Anomalous electron transport in epitaxial NdNiO3 films

Ojha, Shashank Kumar; Ray, Sujay; Das, Tanmoy; Middey, S.; Sarkar, Sagar; Mahadevan, Priya; Wang, Zhen; Zhu, Yimei; Liu, Xiaoran; Kareev, M.; Chakhalian, J.

doi:10.1103/PhysRevB.99.235153

Title: Anomalous electron transport in epitaxial ${NdNiO}_{3}$ films

Abstract

The origin of simultaneous electronic, structural, and magnetic transitions in bulk rare-earth nickelates (RENiO₃) remains puzzling with multiple conflicting reports on the nature of these entangled phase transitions. Heterostructure engineering of these materials offers unique opportunity to decouple the metal-insulator transition (MIT) from the magnetic transition. Yet, the evolution of underlying electronic properties across these decoupled transitions remains largely unexplored. In order to address this, we have calculated Hall effect on a series of epitaxial ${NdNiO}_{3}$ films, spanning a variety of electronic and magnetic phases. We find that the MIT results in only a partially gapped Fermi surface, whereas the full insulating phase forms below the magnetic transition. Moreover, we also find a systematic reduction of the Hall coefficient R_H in the metallic phase of these films with epitaxial strain and also a surprising transition to a negative value at large compressive strain. The partially gapped, weakly insulating, paramagnetic phase is reminiscence of pseudogap behavior of high-T_c cuprates. The precursor metallic phase, which undergoes transition to the insulating phase, is a non-Fermi liquid with a temperature exponent n of resistivity of 1, whereas the exponent increases to 4/3 in the noninsulating samples. Such a nickelate phase diagram with sign reversal of R_H, a pseudogap phase, and non-Fermi-liquid behavior is intriguingly similar to high-T_c cuprates, giving crucial guidelines to engineer unconventional superconductivity in oxide heterostructures.

Authors:

Ojha, Shashank Kumar ^[1]; Ray, Sujay ^[1]; Das, Tanmoy ^[1];

^[1]; Sarkar, Sagar ^[2]; Mahadevan, Priya ^[2]; Wang, Zhen ^[3];

^[3]; Liu, Xiaoran ^[4]; Kareev, M. ^[4]; Chakhalian, J. ^[4]

Indian Inst. of Science, Bengaluru (India)
S.N. Bose National Center for Basic Sciences, Kolkata (India)
Brookhaven National Lab. (BNL), Upton, NY (United States)
Rutgers Univ., Piscataway, NJ (United States)

Publication Date:: 2019-06-27

Research Org.:: Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1561256

Alternate Identifier(s):: OSTI ID: 1529699

Report Number(s):: BNL-212072-2019-JAAM
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US2000610

Grant/Contract Number:: SC0012704; SC00012375; AC02-98CH10886; DOE DE-SC 00012375

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 99; Journal Issue: 23; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Ojha, Shashank Kumar, Ray, Sujay, Das, Tanmoy, Middey, S., Sarkar, Sagar, Mahadevan, Priya, Wang, Zhen, Zhu, Yimei, Liu, Xiaoran, Kareev, M., and Chakhalian, J.. Anomalous electron transport in epitaxial NdNiO3 films.  United States: N. p., 2019. 
Web.  doi:10.1103/PhysRevB.99.235153.

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                    Ojha, Shashank Kumar, Ray, Sujay, Das, Tanmoy, Middey, S., Sarkar, Sagar, Mahadevan, Priya, Wang, Zhen, Zhu, Yimei, Liu, Xiaoran, Kareev, M., & Chakhalian, J.. Anomalous electron transport in epitaxial NdNiO3 films.  United States.  https://doi.org/10.1103/PhysRevB.99.235153

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                    Ojha, Shashank Kumar, Ray, Sujay, Das, Tanmoy, Middey, S., Sarkar, Sagar, Mahadevan, Priya, Wang, Zhen, Zhu, Yimei, Liu, Xiaoran, Kareev, M., and Chakhalian, J.. Thu .  
"Anomalous electron transport in epitaxial NdNiO3 films".  United States.  https://doi.org/10.1103/PhysRevB.99.235153.  https://www.osti.gov/servlets/purl/1561256.

