Accelerated discovery and mechanical property characterization of bioresorbable amorphous alloys in the Mg–Zn–Ca and the Fe–Mg–Zn systems using high-throughput methods

Datye, Amit; Alexander Kube, Sebastian; Verma, Devendra; Schroers, Jan; Schwarz, Udo D.

doi:10.1039/C9TB01302D

Title: Accelerated discovery and mechanical property characterization of bioresorbable amorphous alloys in the Mg–Zn–Ca and the Fe–Mg–Zn systems using high-throughput methods

Abstract

High throughput discovery of amorphous bioresorbable alloys. Top: combinatorial sputtering setup. Bottom: composition of libraries deposited on silicon (Si) wafers for (a) magnesium (Mg)–zinc (Zn)–calcium (Ca) and the (b) iron (Fe)–Mg–Zn systems.

Authors:

^[1]; Alexander Kube, Sebastian ^[1]; Verma, Devendra ^[2]; Schroers, Jan ^[1]; Schwarz, Udo D. ^[3]

Department of Mechanical Engineering and Materials Science, Yale University, New Haven, USA
Nanoscience Instruments, Phoenix, USA
Department of Mechanical Engineering and Materials Science, Yale University, New Haven, USA, Department of Chemical Engineering

Publication Date:: Wed Sep 11 00:00:00 EDT 2019

Sponsoring Org.:: USDOE

OSTI Identifier:: 1557336

Grant/Contract Number:: SC0016179

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Journal of Materials Chemistry. B

Additional Journal Information:: Journal Name: Journal of Materials Chemistry. B Journal Volume: 7 Journal Issue: 35; Journal ID: ISSN 2050-750X

Publisher:: Royal Society of Chemistry (RSC)

Country of Publication:: United Kingdom

Language:: English

Citation Formats


                    Datye, Amit, Alexander Kube, Sebastian, Verma, Devendra, Schroers, Jan, and Schwarz, Udo D. Accelerated discovery and mechanical property characterization of bioresorbable amorphous alloys in the Mg–Zn–Ca and the Fe–Mg–Zn systems using high-throughput methods.  United Kingdom: N. p., 2019. 
Web.  doi:10.1039/C9TB01302D.

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                    Datye, Amit, Alexander Kube, Sebastian, Verma, Devendra, Schroers, Jan, & Schwarz, Udo D. Accelerated discovery and mechanical property characterization of bioresorbable amorphous alloys in the Mg–Zn–Ca and the Fe–Mg–Zn systems using high-throughput methods.  United Kingdom.  https://doi.org/10.1039/C9TB01302D

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                    Datye, Amit, Alexander Kube, Sebastian, Verma, Devendra, Schroers, Jan, and Schwarz, Udo D. Wed .  
"Accelerated discovery and mechanical property characterization of bioresorbable amorphous alloys in the Mg–Zn–Ca and the Fe–Mg–Zn systems using high-throughput methods".  United Kingdom.  https://doi.org/10.1039/C9TB01302D.

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@article{osti_1557336,

  title        = {Accelerated discovery and mechanical property characterization of bioresorbable amorphous alloys in the Mg–Zn–Ca and the Fe–Mg–Zn systems using high-throughput methods},

  author       = {Datye, Amit and Alexander Kube, Sebastian and Verma, Devendra and Schroers, Jan and Schwarz, Udo D.},

  abstractNote = {High throughput discovery of amorphous bioresorbable alloys. Top: combinatorial sputtering setup. Bottom: composition of libraries deposited on silicon (Si) wafers for (a) magnesium (Mg)–zinc (Zn)–calcium (Ca) and the (b) iron (Fe)–Mg–Zn systems.},

  doi          = {10.1039/C9TB01302D},

  journal      = {Journal of Materials Chemistry. B},

  number       = 35,

  volume       = 7,

  place        = {United Kingdom},

  year         = {Wed Sep 11 00:00:00 EDT 2019},

  month        = {Wed Sep 11 00:00:00 EDT 2019}

}

Copy to clipboard

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Title: Accelerated discovery and mechanical property characterization of bioresorbable amorphous alloys in the Mg–Zn–Ca and the Fe–Mg–Zn systems using high-throughput methods

Abstract

Citation Formats

A review on magnesium alloys as biodegradable materials journal, May 2010

Magnesium and its alloys as orthopedic biomaterials: A review journal, March 2006

