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Title: Anomalous electron transport in epitaxial NdNiO 3 films

Abstract

The origin of simultaneous electronic, structural, and magnetic transitions in bulk rare-earth nickelates (RENiO3) remains puzzling with multiple conflicting reports on the nature of these entangled phase transitions. Heterostructure engineering of these materials offers unique opportunity to decouple the metal-insulator transition (MIT) from the magnetic transition. Yet, the evolution of underlying electronic properties across these decoupled transitions remains largely unexplored. In order to address this, we have calculated Hall effect on a series of epitaxial NdNiO 3 films, spanning a variety of electronic and magnetic phases. We find that the MIT results in only a partially gapped Fermi surface, whereas the full insulating phase forms below the magnetic transition. Moreover, we also find a systematic reduction of the Hall coefficient RH in the metallic phase of these films with epitaxial strain and also a surprising transition to a negative value at large compressive strain. The partially gapped, weakly insulating, paramagnetic phase is reminiscence of pseudogap behavior of high-Tc cuprates. The precursor metallic phase, which undergoes transition to the insulating phase, is a non-Fermi liquid with a temperature exponent n of resistivity of 1, whereas the exponent increases to 4/3 in the noninsulating samples. Such a nickelate phase diagram with sign reversal of RH, a pseudogap phase, and non-Fermi-liquid behavior is intriguingly similar to high-Tc cuprates, giving crucial guidelines to engineer unconventional superconductivity in oxide heterostructures.

Authors:
 [1];  [1];  [1]; ORCiD logo [1];  [2];  [2];  [3]; ORCiD logo [3];  [4];  [4];  [4]
  1. Indian Inst. of Science, Bengaluru (India)
  2. S.N. Bose National Center for Basic Sciences, Kolkata (India)
  3. Brookhaven National Lab. (BNL), Upton, NY (United States)
  4. Rutgers Univ., Piscataway, NJ (United States)
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1561256
Alternate Identifier(s):
OSTI ID: 1529699
Report Number(s):
BNL-212072-2019-JAAM
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US2000610
Grant/Contract Number:  
SC0012704; SC00012375; AC02-98CH10886; DOE DE-SC 00012375
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 99; Journal Issue: 23; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Ojha, Shashank Kumar, Ray, Sujay, Das, Tanmoy, Middey, S., Sarkar, Sagar, Mahadevan, Priya, Wang, Zhen, Zhu, Yimei, Liu, Xiaoran, Kareev, M., and Chakhalian, J. Anomalous electron transport in epitaxial NdNiO3 films. United States: N. p., 2019. Web. doi:10.1103/PhysRevB.99.235153.
Ojha, Shashank Kumar, Ray, Sujay, Das, Tanmoy, Middey, S., Sarkar, Sagar, Mahadevan, Priya, Wang, Zhen, Zhu, Yimei, Liu, Xiaoran, Kareev, M., & Chakhalian, J. Anomalous electron transport in epitaxial NdNiO3 films. United States. doi:10.1103/PhysRevB.99.235153.
Ojha, Shashank Kumar, Ray, Sujay, Das, Tanmoy, Middey, S., Sarkar, Sagar, Mahadevan, Priya, Wang, Zhen, Zhu, Yimei, Liu, Xiaoran, Kareev, M., and Chakhalian, J. Thu . "Anomalous electron transport in epitaxial NdNiO3 films". United States. doi:10.1103/PhysRevB.99.235153. https://www.osti.gov/servlets/purl/1561256.
@article{osti_1561256,
title = {Anomalous electron transport in epitaxial NdNiO3 films},
author = {Ojha, Shashank Kumar and Ray, Sujay and Das, Tanmoy and Middey, S. and Sarkar, Sagar and Mahadevan, Priya and Wang, Zhen and Zhu, Yimei and Liu, Xiaoran and Kareev, M. and Chakhalian, J.},
abstractNote = {The origin of simultaneous electronic, structural, and magnetic transitions in bulk rare-earth nickelates (RENiO3) remains puzzling with multiple conflicting reports on the nature of these entangled phase transitions. Heterostructure engineering of these materials offers unique opportunity to decouple the metal-insulator transition (MIT) from the magnetic transition. Yet, the evolution of underlying electronic properties across these decoupled transitions remains largely unexplored. In order to address this, we have calculated Hall effect on a series of epitaxial NdNiO3 films, spanning a variety of electronic and magnetic phases. We find that the MIT results in only a partially gapped Fermi surface, whereas the full insulating phase forms below the magnetic transition. Moreover, we also find a systematic reduction of the Hall coefficient RH in the metallic phase of these films with epitaxial strain and also a surprising transition to a negative value at large compressive strain. The partially gapped, weakly insulating, paramagnetic phase is reminiscence of pseudogap behavior of high-Tc cuprates. The precursor metallic phase, which undergoes transition to the insulating phase, is a non-Fermi liquid with a temperature exponent n of resistivity of 1, whereas the exponent increases to 4/3 in the noninsulating samples. Such a nickelate phase diagram with sign reversal of RH, a pseudogap phase, and non-Fermi-liquid behavior is intriguingly similar to high-Tc cuprates, giving crucial guidelines to engineer unconventional superconductivity in oxide heterostructures.},
doi = {10.1103/PhysRevB.99.235153},
journal = {Physical Review B},
number = 23,
volume = 99,
place = {United States},
year = {2019},
month = {6}
}

