Two regimes of ionization-induced recovery in SrTiO3 under irradiation

Weber, William; Xue, Haizhou; Zarkadoula, Eva; Zhang, Yanwen

doi:10.1016/j.scriptamat.2019.08.013

Title: Two regimes of ionization-induced recovery in SrTiO₃ under irradiation

Journal Article · 01 December 2019 · Scripta Materialia

DOI: https://doi.org/10.1016/j.scriptamat.2019.08.013 · OSTI ID:1559652

^[1]; Xue, Haizhou ^[2];

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Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States)

Irradiation of pre-damaged SrTiO₃ with 2 MeV He, 1.2 MeV C, 5 MeV C and 12 MeV O ions reveals two regimes of ionization-induced recovery. For C and O ions, with electronic energy loss between 1.6 and 3 keV/nm, recovery cross-sections range from 0.27 to 0.38 nm², and molecular dynamics confirms recovery related to ionization-induced thermal spikes via electron-phonon coupling. Lastly, at lower electronic energy losses, recovery cross-sections decrease to about 5.5 × 10^-4 nm² for 2 MeV He ions and 1.0 × 10^-5 nm² for 200 keV electrons, which suggests recovery associated with local electronic excitation processes.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1559652

Alternate ID(s):: OSTI ID: 1557924

Journal Information:: Scripta Materialia, Vol. 173, Issue N/A; ISSN 1359-6462

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 11 works

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References (30)

