Two regimes of ionization-induced recovery in SrTiO3 under irradiation

Weber, William; Xue, Haizhou; Zarkadoula, Eva; Zhang, Yanwen

doi:10.1016/j.scriptamat.2019.08.013

Title: Two regimes of ionization-induced recovery in SrTiO₃ under irradiation

Abstract

Irradiation of pre-damaged SrTiO₃ with 2 MeV He, 1.2 MeV C, 5 MeV C and 12 MeV O ions reveals two regimes of ionization-induced recovery. For C and O ions, with electronic energy loss between 1.6 and 3 keV/nm, recovery cross-sections range from 0.27 to 0.38 nm², and molecular dynamics confirms recovery related to ionization-induced thermal spikes via electron-phonon coupling. Lastly, at lower electronic energy losses, recovery cross-sections decrease to about 5.5 × 10^-4 nm² for 2 MeV He ions and 1.0 × 10^-5 nm² for 200 keV electrons, which suggests recovery associated with local electronic excitation processes.

Authors:

^[1]; Xue, Haizhou ^[2];

^[1];

^[1]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States)

Publication Date:: Sun Dec 01 00:00:00 EST 2019

Research Org.:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1559652

Alternate Identifier(s):: OSTI ID: 1557924

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Scripta Materialia

Additional Journal Information:: Journal Volume: 173; Journal Issue: N/A; Journal ID: ISSN 1359-6462

Publisher:: Elsevier

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Weber, William, Xue, Haizhou, Zarkadoula, Eva, and Zhang, Yanwen. Two regimes of ionization-induced recovery in SrTiO3 under irradiation.  United States: N. p., 2019. 
Web.  doi:10.1016/j.scriptamat.2019.08.013.

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                    Weber, William, Xue, Haizhou, Zarkadoula, Eva, & Zhang, Yanwen. Two regimes of ionization-induced recovery in SrTiO3 under irradiation.  United States.  https://doi.org/10.1016/j.scriptamat.2019.08.013

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                    Weber, William, Xue, Haizhou, Zarkadoula, Eva, and Zhang, Yanwen. Sun .  
"Two regimes of ionization-induced recovery in SrTiO3 under irradiation".  United States.  https://doi.org/10.1016/j.scriptamat.2019.08.013.  https://www.osti.gov/servlets/purl/1559652.

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@article{osti_1559652,

  title        = {Two regimes of ionization-induced recovery in SrTiO3 under irradiation},

  author       = {Weber, William and Xue, Haizhou and Zarkadoula, Eva and Zhang, Yanwen},

  abstractNote = {Irradiation of pre-damaged SrTiO3 with 2 MeV He, 1.2 MeV C, 5 MeV C and 12 MeV O ions reveals two regimes of ionization-induced recovery. For C and O ions, with electronic energy loss between 1.6 and 3 keV/nm, recovery cross-sections range from 0.27 to 0.38 nm2, and molecular dynamics confirms recovery related to ionization-induced thermal spikes via electron-phonon coupling. Lastly, at lower electronic energy losses, recovery cross-sections decrease to about 5.5 × 10-4 nm2 for 2 MeV He ions and 1.0 × 10-5 nm2 for 200 keV electrons, which suggests recovery associated with local electronic excitation processes.},

  doi          = {10.1016/j.scriptamat.2019.08.013},

  journal      = {Scripta Materialia},

  number       = N/A,

  volume       = 173,

  place        = {United States},

  year         = {Sun Dec 01 00:00:00 EST 2019},

  month        = {Sun Dec 01 00:00:00 EST 2019}

}

Copy to clipboard

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Works referencing / citing this record:

Molecular dynamics simulations of the response of pre-damaged SrTiO ₃ and KTaO ₃ to fast heavy ions
journal, January 2020

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Title: Two regimes of ionization-induced recovery in SrTiO3 under irradiation

Abstract

Citation Formats

On the conflicting roles of ionizing radiation in ceramics journal, May 2002

The role of electronic energy loss in ion beam modification of materials journal, February 2015

Synergy of elastic and inelastic energy loss on ion track formation in SrTiO3 journal, January 2015

Two-stage synergy of electronic energy loss with defects in LiTaO 3 under ion irradiation journal, March 2018

High-κ gate dielectrics: Current status and materials properties considerations journal, May 2001

Room-temperature ferroelectricity in strained SrTiO3 journal, August 2004

Electronic transport in doped SrTiO 3 : Conduction mechanisms and potential applications journal, April 2010

Persistent optically induced magnetism in oxygen-deficient strontium titanate journal, March 2014

Highly conductive nanolayers on strontium titanate produced by preferential ion-beam etching journal, July 2005