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    Works referencing / citing this record:

    Superconductivity in iron compounds
    journal, December 2011


    High temperature superconductivity in the cuprates: Materials, phenomena and a mechanism
    conference, January 2018

    • Banerjee, Sumilan; Dasgupta, Chandan; Mukerjee, Subroto
    • ADVANCED MATERIALS: Proceedings of the International Workshop on Advanced Materials (IWAM-2017), AIP Conference Proceedings
    • DOI: 10.1063/1.5050718

    Epitaxial strain modulated electronic properties of interface controlled nickelate superlattices
    journal, July 2018


    Ground-state oxygen holes and the metal–insulator transition in the negative charge-transfer rare-earth nickelates
    journal, October 2016

    • Bisogni, Valentina; Catalano, Sara; Green, Robert J.
    • Nature Communications, Vol. 7, Issue 1
    • DOI: 10.1038/ncomms13017

    Role of magnetic and orbital ordering at the metal-insulator transition in NdNiO 3
    journal, March 2006


    Effect of Zn impurities on the normal-state Hall angle in single-crystal YBa_{2}Cu_{3-x}Zn_{x}O_{7-δ}
    journal, October 1991


    Hall effect in single crystal Ca 2 x Sr x RuO 4
    journal, April 2001


    Electron pockets in the Fermi surface of hole-doped high-Tc superconductors
    journal, November 2007

    • LeBoeuf, David; Doiron-Leyraud, Nicolas; Levallois, Julien
    • Nature, Vol. 450, Issue 7169
    • DOI: 10.1038/nature06332

    Latent instabilities in metallic LaNiO3 films by strain control of Fermi-surface topology
    journal, March 2015

    • Yoo, Hyang Keun; Hyun, Seung Ill; Moreschini, Luca
    • Scientific Reports, Vol. 5, Issue 1
    • DOI: 10.1038/srep08746

    Rare-earth nickelates R NiO 3 : thin films and heterostructures
    journal, February 2018


    Charge disproportionation and search for orbital ordering in Nd Ni O 3 by use of resonant x-ray diffraction
    journal, October 2005


    Angle-resolved photoemission studies of the cuprate superconductors
    journal, April 2003

    • Damascelli, Andrea; Hussain, Zahid; Shen, Zhi-Xun
    • Reviews of Modern Physics, Vol. 75, Issue 2
    • DOI: 10.1103/revmodphys.75.473

    Combined effects of pairing fluctuations and a pseudogap in the cuprate Hall coefficient
    journal, April 2019


    Direct Observation of Charge Order in an Epitaxial NdNiO 3 Film
    journal, March 2002


    Structurally triggered metal-insulator transition in rare-earth nickelates
    journal, November 2017


    Non-Fermi liquids in oxide heterostructures
    journal, May 2018


    Disentangled Cooperative Orderings in Artificial Rare-Earth Nickelates
    journal, April 2018


