Long mean free paths of room-temperature THz acoustic phonons in a high thermal conductivity material
Abstract
We report measurements of room-temperature mean free paths of long-lived THz acoustic phonons in wurtzite GaN. Longitudinal phonon wave packets are excited and probed by femtosecond laser pulses in two InGaN-GaN multiple quantum well structures separated by a GaN layer. By measuring the temperature dependence of the phonon attenuation in the range 80–300 K we isolate the intrinsic phonon mean free path at 300 K which is found to be 5.3 and 3.5 μm at 1.06 and 1.43 THz, respectively. The measurements are found to be in good agreement with ab initio calculations which show that the main channel of the acoustic phonon decay is a three-phonon scattering process involving the acoustic phonon and two high-frequency optical phonons. Here, our results indicate that the contribution of low-THz acoustic phonons to thermal transport in GaN is relatively smaller than in Si; thus finite size effects are expected to be less important in GaN.
- Authors:
-
- National Taiwan Univ., Taipei (Taiwan)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
- Univ. of Houston, Houston, TX (United States)
- Univ. of Houston, Houston, TX (United States); Academia Sinica, Taipei (Taiwan)
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1560498
- Alternate Identifier(s):
- OSTI ID: 1560312
- Grant/Contract Number:
- AC05-00OR22725; FG02-00ER15087
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 100; Journal Issue: 9; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Chou, Ting -Han, Lindsay, Lucas R., Maznev, Alexei A., Gandhi, Jateen S., Stokes, Donna W., Forrest, Rebecca L., Bensaoula, Abdelhak, Nelson, Keith A., and Sun, Chi -Kuang. Long mean free paths of room-temperature THz acoustic phonons in a high thermal conductivity material. United States: N. p., 2019.
Web. doi:10.1103/PhysRevB.100.094302.
Chou, Ting -Han, Lindsay, Lucas R., Maznev, Alexei A., Gandhi, Jateen S., Stokes, Donna W., Forrest, Rebecca L., Bensaoula, Abdelhak, Nelson, Keith A., & Sun, Chi -Kuang. Long mean free paths of room-temperature THz acoustic phonons in a high thermal conductivity material. United States. https://doi.org/10.1103/PhysRevB.100.094302
Chou, Ting -Han, Lindsay, Lucas R., Maznev, Alexei A., Gandhi, Jateen S., Stokes, Donna W., Forrest, Rebecca L., Bensaoula, Abdelhak, Nelson, Keith A., and Sun, Chi -Kuang. Wed .
"Long mean free paths of room-temperature THz acoustic phonons in a high thermal conductivity material". United States. https://doi.org/10.1103/PhysRevB.100.094302. https://www.osti.gov/servlets/purl/1560498.
@article{osti_1560498,
title = {Long mean free paths of room-temperature THz acoustic phonons in a high thermal conductivity material},
author = {Chou, Ting -Han and Lindsay, Lucas R. and Maznev, Alexei A. and Gandhi, Jateen S. and Stokes, Donna W. and Forrest, Rebecca L. and Bensaoula, Abdelhak and Nelson, Keith A. and Sun, Chi -Kuang},
abstractNote = {We report measurements of room-temperature mean free paths of long-lived THz acoustic phonons in wurtzite GaN. Longitudinal phonon wave packets are excited and probed by femtosecond laser pulses in two InGaN-GaN multiple quantum well structures separated by a GaN layer. By measuring the temperature dependence of the phonon attenuation in the range 80–300 K we isolate the intrinsic phonon mean free path at 300 K which is found to be 5.3 and 3.5 μm at 1.06 and 1.43 THz, respectively. The measurements are found to be in good agreement with ab initio calculations which show that the main channel of the acoustic phonon decay is a three-phonon scattering process involving the acoustic phonon and two high-frequency optical phonons. Here, our results indicate that the contribution of low-THz acoustic phonons to thermal transport in GaN is relatively smaller than in Si; thus finite size effects are expected to be less important in GaN.},
doi = {10.1103/PhysRevB.100.094302},
journal = {Physical Review B},
number = 9,
volume = 100,
place = {United States},
year = {Wed Sep 04 00:00:00 EDT 2019},
month = {Wed Sep 04 00:00:00 EDT 2019}
}
Web of Science
Works referenced in this record:
Measuring Phonon Mean Free Path Distributions by Probing Quasiballistic Phonon Transport in Grating Nanostructures
journal, November 2015
- Zeng, Lingping; Collins, Kimberlee C.; Hu, Yongjie
- Scientific Reports, Vol. 5, Issue 1
Thermal conductivity of GaN, , and SiC from 150 K to 850 K
journal, January 2019
- Zheng, Qiye; Li, Chunhua; Rai, Akash
- Physical Review Materials, Vol. 3, Issue 1
Heat under the microscope
journal, August 2014
- Maasilta, Ilari; Minnich, Austin J.
