge order has only been observed along the high-symmetry Cu–O bond directions. Here, using resonant soft X-ray scattering, we investigate the evolution of the full momentum space topology of charge correlations in T'-(Nd,Pr)2CuO4 as a function of electron doping. We report that, when the parent Mott insulator is doped, charge correlations first emerge with full rotational symmetry in momentum space, indicating glassy charge density modulation in real space possibly seeded by local defects. At higher doping levels, the orientation of charge correlations is locked to the Cu–O bond directions, restoring a more conventional long-ranged bidirectional charge order. Through charge susceptibility calculations, we reproduce the evolution in topology of charge correlations across the antiferromagnetic phase boundary and propose a revised phase diagram of T-Ln2CuO4 with a superconducting region extending toward the Mott limit.
- Authors:
-
- Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Physics
- Univ. of California, Berkeley, CA (United States). Dept. of Physics; Univ. of California, San Diego, CA (United States). Dept. of Physics
- Univ. of California, Berkeley, CA (United States). Dept. of Physics
- Helmholtz-Zentrum Berlin für Materialien und Energie, Berlin (Germany)
- Canadian Light Sources, Inc., Saskatoon, SK (Canada)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
- NTT Basic Research Laboratories, NTT corporation, Atsugi (Japan)
- Indian Inst. of Science, Bangalore (India). Dept. of Physics
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1561910
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Physics
- Additional Journal Information:
- Journal Volume: 15; Journal Issue: 4; Journal ID: ISSN 1745-2473
- Publisher:
- Nature Publishing Group (NPG)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Kang, Mingu, Pelliciari, Jonathan, Frano, Alex, Breznay, Nicholas, Schierle, Enrico, Weschke, Eugen, Sutarto, Ronny, He, Feizhou, Shafer, Padraic, Arenholz, Elke, Chen, Mo, Zhang, Keto, Ruiz, Alejandro, Hao, Zeyu, Lewin, Sylvia, Analytis, James, Krockenberger, Yoshiharu, Yamamoto, Hideki, Das, Tanmoy, and Comin, Riccardo. Evolution of charge order topology across a magnetic phase transition in cuprate superconductors. United States: N. p., 2019.
Web. doi:10.1038/s41567-018-0401-8.
Kang, Mingu, Pelliciari, Jonathan, Frano, Alex, Breznay, Nicholas, Schierle, Enrico, Weschke, Eugen, Sutarto, Ronny, He, Feizhou, Shafer, Padraic, Arenholz, Elke, Chen, Mo, Zhang, Keto, Ruiz, Alejandro, Hao, Zeyu, Lewin, Sylvia, Analytis, James, Krockenberger, Yoshiharu, Yamamoto, Hideki, Das, Tanmoy, & Comin, Riccardo. Evolution of charge order topology across a magnetic phase transition in cuprate superconductors. United States. https://doi.org/10.1038/s41567-018-0401-8
Kang, Mingu, Pelliciari, Jonathan, Frano, Alex, Breznay, Nicholas, Schierle, Enrico, Weschke, Eugen, Sutarto, Ronny, He, Feizhou, Shafer, Padraic, Arenholz, Elke, Chen, Mo, Zhang, Keto, Ruiz, Alejandro, Hao, Zeyu, Lewin, Sylvia, Analytis, James, Krockenberger, Yoshiharu, Yamamoto, Hideki, Das, Tanmoy, and Comin, Riccardo. Mon .
"Evolution of charge order topology across a magnetic phase transition in cuprate superconductors". United States. https://doi.org/10.1038/s41567-018-0401-8. https://www.osti.gov/servlets/purl/1561910.
@article{osti_1561910,
title = {Evolution of charge order topology across a magnetic phase transition in cuprate superconductors},
author = {Kang, Mingu and Pelliciari, Jonathan and Frano, Alex and Breznay, Nicholas and Schierle, Enrico and Weschke, Eugen and Sutarto, Ronny and He, Feizhou and Shafer, Padraic and Arenholz, Elke and Chen, Mo and Zhang, Keto and Ruiz, Alejandro and Hao, Zeyu and Lewin, Sylvia and Analytis, James and Krockenberger, Yoshiharu and Yamamoto, Hideki and Das, Tanmoy and Comin, Riccardo},
abstractNote = {Charge order is now accepted as an integral constituent of cuprate high-temperature superconductors, one that is intimately related to other electronic instabilities including antiferromagnetism and superconductivity. Unlike conventional Peierls density waves, the charge correlations in cuprates have been predicted to display a rich momentum space topology depending on the underlying fermiology. However, charge order has only been observed along the high-symmetry Cu–O bond directions. Here, using resonant soft X-ray scattering, we investigate the evolution of the full momentum space topology of charge correlations in T'-(Nd,Pr)2CuO4 as a function of electron doping. We report that, when the parent Mott insulator is doped, charge correlations first emerge with full rotational symmetry in momentum space, indicating glassy charge density modulation in real space possibly seeded by local defects. At higher doping levels, the orientation of charge correlations is locked to the Cu–O bond directions, restoring a more conventional long-ranged bidirectional charge order. Through charge susceptibility calculations, we reproduce the evolution in topology of charge correlations across the antiferromagnetic phase boundary and propose a revised phase diagram of T-Ln2CuO4 with a superconducting region extending toward the Mott limit.},
doi = {10.1038/s41567-018-0401-8},
journal = {Nature Physics},
number = 4,
volume = 15,
place = {United States},
year = {Mon Jan 21 00:00:00 EST 2019},
month = {Mon Jan 21 00:00:00 EST 2019}
}
Web of Science
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