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@article{osti_1561256,

  title        = {Anomalous electron transport in epitaxial NdNiO3 films},

  author       = {Ojha, Shashank Kumar and Ray, Sujay and Das, Tanmoy and Middey, S. and Sarkar, Sagar and Mahadevan, Priya and Wang, Zhen and Zhu, Yimei and Liu, Xiaoran and Kareev, M. and Chakhalian, J.},

  abstractNote = {The origin of simultaneous electronic, structural, and magnetic transitions in bulk rare-earth nickelates (RENiO3) remains puzzling with multiple conflicting reports on the nature of these entangled phase transitions. Heterostructure engineering of these materials offers unique opportunity to decouple the metal-insulator transition (MIT) from the magnetic transition. Yet, the evolution of underlying electronic properties across these decoupled transitions remains largely unexplored. In order to address this, we have calculated Hall effect on a series of epitaxial NdNiO3 films, spanning a variety of electronic and magnetic phases. We find that the MIT results in only a partially gapped Fermi surface, whereas the full insulating phase forms below the magnetic transition. Moreover, we also find a systematic reduction of the Hall coefficient RH in the metallic phase of these films with epitaxial strain and also a surprising transition to a negative value at large compressive strain. The partially gapped, weakly insulating, paramagnetic phase is reminiscence of pseudogap behavior of high-Tc cuprates. The precursor metallic phase, which undergoes transition to the insulating phase, is a non-Fermi liquid with a temperature exponent n of resistivity of 1, whereas the exponent increases to 4/3 in the noninsulating samples. Such a nickelate phase diagram with sign reversal of RH, a pseudogap phase, and non-Fermi-liquid behavior is intriguingly similar to high-Tc cuprates, giving crucial guidelines to engineer unconventional superconductivity in oxide heterostructures.},

  doi          = {10.1103/PhysRevB.99.235153},

  journal      = {Physical Review B},

  number       = 23,

  volume       = 99,

  place        = {United States},

  year         = {2019},

  month        = {6}

}

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Figures / Tables:

FIG. 1: (a) NdNiO₃ thin film on single crystalline substrate. (b) Pseudocubic in-plane lattice constant for the substrates used in this work and the corresponding epitaxial strain for NNO. (c) HAADF-STEM image (with false color) of a 20 u.c. NdNiO₃ film on NdGaO₃ substrate.

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Works referencing / citing this record:

Mass divergence type metal-insulator transition in charge transfer rare-earth nickelates
journal, September 2019

Santhosh Kumar, K.; Phanindra, E. V.; Rana, D. S.
Physical Review B, Vol. 100, Issue 12
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Conductivity noise across temperature driven transitions of rare-earth nickelate heterostructures
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Daptary, Gopi Nath; Kumar, Siddharth; Kareev, M.
arXiv
DOI: 10.48550/arxiv.1908.06413

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Title: Anomalous electron transport in epitaxial NdNiO 3 films

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Generalized Gradient Approximation Made Simple journal, October 1996

Correlation between linear resistivity and T c in the Bechgaard salts and the pnictide superconductor Ba ( Fe 1 − x Co x ) 2 As 2 journal, December 2009

Landau Theory of Charge and Spin Ordering in the Nickelates journal, January 2011

Turning a Nickelate Fermi Surface into a Cupratelike One through Heterostructuring journal, June 2009

Monoclinic and Correlated Metal Phase in VO 2 as Evidence of the Mott Transition: Coherent Phonon Analysis journal, December 2006

Projector augmented-wave method journal, December 1994

Resonant x-ray scattering experiments on electronic orderings in NdNiO 3 single crystals journal, January 2005

Physics of Ultrathin Films and Heterostructures of Rare-Earth Nickelates journal, July 2016

Spin and charge ordering in self-doped Mott insulators journal, May 2000

Orbital Order and Possible Superconductivity in LaNiO 3 / LaMO 3 Superlattices journal, January 2008

Hall effect measurements on epitaxial SmNiO 3 thin films and implications for antiferromagnetism journal, March 2013

From ultrasoft pseudopotentials to the projector augmented-wave method journal, January 1999

Superconductivity and topological Fermi surface transitions in electron-doped cuprates near optimal doping journal, December 2008

Electronic structure of nickelates: From two-dimensional heterostructures to three-dimensional bulk materials journal, December 2010

Low-energy description of the metal-insulator transition in the rare-earth nickelates journal, February 2015

Experimental evidence for bipolaron condensation as a mechanism for the metal-insulator transition in rare-earth nickelates journal, January 2018

Orbital reflectometry of oxide heterostructures journal, February 2011

Topological properties and dynamics of magnetic skyrmions journal, December 2013

Asymmetric Orbital-Lattice Interactions in Ultrathin Correlated Oxide Films journal, September 2011

Tuning the metal-insulator transition in NdNiO 3 heterostructures via Fermi surface instability and spin fluctuations journal, July 2015

Evolution of the Hall Coefficient and the Peculiar Electronic Structure of the Cuprate Superconductors journal, May 2004

