Local magnetic cluster size identified by neutron total scattering in the site-diluted spin glass
Abstract
A detailed structure analysis for the site-diluted SnxFe4-xN (x = 0.25, 0.41, and 0.88) has been carried out through complex modeling of the neutron total scattering data. We present quantitative evidence showing the local ferromagnetic cluster size extending to ~8 Å on average when Sn0.88Fe3.12N undergoes the spin-glass transition (the other two not showing such a transition). In conclusion, the modeling methodology used in this work involving the corefinement of the nuclear and magnetic structure in both real and reciprocal space can potentially be applied generally to explore a variety of spin-glass material problems.
- Authors:
-
[4];
[4]
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
- RWTH Aachen Univ., Aachen (Germany); Max Planck Institute for Solid State Research, Stuttgart (Germany)
- RWTH Aachen Univ., Aachen (Germany)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1560493
- Alternate Identifier(s):
- OSTI ID: 1542686
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 100; Journal Issue: 1; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Zhang, Yuanpeng, Scholz, Tanja, Dronskowski, Richard, McDonnell, Marshall T., and Tucker, Matthew G. Local magnetic cluster size identified by neutron total scattering in the site-diluted spin glass SnxFe4-xN (x=0.88). United States: N. p., 2019.
Web. doi:10.1103/PhysRevB.100.014419.
Zhang, Yuanpeng, Scholz, Tanja, Dronskowski, Richard, McDonnell, Marshall T., & Tucker, Matthew G. Local magnetic cluster size identified by neutron total scattering in the site-diluted spin glass SnxFe4-xN (x=0.88). United States. https://doi.org/10.1103/PhysRevB.100.014419
Zhang, Yuanpeng, Scholz, Tanja, Dronskowski, Richard, McDonnell, Marshall T., and Tucker, Matthew G. Tue .
"Local magnetic cluster size identified by neutron total scattering in the site-diluted spin glass SnxFe4-xN (x=0.88)". United States. https://doi.org/10.1103/PhysRevB.100.014419. https://www.osti.gov/servlets/purl/1560493.
@article{osti_1560493,
title = {Local magnetic cluster size identified by neutron total scattering in the site-diluted spin glass SnxFe4-xN (x=0.88)},
author = {Zhang, Yuanpeng and Scholz, Tanja and Dronskowski, Richard and McDonnell, Marshall T. and Tucker, Matthew G.},
abstractNote = {A detailed structure analysis for the site-diluted SnxFe4-xN (x = 0.25, 0.41, and 0.88) has been carried out through complex modeling of the neutron total scattering data. We present quantitative evidence showing the local ferromagnetic cluster size extending to ~8 Å on average when Sn0.88Fe3.12N undergoes the spin-glass transition (the other two not showing such a transition). In conclusion, the modeling methodology used in this work involving the corefinement of the nuclear and magnetic structure in both real and reciprocal space can potentially be applied generally to explore a variety of spin-glass material problems.},
doi = {10.1103/PhysRevB.100.014419},
journal = {Physical Review B},
number = 1,
volume = 100,
place = {United States},
year = {Tue Jul 16 00:00:00 EDT 2019},
month = {Tue Jul 16 00:00:00 EDT 2019}
}
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Figures / Tables:
Figure. 1: The conceptual diagram showing the two different approaches for modeling the total scattering data. Apart from the pure-nuclear Rietveld refinement, all the other three approaches are used in the paper. Here short names are given for the four approaches – UN, UNM, SN and SNM, where ‘U’ representsmore »
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Works referencing / citing this record:
Spin-glass behavior in Co-based antiperovskite compound SnNCo 3
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