Tuning the Interface Conductivity of LaAlO 3 /SrTiO 3 Using Ion Beams: Implications for Patterning journal, November 2013

Damage evolution and waveguide formation in SrTiO3 crystal irradiated by tens of MeV Si ions journal, September 2017

Recent Advances on Carrier and Exciton Self-Trapping in Strontium Titanate: Understanding the Luminescence Emissions journal, February 2019

Role of the microstructure in the neutron and gamma-ray irradiation stability of solution-derived Ba0.5Sr0.5TiO3 thin films journal, April 2015

Materials Science of High-Level Nuclear Waste Immobilization journal, January 2009

Dose rate and temperature effects in radiation disorder creation in SrTiO3 journal, November 2002

Response of strontium titanate to ion and electron irradiation journal, May 2009

Amorphization due to electronic energy deposition in defective strontium titanate journal, April 2017

Synergistically-enhanced ion track formation in pre-damaged strontium titanate by energetic heavy ions journal, May 2018

Swift heavy ion track formation in SrTiO 3 and TiO 2 under random, channeling and near-channeling conditions journal, April 2017

Effect of doping on the radiation response of conductive Nb–SrTiO3 journal, May 2013

Revealing ionization-induced dynamic recovery in ion-irradiated SrTiO3 journal, May 2018

Study of ion beam induced epitaxial crystallization of SrTiO3 journal, April 2000

New ion beam materials laboratory for materials modification and irradiation effects research journal, November 2014

Accumulation and thermal recovery of disorder in Au2+-irradiated SrTiO3 journal, February 2001

Synergy of inelastic and elastic energy loss: Temperature effects and electronic stopping power dependence journal, January 2016

DL_POLY_3: new dimensions in molecular dynamics simulations via massive parallelism journal, January 2006

Phase stability and interfacial structures in the SrO–SrTiO 3 system journal, March 1997

Coupled electronic and atomic effects on defect evolution in silicon carbide under ion irradiation journal, December 2017

Visible-light-accelerated oxygen vacancy migration in strontium titanate journal, September 2015

Molecular dynamics simulations of the response of pre-damaged SrTiO 3 and KTaO 3 to fast heavy ions journal, January 2020

Title: Two regimes of ionization-induced recovery in SrTiO₃ under irradiation

On the conflicting roles of ionizing radiation in ceramics
journal, May 2002

The role of electronic energy loss in ion beam modification of materials
journal, February 2015

Synergy of elastic and inelastic energy loss on ion track formation in SrTiO3
journal, January 2015

Two-stage synergy of electronic energy loss with defects in LiTaO 3 under ion irradiation
journal, March 2018

High-κ gate dielectrics: Current status and materials properties considerations
journal, May 2001

Room-temperature ferroelectricity in strained SrTiO₃
journal, August 2004

Electronic transport in doped ${SrTiO}_{3}$ : Conduction mechanisms and potential applications
journal, April 2010

Persistent optically induced magnetism in oxygen-deficient strontium titanate
journal, March 2014

Highly conductive nanolayers on strontium titanate produced by preferential ion-beam etching
journal, July 2005

Tuning the Interface Conductivity of LaAlO ₃ /SrTiO ₃ Using Ion Beams: Implications for Patterning
journal, November 2013

Damage evolution and waveguide formation in SrTiO3 crystal irradiated by tens of MeV Si ions
journal, September 2017

Recent Advances on Carrier and Exciton Self-Trapping in Strontium Titanate: Understanding the Luminescence Emissions
journal, February 2019

Role of the microstructure in the neutron and gamma-ray irradiation stability of solution-derived Ba0.5Sr0.5TiO3 thin films
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Materials Science of High-Level Nuclear Waste Immobilization
journal, January 2009

Dose rate and temperature effects in radiation disorder creation in SrTiO3
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Response of strontium titanate to ion and electron irradiation
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Amorphization due to electronic energy deposition in defective strontium titanate
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Swift heavy ion track formation in SrTiO ₃ and TiO ₂ under random, channeling and near-channeling conditions
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Study of ion beam induced epitaxial crystallization of SrTiO3
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Synergy of inelastic and elastic energy loss: Temperature effects and electronic stopping power dependence
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DL_POLY_3: new dimensions in molecular dynamics simulations via massive parallelism
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Phase stability and interfacial structures in the SrO–SrTiO ₃ system
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Coupled electronic and atomic effects on defect evolution in silicon carbide under ion irradiation
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Visible-light-accelerated oxygen vacancy migration in strontium titanate
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Molecular dynamics simulations of the response of pre-damaged SrTiO ₃ and KTaO ₃ to fast heavy ions
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