Tunable Charge and Spin Order in PrNiO 3 Thin Films and Superlattices journal, November 2014

Angle-resolved photoemission studies of the cuprate superconductors journal, April 2003

Superconducting dome in MoS 2 and TiSe 2 generated by quasiparticle-phonon coupling journal, March 2015

Charge Disproportionation without Charge Transfer in the Rare-Earth-Element Nickelates as a Possible Mechanism for the Metal-Insulator Transition journal, March 2014

Research Update: Orbital polarization in LaNiO 3 -based heterostructures journal, June 2015

Strain and composition dependence of orbital polarization in nickel oxide superlattices journal, September 2013

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set journal, July 1996

Non-Fermi liquids in oxide heterostructures journal, May 2018

Correlation between stoichiometry, strain, and metal-insulator transitions of NdNiO 3 films journal, March 2015

Site-Selective Mott Transition in Rare-Earth-Element Nickelates journal, October 2012

Role of magnetic and orbital ordering at the metal-insulator transition in NdNiO 3 journal, March 2006

Electron-hole doping of the metal-insulator transition compound RENiO3 journal, February 1994

Intermediate coupling model of the cuprates journal, May 2014

Rare-earth nickelates R NiO 3 : thin films and heterostructures journal, February 2018

Pressure-Induced Non-Fermi-Liquid Behavior of PrNiO 3 journal, June 2005

Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set journal, October 1996

Progress in perovskite nickelate research journal, July 2008

Doping Dependence of Pseudogap and Related Charge Dynamics in Nd 2 − x Ce x CuO 4 journal, October 2001

Bond disproportionation and dynamical charge fluctuations in the perovskite rare-earth nickelates journal, November 2016

Pseudogap Dependence of the Optical Conductivity Spectra of Ca 3 Ru 2 O 7 : A Possible Contribution of the Orbital Flip Excitation journal, March 2007

Dynamical Mean-Field Theory of Nickelate Superlattices journal, November 2011

Spin Fluctuations and the Peak-Dip-Hump Feature in the Photoemission Spectrum of Actinides journal, January 2012

Temperature-dependence of the Hall coefficient of NdNiO 3 thin films journal, October 2013

Scattering and Pairing in Cuprate Superconductors journal, August 2010

Ground-state oxygen holes and the metal–insulator transition in the negative charge-transfer rare-earth nickelates journal, October 2016

Hall effect in single crystal Ca 2 − x Sr x RuO 4 journal, April 2001

Low-temperature electronic properties of a normal conducting perovskite oxide (LaNiO3) journal, August 1991

Effect of Zn impurities on the normal-state Hall angle in single-crystal YBa_{2}Cu_{3-x}Zn_{x}O_{7-δ} journal, October 1991

Hall-effect measurements of HgBa 2 CaCu 2 O 6 + δ journal, August 1994

Hole superconductivity in the electron-doped superconductor Pr 2 − x Ce x Cu O 4 journal, July 2007

Pure electronic metal-insulator transition at the interface of complex oxides journal, June 2016

Fermi surfaces, electron-hole asymmetry, and correlation kink in a three-dimensional Fermi liquid LaNiO 3 journal, March 2009

Pseudogap formation above the superconducting dome in iron pnictides journal, January 2014

Impact of antiferromagnetism on the optical properties of rare-earth nickelates journal, July 2017

Structural, magnetic and electronic properties of perovskites (R = rare earth) journal, February 1997

Gaps and pseudogaps in perovskite rare earth nickelates journal, June 2015

Metal-insulator transition in a two-band model for the perovskite nickelates journal, October 2011

Heterointerface engineered electronic and magnetic phases of NdNiO3 thin films journal, November 2013

Latent instabilities in metallic LaNiO3 films by strain control of Fermi-surface topology journal, March 2015

Recent Developments in Non-Fermi Liquid Theory journal, March 2018

Evidence for a Quantum Phase Transition in Pr 2 − x Ce x CuO 4 − δ from Transport Measurements journal, April 2004

Mott Electrons in an Artificial Graphenelike Crystal of Rare-Earth Nickelate journal, February 2016

Novel Electronic Behavior Driving NdNiO 3 Metal-Insulator Transition journal, July 2015

Hall effect in the two-dimensional Luttinger liquid journal, October 1991

Quantum criticality in heavy-fermion metals journal, March 2008

High temperature superconductivity in the cuprates: Materials, phenomena and a mechanism conference, January 2018

Superconductivity in iron compounds journal, December 2011

Tuning bad metal and non-Fermi liquid behavior in a Mott material: Rare-earth nickelate thin films journal, November 2015

Epitaxial strain modulated electronic properties of interface controlled nickelate superlattices journal, July 2018