    Erratum: Dynamical Mean-Field Theory of Nickelate Superlattices [Phys. Rev. Lett. 107 , 206804 (2011)]
    journal, April 2013


    Recent Developments in Non-Fermi Liquid Theory
    journal, March 2018


    Turning a Nickelate Fermi Surface into a Cupratelike One through Heterostructuring
    journal, June 2009


    Pressure-Induced Non-Fermi-Liquid Behavior of PrNiO 3
    journal, June 2005


    Gaps and pseudogaps in perovskite rare earth nickelates
    journal, June 2015

    • Allen, S. James; Hauser, Adam J.; Mikheev, Evgeny
    • APL Materials, Vol. 3, Issue 6
    • DOI: 10.1063/1.4907771

    Low-dimensional Mott material: Transport in ultrathin epitaxial LaNiO3 films
    journal, February 2010

    • Son, Junwoo; Moetakef, Pouya; LeBeau, James M.
    • Applied Physics Letters, Vol. 96, Issue 6
    • DOI: 10.1063/1.3309713

    Pseudogap formation above the superconducting dome in iron pnictides
    journal, January 2014


    Scattering and Pairing in Cuprate Superconductors
    journal, August 2010


    Hole superconductivity in the electron-doped superconductor Pr 2 x Ce x Cu O 4
    journal, July 2007


    Research Update: Orbital polarization in LaNiO 3 -based heterostructures
    journal, June 2015

    • Disa, Ankit S.; Walker, F. J.; Ismail-Beigi, Sohrab
    • APL Materials, Vol. 3, Issue 6
    • DOI: 10.1063/1.4921456

    Fermi surfaces, electron-hole asymmetry, and correlation kink in a three-dimensional Fermi liquid LaNiO 3
    journal, March 2009


    Electronic structure of nickelates: From two-dimensional heterostructures to three-dimensional bulk materials
    journal, December 2010


    Pseudogap Dependence of the Optical Conductivity Spectra of Ca 3 Ru 2 O 7 : A Possible Contribution of the Orbital Flip Excitation
    journal, March 2007


    Low-temperature electronic properties of a normal conducting perovskite oxide (LaNiO3)
    journal, August 1991


    Orbital reflectometry of oxide heterostructures
    journal, February 2011

    • Benckiser, Eva; Haverkort, Maurits W.; Brück, Sebastian
    • Nature Materials, Vol. 10, Issue 3
    • DOI: 10.1038/nmat2958

    Tunable Charge and Spin Order in PrNiO 3 Thin Films and Superlattices
    journal, November 2014


    Dynamical Mean-Field Theory of Nickelate Superlattices
    journal, November 2011


    Bond disproportionation and dynamical charge fluctuations in the perovskite rare-earth nickelates
    journal, November 2016


    Resonant x-ray scattering experiments on electronic orderings in NdNiO 3 single crystals
    journal, January 2005


    Tuning the metal-insulator transition in NdNiO 3 heterostructures via Fermi surface instability and spin fluctuations
    journal, July 2015


    Heterointerface engineered electronic and magnetic phases of NdNiO3 thin films
    journal, November 2013

    • Liu, Jian; Kargarian, Mehdi; Kareev, Mikhail
    • Nature Communications, Vol. 4, Issue 1
    • DOI: 10.1038/ncomms3714

    Change of carrier density at the pseudogap critical point of a cuprate superconductor
    journal, February 2016


    Spin Fluctuations and the Peak-Dip-Hump Feature in the Photoemission Spectrum of Actinides
    journal, January 2012


    Asymmetric Orbital-Lattice Interactions in Ultrathin Correlated Oxide Films
    journal, September 2011


    Metal-insulator transition in a two-band model for the perovskite nickelates
    journal, October 2011


    From quantum matter to high-temperature superconductivity in copper oxides
    journal, February 2015

    • Keimer, B.; Kivelson, S. A.; Norman, M. R.
    • Nature, Vol. 518, Issue 7538
    • DOI: 10.1038/nature14165

    Landau Theory of Charge and Spin Ordering in the Nickelates
    journal, January 2011