- Physics Today, Vol. 67, Issue 8
Intrinsic lattice thermal conductivity of semiconductors from first principles
journal, December 2007
- Broido, D. A.; Malorny, M.; Birner, G.
- Applied Physics Letters, Vol. 91, Issue 23
Giant anharmonic phonon scattering in PbTe
journal, June 2011
- Delaire, O.; Ma, J.; Marty, K.
- Nature Materials, Vol. 10, Issue 8, p. 614-619
Lifetimes of Confined Acoustic Phonons in Ultrathin Silicon Membranes
journal, February 2013
- Cuffe, J.; Ristow, O.; Chávez, E.
- Physical Review Letters, Vol. 110, Issue 9
Ab initio thermal transport in compound semiconductors
journal, April 2013
- Lindsay, L.; Broido, D. A.; Reinecke, T. L.
- Physical Review B, Vol. 87, Issue 16
Accurate dependence of gallium nitride thermal conductivity on dislocation density
journal, August 2006
- Mion, C.; Muth, J. F.; Preble, E. A.
- Applied Physics Letters, Vol. 89, Issue 9
Picosecond ultrasonic measurements of attenuation of longitudinal acoustic phonons in silicon
journal, November 2009
- Daly, B. C.; Kang, K.; Wang, Y.
- Physical Review B, Vol. 80, Issue 17
Phonons and related crystal properties from density-functional perturbation theory
journal, July 2001
- Baroni, Stefano; de Gironcoli, Stefano; Dal Corso, Andrea
- Reviews of Modern Physics, Vol. 73, Issue 2
Four-phonon scattering significantly reduces intrinsic thermal conductivity of solids
journal, October 2017
- Feng, Tianli; Lindsay, Lucas; Ruan, Xiulin
- Physical Review B, Vol. 96, Issue 16
Direct measurement of individual phonon lifetimes in the clathrate compound Ba7.81Ge40.67Au5.33
journal, September 2017
- Lory, Pierre-François; Pailhès, Stéphane; Giordano, Valentina M.
- Nature Communications, Vol. 8, Issue 1
THz acoustic phonon spectroscopy and nanoscopy by using piezoelectric semiconductor heterostructures
journal, February 2015
- Mante, Pierre-Adrien; Huang, Yu-Ru; Yang, Szu-Chi
- Ultrasonics, Vol. 56
Phonon-isotope scattering and thermal conductivity in materials with a large isotope effect: A first-principles study
journal, October 2013
- Lindsay, L.; Broido, D. A.; Reinecke, T. L.
- Physical Review B, Vol. 88, Issue 14
Coherent Acoustic Phonon Oscillations in Semiconductor Multiple Quantum Wells with Piezoelectric Fields
journal, January 2000
- Sun, Chi-Kuang; Liang, Jian-Chin; Yu, Xiang-Yang
- Physical Review Letters, Vol. 84, Issue 1
Nanoscale thermal transport. II. 2003–2012
journal, March 2014
- Cahill, David G.; Braun, Paul V.; Chen, Gang
- Applied Physics Reviews, Vol. 1, Issue 1
Intrinsic phonon relaxation times from first-principles studies of the thermal conductivities of Si and Ge
journal, February 2010
- Ward, A.; Broido, D. A.
- Physical Review B, Vol. 81, Issue 8
Resonant bonding leads to low lattice thermal conductivity
journal, April 2014
- Lee, Sangyeop; Esfarjani, Keivan; Luo, Tengfei
- Nature Communications, Vol. 5, Issue 1
Non-diffusive thermal transport in GaAs at micron length scales
journal, October 2015
- Johnson, Jeremy A.; Eliason, Jeffrey K.; Maznev, Alexei A.
- Journal of Applied Physics, Vol. 118, Issue 15
Inelastic x-ray scattering measurements of phonon dispersion and lifetimes in PbTe 1− x Se x alloys
journal, September 2015
- Tian, Zhiting; Li, Mingda; Ren, Zhensong
- Journal of Physics: Condensed Matter, Vol. 27, Issue 37
THz Acoustic Spectroscopy by using Double Quantum Wells and Ultrafast Optical Spectroscopy
journal, June 2016
- Wei, Fan Jun; Yeh, Yu-Hsiang; Sheu, Jinn-Kong
- Scientific Reports, Vol. 6, Issue 1
Transmission of light through quantum heterostructures modulated by coherent acoustic phonons
journal, February 2004
- Chern, Gia-Wei; Lin, Kung-Hsuan; Sun, Chi-Kuang
- Journal of Applied Physics, Vol. 95, Issue 3
Anharmonic decay of subterahertz coherent acoustic phonons in GaN
journal, January 2007
- Liu, Tzu-Ming; Sun, Shih-Ze; Chang, Chieh-Feng
- Applied Physics Letters, Vol. 90, Issue 4
First-Principles Determination of Ultrahigh Thermal Conductivity of Boron Arsenide: A Competitor for Diamond?
journal, July 2013
- Lindsay, L.; Broido, D. A.; Reinecke, T. L.