Combined effects of pairing fluctuations and a pseudogap in the cuprate Hall coefficient journal, April 2019

Hidden Fermi-liquid Charge Transport in the Antiferromagnetic Phase of the Electron-Doped Cuprate Superconductors journal, November 2016

Direct Observation of Charge Order in an Epitaxial NdNiO 3 Film journal, March 2002

Electron pockets in the Fermi surface of hole-doped high-Tc superconductors journal, November 2007

Disentangled Cooperative Orderings in Artificial Rare-Earth Nickelates journal, April 2018

Orbital control in strained ultra-thin LaNiO 3 /LaAlO 3 superlattices journal, November 2011

Title: Anomalous electron transport in epitaxial ${NdNiO}_{3}$ films

Generalized Gradient Approximation Made Simple
journal, October 1996

Correlation between linear resistivity and $T_{c}$ in the Bechgaard salts and the pnictide superconductor $Ba {({Fe}_{1 - x} {Co}_{x})}_{2} {As}_{2}$
journal, December 2009

Landau Theory of Charge and Spin Ordering in the Nickelates
journal, January 2011

Turning a Nickelate Fermi Surface into a Cupratelike One through Heterostructuring
journal, June 2009

Monoclinic and Correlated Metal Phase in ${VO}_{2}$ as Evidence of the Mott Transition: Coherent Phonon Analysis
journal, December 2006

Projector augmented-wave method
journal, December 1994

Resonant x-ray scattering experiments on electronic orderings in ${NdNiO}_{3}$ single crystals
journal, January 2005

Physics of Ultrathin Films and Heterostructures of Rare-Earth Nickelates
journal, July 2016

Spin and charge ordering in self-doped Mott insulators
journal, May 2000

Orbital Order and Possible Superconductivity in ${LaNiO}_{3} / {LaMO}_{3}$ Superlattices
journal, January 2008

Hall effect measurements on epitaxial SmNiO $_{3}$ thin films and implications for antiferromagnetism
journal, March 2013

From ultrasoft pseudopotentials to the projector augmented-wave method
journal, January 1999

Superconductivity and topological Fermi surface transitions in electron-doped cuprates near optimal doping
journal, December 2008

Electronic structure of nickelates: From two-dimensional heterostructures to three-dimensional bulk materials
journal, December 2010

Low-energy description of the metal-insulator transition in the rare-earth nickelates
journal, February 2015

Experimental evidence for bipolaron condensation as a mechanism for the metal-insulator transition in rare-earth nickelates
journal, January 2018

Orbital reflectometry of oxide heterostructures
journal, February 2011

Topological properties and dynamics of magnetic skyrmions
journal, December 2013

Asymmetric Orbital-Lattice Interactions in Ultrathin Correlated Oxide Films
journal, September 2011

Tuning the metal-insulator transition in ${NdNiO}_{3}$ heterostructures via Fermi surface instability and spin fluctuations
journal, July 2015

Evolution of the Hall Coefficient and the Peculiar Electronic Structure of the Cuprate Superconductors
journal, May 2004

Tunable Charge and Spin Order in ${PrNiO}_{3}$ Thin Films and Superlattices
journal, November 2014

Angle-resolved photoemission studies of the cuprate superconductors
journal, April 2003

Superconducting dome in ${MoS}_{2}$ and ${TiSe}_{2}$ generated by quasiparticle-phonon coupling
journal, March 2015

Charge Disproportionation without Charge Transfer in the Rare-Earth-Element Nickelates as a Possible Mechanism for the Metal-Insulator Transition
journal, March 2014

Research Update: Orbital polarization in LaNiO ₃ -based heterostructures
journal, June 2015

Strain and composition dependence of orbital polarization in nickel oxide superlattices
journal, September 2013

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set
journal, July 1996

Non-Fermi liquids in oxide heterostructures
journal, May 2018

Correlation between stoichiometry, strain, and metal-insulator transitions of NdNiO ₃ films
journal, March 2015

Site-Selective Mott Transition in Rare-Earth-Element Nickelates
journal, October 2012

Role of magnetic and orbital ordering at the metal-insulator transition in ${NdNiO}_{3}$
journal, March 2006

Electron-hole doping of the metal-insulator transition compound RENiO3
journal, February 1994

Intermediate coupling model of the cuprates
journal, May 2014

Rare-earth nickelates R NiO ₃ : thin films and heterostructures
journal, February 2018

Pressure-Induced Non-Fermi-Liquid Behavior of ${PrNiO}_{3}$
journal, June 2005

Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996

Progress in perovskite nickelate research
journal, July 2008

Doping Dependence of Pseudogap and Related Charge Dynamics in ${Nd}_{2 - x} {Ce}_{x} {CuO}_{4}$
journal, October 2001