    Charge Disproportionation without Charge Transfer in the Rare-Earth-Element Nickelates as a Possible Mechanism for the Metal-Insulator Transition
    journal, March 2014


    Mott Transition and Magnetism in Rare Earth Nickelates and its Fingerprint on the X-ray Scattering
    journal, September 2017


    Pure electronic metal-insulator transition at the interface of complex oxides
    journal, June 2016

    • Meyers, D.; Liu, Jian; Freeland, J. W.
    • Scientific Reports, Vol. 6, Issue 1
    • DOI: 10.1038/srep27934

    Evidence for a Quantum Phase Transition in Pr 2 x Ce x CuO 4 δ from Transport Measurements
    journal, April 2004


    Topological properties and dynamics of magnetic skyrmions
    journal, December 2013


    Projector augmented-wave method
    journal, December 1994


    Superconducting dome in MoS 2 and TiSe 2 generated by quasiparticle-phonon coupling
    journal, March 2015


    Doping Dependence of Pseudogap and Related Charge Dynamics in Nd 2 x Ce x CuO 4
    journal, October 2001


    Site-Selective Probe of Magnetic Excitations in Rare-Earth Nickelates Using Resonant Inelastic X-ray Scattering
    journal, July 2018


    Existence of electron and hole pockets and partial gap opening in the correlated semimetal Ca 3 Ru 2 O 7
    journal, January 2018


    Site-Selective Mott Transition in Rare-Earth-Element Nickelates
    journal, October 2012


    Novel Electronic Behavior Driving NdNiO 3 Metal-Insulator Transition
    journal, July 2015


    Orbital control in strained ultra-thin LaNiO 3 /LaAlO 3 superlattices
    journal, November 2011


    Physics of Ultrathin Films and Heterostructures of Rare-Earth Nickelates
    journal, July 2016


    Low-energy description of the metal-insulator transition in the rare-earth nickelates
    journal, February 2015


    Strain and composition dependence of orbital polarization in nickel oxide superlattices
    journal, September 2013


    Superconductivity and topological Fermi surface transitions in electron-doped cuprates near optimal doping
    journal, December 2008

    • Das, Tanmoy; Markiewicz, R. S.; Bansil, A.
    • Journal of Physics and Chemistry of Solids, Vol. 69, Issue 12
    • DOI: 10.1016/j.jpcs.2008.06.018

    Intermediate coupling model of the cuprates
    journal, May 2014


    Hidden Fermi-liquid Charge Transport in the Antiferromagnetic Phase of the Electron-Doped Cuprate Superconductors
    journal, November 2016


    Monoclinic and Correlated Metal Phase in VO 2 as Evidence of the Mott Transition: Coherent Phonon Analysis
    journal, December 2006


    Temperature-dependence of the Hall coefficient of NdNiO 3 thin films
    journal, October 2013

    • Hauser, Adam J.; Mikheev, Evgeny; Moreno, Nelson E.
    • Applied Physics Letters, Vol. 103, Issue 18
    • DOI: 10.1063/1.4828557

    Generalized Gradient Approximation Made Simple
    journal, October 1996

    • Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
    • Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
    • DOI: 10.1103/physrevlett.77.3865

    Hall effect measurements on epitaxial SmNiO 3 thin films and implications for antiferromagnetism
    journal, March 2013


    Hall-effect measurements of HgBa 2 CaCu 2 O 6 + δ
    journal, August 1994


    Structural, magnetic and electronic properties of perovskites (R = rare earth)
    journal, February 1997


    Optical spectroscopy and the nature of the insulating state of rare-earth nickelates
    journal, October 2015


    Strong charge fluctuations manifested in the high-temperature Hall coefficient of high- T c cuprates
    journal, January 2007


    Evolution of the Hall Coefficient and the Peculiar Electronic Structure of the Cuprate Superconductors
    journal, May 2004


    Experimental evidence for bipolaron condensation as a mechanism for the metal-insulator transition in rare-earth nickelates
    journal, January 2018


    Quantum criticality in heavy-fermion metals
    journal, March 2008

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    • Nature Physics, Vol. 4, Issue 3
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