- Physical Review Letters, Vol. 111, Issue 2, Article No. 025901
Broadband terahertz ultrasonic transducer based on a laser-driven piezoelectric semiconductor superlattice
journal, January 2012
- Maznev, A. A.; Manke, Kara J.; Lin, Kung-Hsuan
- Ultrasonics, Vol. 52, Issue 1
Spectral concentration of thermal conductivity in GaN—A first-principles study
journal, June 2018
- Garg, Jivtesh; Luo, Tengfei; Chen, Gang
- Applied Physics Letters, Vol. 112, Issue 25
Phonon Lifetime Investigation of Anharmonicity and Thermal Conductivity of by Neutron Scattering and Theory
journal, April 2013
- Pang, Judy W. L.; Buyers, William J. L.; Chernatynskiy, Aleksandr
- Physical Review Letters, Vol. 110, Issue 15
Femtosecond optical generation and detection of coherent acoustic phonons in GaN single crystals
journal, August 2007
- Wu, S.; Geiser, P.; Jun, J.
- Physical Review B, Vol. 76, Issue 8
Spectral mapping of thermal conductivity through nanoscale ballistic transport
journal, June 2015
- Hu, Yongjie; Zeng, Lingping; Minnich, Austin J.
- Nature Nanotechnology, Vol. 10, Issue 8
Terahertz coherent acoustic experiments with semiconductor superlattices
journal, November 2011
- Huynh, A.; Perrin, B.; Jusserand, B.
- Applied Physics Letters, Vol. 99, Issue 19
Fundamental Cooling Limits for High Power Density Gallium Nitride Electronics
journal, June 2015
- Yoonjin Won, ; Agonafer, Damena
- IEEE Transactions on Components, Packaging and Manufacturing Technology, Vol. 5, Issue 6
Direct measurement of coherent subterahertz acoustic phonons mean free path in GaAs
journal, May 2016
- Legrand, R.; Huynh, A.; Jusserand, B.
- Physical Review B, Vol. 93, Issue 18
Direct Measurement of Room-Temperature Nondiffusive Thermal Transport Over Micron Distances in a Silicon Membrane
journal, January 2013
- Johnson, Jeremy A.; Maznev, A. A.; Cuffe, John
- Physical Review Letters, Vol. 110, Issue 2
Limits to Fourier theory in high thermal conductivity single crystals
journal, November 2015
- Wilson, R. B.; Cahill, David G.
- Applied Physics Letters, Vol. 107, Issue 20
Phonon conduction in PbSe, PbTe, and PbTe Se from first-principles calculations
journal, May 2012
- Tian, Zhiting; Garg, Jivtesh; Esfarjani, Keivan
- Physical Review B, Vol. 85, Issue 18
Propagation of THz acoustic wave packets in GaN at room temperature
journal, February 2018
- Maznev, A. A.; Hung, T. -C.; Yao, Y. -T.
- Applied Physics Letters, Vol. 112, Issue 6
Thermal Conductivity and Large Isotope Effect in GaN from First Principles
journal, August 2012
- Lindsay, L.; Broido, D. A.; Reinecke, T. L.
- Physical Review Letters, Vol. 109, Issue 9
Terahertz electron distribution modulation in piezoelectric multiple quantum wells using coherent acoustic nanowaves
journal, August 2004
- Lin, Kung-Hsuan; Chern, Gia-Wei; Huang, Yue-Kai
- Physical Review B, Vol. 70, Issue 7
Optic phonon bandwidth and lattice thermal conductivity: The case of ( , S, Se, Te)
journal, June 2016
- Mukhopadhyay, S.; Lindsay, L.; Parker, D. S.
- Physical Review B, Vol. 93, Issue 22
Phonon scattering rates and atomic ordering in investigated with inelastic neutron scattering and synchrotron diffraction
journal, October 2014
- Ma, J.; Delaire, O.; Specht, E. D.
- Physical Review B, Vol. 90, Issue 13
Reconstructing phonon mean-free-path contributions to thermal conductivity using nanoscale membranes
journal, June 2015
- Cuffe, John; Eliason, Jeffrey K.; Maznev, A. A.
- Physical Review B, Vol. 91, Issue 24
Self-Consistent Equations Including Exchange and Correlation Effects
journal, November 1965
- Kohn, W.; Sham, L. J.
- Physical Review, Vol. 140, Issue 4A, p. A1133-A1138
Direct Measurement of Room Temperature Non-diffusive Thermal Transport Over Micron Distances in a Silicon Membrane
text, January 2012
- Johnson, Jeremy A.; Maznev, A. A.; Cuffe, John
- arXiv
Lifetimes of Confined Acoustic Phonons in Ultra-Thin Silicon Membranes
text, January 2012
- Cuffe, J.; Ristow, O.; Chávez, E.
- arXiv
Direct measurement of coherent subterahertz acoustic phonons mean free path in GaAs
text, January 2015
- Legrand, Romain; Huynh, Agnès; Jusserand, Bernard
- arXiv