Combinatorial development of bulk metallic glasses journal, April 2014

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Bulk metallic glasses for biomedical applications journal, September 2009

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MgZnCa glasses without clinically observable hydrogen evolution for biodegradable implants journal, September 2009

Extraction of Anisotropic Mechanical Properties From Nanoindentation of SiC-6H Single Crystals journal, June 2016

Metallic glasses as structural materials journal, February 2006

Measuring the elastic properties of anisotropic materials by means of indentation experiments journal, August 1994

Cold drawn bioabsorbable ferrous and ferrous composite wires: An evaluation of in vitro vascular cytocompatibility journal, November 2013

Biodegradable intestinal stents: A review journal, October 2014

A combinatorial thin film sputtering approach for synthesizing and characterizing ternary ZrCuAl metallic glasses journal, September 2007

Observations of the galvanostatic dissolution of pure magnesium journal, December 2012

Metallic Biomaterials: Current Challenges and Opportunities journal, July 2017

Glass forming ability and thermal stability of ternary Ca–Mg–Zn bulk metallic glasses journal, October 2005

An improved technique for determining hardness and elastic modulus using load and displacement sensing indentation experiments journal, June 1992

Mg–Ca–Zn Bulk Metallic Glasses with High Strength and Significant Ductility journal, August 2005

Corrosion resistance of resorbable Ca-Mg-Zn-Yb metallic glasses in Ringer's solution journal, May 2018

High throughput combinatorial analysis of mechanical and electrochemical properties of Li[Ni x Co y Mn z ]O 2 cathode journal, December 2016

Measurement of hardness and elastic modulus by instrumented indentation: Advances in understanding and refinements to methodology journal, January 2004

Formation and stability of complex metallic phases including quasicrystals explored through combinatorial methods journal, May 2019

Tensile Plasticity in Metallic Glasses with Pronounced β Relaxations journal, January 2012

Properties of Ce -based bulk metallic glass-forming alloys journal, December 2004

3D printing metals like thermoplastics: Fused filament fabrication of metallic glasses journal, September 2018

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Nanomoulding with amorphous metals journal, February 2009

Short-Term and Long-Term Effects of Orthopedic Biodegradable Implants journal, January 2011

Mechanical and Fatigue Behavior of Ca 65 Mg 15 Zn 20 Bulk-Metallic Glass journal, January 2009

Exploring a wider range of Mg–Ca–Zn metallic glass as biocompatible alloys using combinatorial sputtering journal, January 2017

3D metallic glass cellular structures journal, February 2016

Progress of biodegradable metals journal, October 2014

Assessing the corrosion of biodegradable magnesium implants: A critical review of current methodologies and their limitations journal, March 2012

Indentation modulus of elastically anisotropic half spaces journal, May 1993

Regulation of cell-cell fusion by nanotopography journal, September 2016

Biodegradable Metals for Cardiovascular Stent Application: Interests and New Opportunities journal, June 2011

Zinc-based bulk metallic glasses journal, August 2010

The relative influence of the topography and chemistry of TiAl6V4 surfaces on osteoblastic cell behaviour journal, August 2000

Relative influence of surface topography and surface chemistry on cell response to bone implant materials. Part 1: Physico-chemical effects journal, March 2010

Ca–Mg–Zn bulk metallic glasses as bioresorbable metals journal, July 2012

Correlations for predicting plasticity or brittleness of metallic glasses journal, May 2007

Relative influence of surface topography and surface chemistry on cell response to bone implant materials. Part 2: Biological aspects journal, March 2010

Magnesium biomaterials: past, present and future journal, August 2012

Hardness and plastic deformation in a bulk metallic glass journal, February 2005

A review on magnesium alloys as biodegradable materials
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Magnesium and its alloys as orthopedic biomaterials: A review
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Combinatorial development of bulk metallic glasses
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Biodegradable metals
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Bulk metallic glasses for biomedical applications
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Hardness-temperature relationships in metals
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The physical meaning of indentation and scratch hardness
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Biodegradable Metals for Cardiovascular Stents: from Clinical Concerns to Recent Zn-Alloys
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A Combinatorial Approach to Materials Discovery
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Magnesium alloys: Predicting in vivo corrosion with in vitro immersion testing
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Aging and Bone
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Honeycomb Structures of Bulk Metallic Glasses
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Functionalization of Metallic Glasses through Hierarchical Patterning
journal, January 2015