Bond disproportionation and dynamical charge fluctuations in the perovskite rare-earth nickelates
journal, November 2016

Pseudogap Dependence of the Optical Conductivity Spectra of ${Ca}_{3} {Ru}_{2} O_{7}$ : A Possible Contribution of the Orbital Flip Excitation
journal, March 2007

Dynamical Mean-Field Theory of Nickelate Superlattices
journal, November 2011

Spin Fluctuations and the Peak-Dip-Hump Feature in the Photoemission Spectrum of Actinides
journal, January 2012

Temperature-dependence of the Hall coefficient of NdNiO ₃ thin films
journal, October 2013

Scattering and Pairing in Cuprate Superconductors
journal, August 2010

Ground-state oxygen holes and the metal–insulator transition in the negative charge-transfer rare-earth nickelates
journal, October 2016

Hall effect in single crystal ${Ca}_{2 - x} {Sr}_{x} {RuO}_{4}$
journal, April 2001

Low-temperature electronic properties of a normal conducting perovskite oxide (LaNiO3)
journal, August 1991

Effect of Zn impurities on the normal-state Hall angle in single-crystal YBa_{2}Cu_{3-x}Zn_{x}O_{7-δ}
journal, October 1991

Hall-effect measurements of ${HgBa}_{2}$ ${CaCu}_{2}$ $O_{6 + δ}$
journal, August 1994

Hole superconductivity in the electron-doped superconductor $\Pr_{2 - x} {Ce}_{x} Cu O_{4}$
journal, July 2007

Pure electronic metal-insulator transition at the interface of complex oxides
journal, June 2016

Fermi surfaces, electron-hole asymmetry, and correlation kink in a three-dimensional Fermi liquid ${LaNiO}_{3}$
journal, March 2009

Pseudogap formation above the superconducting dome in iron pnictides
journal, January 2014

Impact of antiferromagnetism on the optical properties of rare-earth nickelates
journal, July 2017

Structural, magnetic and electronic properties of perovskites (R = rare earth)
journal, February 1997

Gaps and pseudogaps in perovskite rare earth nickelates
journal, June 2015

Metal-insulator transition in a two-band model for the perovskite nickelates
journal, October 2011

Heterointerface engineered electronic and magnetic phases of NdNiO3 thin films
journal, November 2013

Latent instabilities in metallic LaNiO3 films by strain control of Fermi-surface topology
journal, March 2015

Recent Developments in Non-Fermi Liquid Theory
journal, March 2018

Evidence for a Quantum Phase Transition in $\Pr_{2 - x} {Ce}_{x} {CuO}_{4 - δ}$ from Transport Measurements
journal, April 2004

Mott Electrons in an Artificial Graphenelike Crystal of Rare-Earth Nickelate
journal, February 2016

Novel Electronic Behavior Driving ${NdNiO}_{3}$ Metal-Insulator Transition
journal, July 2015

Hall effect in the two-dimensional Luttinger liquid
journal, October 1991

Quantum criticality in heavy-fermion metals
journal, March 2008

High temperature superconductivity in the cuprates: Materials, phenomena and a mechanism
conference, January 2018

Superconductivity in iron compounds
journal, December 2011

Tuning bad metal and non-Fermi liquid behavior in a Mott material: Rare-earth nickelate thin films
journal, November 2015

Epitaxial strain modulated electronic properties of interface controlled nickelate superlattices
journal, July 2018

Combined effects of pairing fluctuations and a pseudogap in the cuprate Hall coefficient
journal, April 2019

Hidden Fermi-liquid Charge Transport in the Antiferromagnetic Phase of the Electron-Doped Cuprate Superconductors
journal, November 2016

Direct Observation of Charge Order in an Epitaxial ${NdNiO}_{3}$ Film
journal, March 2002

Electron pockets in the Fermi surface of hole-doped high-Tc superconductors
journal, November 2007

Disentangled Cooperative Orderings in Artificial Rare-Earth Nickelates
journal, April 2018

Orbital control in strained ultra-thin LaNiO ₃ /LaAlO ₃ superlattices
journal, November 2011

Low-dimensional Mott material: Transport in ultrathin epitaxial LaNiO3 films
journal, February 2010

Erratum: Dynamical Mean-Field Theory of Nickelate Superlattices [Phys. Rev. Lett. 107 , 206804 (2011)]
journal, April 2013

Mott Transition and Magnetism in Rare Earth Nickelates and its Fingerprint on the X-ray Scattering
journal, September 2017