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Title: High-pressure nuclear inelastic scattering with backscattering monochromatization

Abstract

The capability to perform high-pressure low-temperature nuclear inelastic scattering on125Te and121Sb with a sapphire backscattering monochromator is presented. This technique was applied to measure nuclear inelastic scattering in TeO2at pressures up to 10 GPa and temperatures down to 25 K. The evaluated partial Te densities of phonon states were compared with theoretical calculations and with Raman scattering measured under the same conditions. The high-pressure cell developed in this work can also be used for other techniques at pressures up to at least 100 GPa.

Authors:
 [1];  [1];  [2];  [1];  [1];  [1]; ORCiD logo [3]; ORCiD logo [3]; ORCiD logo [3];  [2]; ORCiD logo [3]
  1. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
  2. Forschungszentrum Jülich GmbH, Jülich (Germany)
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Publication Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1560474
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Synchrotron Radiation (Online)
Additional Journal Information:
Journal Name: Journal of Synchrotron Radiation (Online); Journal Volume: 26; Journal Issue: 5; Journal ID: ISSN 1600-5775
Publisher:
International Union of Crystallography
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS; nuclear inelastic scattering; high pressure; backscattering; nuclear resonance scattering; density of phonon states

Citation Formats

Sergueev, Ilya, Glazyrin, Konstantin, Herrmann, Markus G., Alexeev, Pavel, Wille, Hans -Christian, Leupold, Olaf, May, Andrew F., Pandey, Tribhuwan, Lindsay, Lucas R., Friese, Karen, and Hermann, Raphael P. High-pressure nuclear inelastic scattering with backscattering monochromatization. United States: N. p., 2019. Web. doi:10.1107/S1600577519008853.
Sergueev, Ilya, Glazyrin, Konstantin, Herrmann, Markus G., Alexeev, Pavel, Wille, Hans -Christian, Leupold, Olaf, May, Andrew F., Pandey, Tribhuwan, Lindsay, Lucas R., Friese, Karen, & Hermann, Raphael P. High-pressure nuclear inelastic scattering with backscattering monochromatization. United States. https://doi.org/10.1107/S1600577519008853
Sergueev, Ilya, Glazyrin, Konstantin, Herrmann, Markus G., Alexeev, Pavel, Wille, Hans -Christian, Leupold, Olaf, May, Andrew F., Pandey, Tribhuwan, Lindsay, Lucas R., Friese, Karen, and Hermann, Raphael P. Fri . "High-pressure nuclear inelastic scattering with backscattering monochromatization". United States. https://doi.org/10.1107/S1600577519008853. https://www.osti.gov/servlets/purl/1560474.
@article{osti_1560474,
title = {High-pressure nuclear inelastic scattering with backscattering monochromatization},
author = {Sergueev, Ilya and Glazyrin, Konstantin and Herrmann, Markus G. and Alexeev, Pavel and Wille, Hans -Christian and Leupold, Olaf and May, Andrew F. and Pandey, Tribhuwan and Lindsay, Lucas R. and Friese, Karen and Hermann, Raphael P.},
abstractNote = {The capability to perform high-pressure low-temperature nuclear inelastic scattering on125Te and121Sb with a sapphire backscattering monochromator is presented. This technique was applied to measure nuclear inelastic scattering in TeO2at pressures up to 10 GPa and temperatures down to 25 K. The evaluated partial Te densities of phonon states were compared with theoretical calculations and with Raman scattering measured under the same conditions. The high-pressure cell developed in this work can also be used for other techniques at pressures up to at least 100 GPa.},
doi = {10.1107/S1600577519008853},
journal = {Journal of Synchrotron Radiation (Online)},
number = 5,
volume = 26,
place = {United States},
year = {Fri Aug 23 00:00:00 EDT 2019},
month = {Fri Aug 23 00:00:00 EDT 2019}
}

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