On the conflicting roles of ionizing radiation in ceramics Zinkle, S. J.; Skuratov, V. A.; Hoelzer, D. T. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 191, Issue 1-4 https://doi.org/10.1016/S0168-583X(02)00648-1	journal	May 2002
The role of electronic energy loss in ion beam modification of materials Weber, William J.; Duffy, Dorothy M.; Thomé, Lionel Current Opinion in Solid State and Materials Science, Vol. 19, Issue 1 https://doi.org/10.1016/j.cossms.2014.09.003	journal	February 2015
Synergy of elastic and inelastic energy loss on ion track formation in SrTiO3 Weber, William J.; Zarkadoula, Eva; Pakarinen, Olli H. Scientific Reports, Vol. 5, Issue 1 https://doi.org/10.1038/srep07726	journal	January 2015
Two-stage synergy of electronic energy loss with defects in LiTaO 3 under ion irradiation Sellami, Neila; Crespillo, Miguel L.; Zhang, Yanwen Materials Research Letters, Vol. 6, Issue 6 https://doi.org/10.1080/21663831.2018.1455753	journal	March 2018
High-κ gate dielectrics: Current status and materials properties considerations Wilk, G. D.; Wallace, R. M.; Anthony, J. M. Journal of Applied Physics, Vol. 89, Issue 10 https://doi.org/10.1063/1.1361065	journal	May 2001
Room-temperature ferroelectricity in strained SrTiO₃ Haeni, J. H.; Irvin, P.; Chang, W. Nature, Vol. 430, Issue 7001, p. 758-761 https://doi.org/10.1038/nature02773	journal	August 2004
Electronic transport in doped SrTiO 3 : Conduction mechanisms and potential applications Spinelli, A.; Torija, M. A.; Liu, C. Physical Review B, Vol. 81, Issue 15 https://doi.org/10.1103/PhysRevB.81.155110	journal	April 2010
Persistent optically induced magnetism in oxygen-deficient strontium titanate Rice, W. D.; Ambwani, P.; Bombeck, M. Nature Materials, Vol. 13, Issue 5 https://doi.org/10.1038/nmat3914	journal	March 2014
Highly conductive nanolayers on strontium titanate produced by preferential ion-beam etching Reagor, David W.; Butko, Vladimir Y. Nature Materials, Vol. 4, Issue 8, p. 593-596 https://doi.org/10.1038/nmat1402	journal	July 2005
Tuning the Interface Conductivity of LaAlO ₃ /SrTiO ₃ Using Ion Beams: Implications for Patterning Mathew, Sinu; Annadi, Anil; Chan, Taw Kuei ACS Nano, Vol. 7, Issue 12 https://doi.org/10.1021/nn4028135	journal	November 2013
Damage evolution and waveguide formation in SrTiO3 crystal irradiated by tens of MeV Si ions Liu, Y.; Huang, Q.; Qiao, M. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 406 https://doi.org/10.1016/j.nimb.2016.12.023	journal	September 2017
Recent Advances on Carrier and Exciton Self-Trapping in Strontium Titanate: Understanding the Luminescence Emissions Crespillo, Miguel; Graham, Joseph; Agulló-López, Fernando Crystals, Vol. 9, Issue 2 https://doi.org/10.3390/cryst9020095	journal	February 2019
Role of the microstructure in the neutron and gamma-ray irradiation stability of solution-derived Ba0.5Sr0.5TiO3 thin films Glinšek, Sebastjan; Pečnik, Tanja; Cindro, Vladimir Acta Materialia, Vol. 88 https://doi.org/10.1016/j.actamat.2015.01.028	journal	April 2015
Materials Science of High-Level Nuclear Waste Immobilization Weber, William J.; Navrotsky, Alexandra; Stefanovsky, Sergey MRS Bulletin, Vol. 34, Issue 1 https://doi.org/10.1557/mrs2009.12	journal	January 2009
Dose rate and temperature effects in radiation disorder creation in SrTiO3 Sabathier, C.; Chaumont, J.; Krupa, J. -C Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 196, Issue 3-4 https://doi.org/10.1016/S0168-583X(02)01332-0	journal	November 2002
Response of strontium titanate to ion and electron irradiation Zhang, Y.; Lian, J.; Zhu, Z. Journal of Nuclear Materials, Vol. 389, Issue 2 https://doi.org/10.1016/j.jnucmat.2009.02.014	journal	May 2009
Amorphization due to electronic energy deposition in defective strontium titanate Xue, Haizhou; Zarkadoula, Eva; Liu, Peng Acta Materialia, Vol. 127 https://doi.org/10.1016/j.actamat.2017.01.051	journal	April 2017
Synergistically-enhanced ion track formation in pre-damaged strontium titanate by energetic heavy ions Xue, Haizhou; Zarkadoula, Eva; Sachan, Ritesh Acta Materialia, Vol. 150 https://doi.org/10.1016/j.actamat.2018.03.027	journal	May 2018
Swift heavy ion track formation in SrTiO ₃ and TiO ₂ under random, channeling and near-channeling conditions Karlušić, M.; Jakšić, M.; Lebius, H. Journal of Physics D: Applied Physics, Vol. 50, Issue 20 https://doi.org/10.1088/1361-6463/aa678c	journal	April 2017
Effect of doping on the radiation response of conductive Nb–SrTiO3 Li, Weixing; Rodriguez, Matias D.; Kluth, Patrick Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 302 https://doi.org/10.1016/j.nimb.2013.03.010	journal	May 2013
Revealing ionization-induced dynamic recovery in ion-irradiated SrTiO3 Velişa, Gihan; Wendler, Elke; Xue, Haizhou Acta Materialia, Vol. 149 https://doi.org/10.1016/j.actamat.2018.02.038	journal	May 2018
Study of ion beam induced epitaxial crystallization of SrTiO3 Oyoshi, K.; Hishita, S.; Haneda, H. Journal of Applied Physics, Vol. 87, Issue 7 https://doi.org/10.1063/1.372365	journal	April 2000
New ion beam materials laboratory for materials modification and irradiation effects research Zhang, Y.; Crespillo, M. L.; Xue, H. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 338 https://doi.org/10.1016/j.nimb.2014.07.028	journal	November 2014
Accumulation and thermal recovery of disorder in Au2+-irradiated SrTiO3 Thevuthasan, S.; Jiang, W.; Shutthanandan, V. Journal of Nuclear Materials, Vol. 289, Issue 1-2 https://doi.org/10.1016/S0022-3115(00)00699-1	journal	February 2001
Predictive modeling of synergistic effects in nanoscale ion track formation Zarkadoula, Eva; Pakarinen, Olli H.; Xue, Haizhou Physical Chemistry Chemical Physics, Vol. 17, Issue 35 https://doi.org/10.1039/C5CP02382C	journal	January 2015
Synergy of inelastic and elastic energy loss: Temperature effects and electronic stopping power dependence Zarkadoula, Eva; Xue, Haizhou; Zhang, Yanwen Scripta Materialia, Vol. 110 https://doi.org/10.1016/j.scriptamat.2015.05.044	journal	January 2016
DL_POLY_3: new dimensions in molecular dynamics simulations via massive parallelism Todorov, Ilian T.; Smith, William; Trachenko, Kostya Journal of Materials Chemistry, Vol. 16, Issue 20, p. 1911-1918 https://doi.org/10.1039/b517931a	journal	January 2006
Phase stability and interfacial structures in the SrO–SrTiO ₃ system Mccoy, Michael A.; Grimes, Robin W.; Lee, William E. Philosophical Magazine A, Vol. 75, Issue 3 https://doi.org/10.1080/01418619708207205	journal	March 1997
Coupled electronic and atomic effects on defect evolution in silicon carbide under ion irradiation Zhang, Yanwen; Xue, Haizhou; Zarkadoula, Eva Current Opinion in Solid State and Materials Science, Vol. 21, Issue 6 https://doi.org/10.1016/j.cossms.2017.09.003	journal	December 2017
Visible-light-accelerated oxygen vacancy migration in strontium titanate Li, Y.; Lei, Y.; Shen, B. G. Scientific Reports, Vol. 5, Issue 1 https://doi.org/10.1038/srep14576	journal	September 2015

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Molecular dynamics simulations of the response of pre-damaged SrTiO ₃ and KTaO ₃ to fast heavy ions Zarkadoula, Eva; Zhang, Yanwen; Weber, William J. AIP Advances, Vol. 10, Issue 1 https://doi.org/10.1063/1.5133061	journal	January 2020

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