Elastic constants, hardness and their implications to flow properties of metallic glasses
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Mg-Zn-Ca amorphous alloys for application as temporary implant: Effect of Zn content on the mechanical and corrosion properties
journal, November 2016

Determination of critical cooling rates in metallic glass forming alloy libraries through laser spike annealing
journal, August 2017

The determination of yield strength from hardness measurements
journal, July 1971

Castable Bulk Metallic Glass Strain Wave Gears: Towards Decreasing the Cost of High-Performance Robotics
journal, November 2016

Understanding Magnesium Corrosion—A Framework for Improved Alloy Performance
journal, December 2003

Engineering Cellular Response Using Nanopatterned Bulk Metallic Glass
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Processing of Bulk Metallic Glass
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Corrosion Mechanisms of Magnesium Alloys
journal, September 1999

In vitro corrosion and biocompatibility of binary magnesium alloys
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Mg–Cu–(Y,Nd) pseudo-ternary bulk metallic glasses: The effects of Nd on glass-forming ability and plasticity
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A 200nm thick glass-forming metallic film for fatigue-property enhancements
journal, March 2006

Structural origins of Johari-Goldstein relaxation in a metallic glass
journal, February 2014

Cold-Drawn Bioabsorbable Ferrous and Ferrous Composite Wires: An Evaluation of Mechanical Strength and Fatigue Durability
journal, April 2012

Combinatorial search of thermoelastic shape-memory alloys with extremely small hysteresis width
journal, March 2006

Phase selection motifs in High Entropy Alloys revealed through combinatorial methods: Large atomic size difference favors BCC over FCC
journal, March 2019

Role of partially amorphous structure and alloying elements on the corrosion behavior of Mg–Zn–Ca bulk metallic glass for biomedical applications
journal, December 2015

MgZnCa glasses without clinically observable hydrogen evolution for biodegradable implants
journal, September 2009

Extraction of Anisotropic Mechanical Properties From Nanoindentation of SiC-6H Single Crystals
journal, June 2016

Metallic glasses as structural materials
journal, February 2006

Measuring the elastic properties of anisotropic materials by means of indentation experiments
journal, August 1994

Cold drawn bioabsorbable ferrous and ferrous composite wires: An evaluation of in vitro vascular cytocompatibility
journal, November 2013

Biodegradable intestinal stents: A review
journal, October 2014

A combinatorial thin film sputtering approach for synthesizing and characterizing ternary ZrCuAl metallic glasses
journal, September 2007

Observations of the galvanostatic dissolution of pure magnesium
journal, December 2012

Metallic Biomaterials: Current Challenges and Opportunities
journal, July 2017

Glass forming ability and thermal stability of ternary Ca–Mg–Zn bulk metallic glasses
journal, October 2005

An improved technique for determining hardness and elastic modulus using load and displacement sensing indentation experiments
journal, June 1992

Mg–Ca–Zn Bulk Metallic Glasses with High Strength and Significant Ductility
journal, August 2005

Corrosion resistance of resorbable Ca-Mg-Zn-Yb metallic glasses in Ringer's solution
journal, May 2018

High throughput combinatorial analysis of mechanical and electrochemical properties of Li[Ni x Co y Mn z ]O 2 cathode
journal, December 2016

Measurement of hardness and elastic modulus by instrumented indentation: Advances in understanding and refinements to methodology
journal, January 2004

Formation and stability of complex metallic phases including quasicrystals explored through combinatorial methods
journal, May 2019

Tensile Plasticity in Metallic Glasses with Pronounced $β$ Relaxations
journal, January 2012

Properties of $Ce$ -based bulk metallic glass-forming alloys
journal, December 2004

3D printing metals like thermoplastics: Fused filament fabrication of metallic glasses
journal, September 2018

Bioresorbable implants — practical considerations
journal, July 1996

Nanomoulding with amorphous metals
journal, February 2009

Short-Term and Long-Term Effects of Orthopedic Biodegradable Implants
journal, January 2011

Mechanical and Fatigue Behavior of Ca ₆₅ Mg ₁₅ Zn ₂₀ Bulk-Metallic Glass
journal, January 2009

Exploring a wider range of Mg–Ca–Zn metallic glass as biocompatible alloys using combinatorial sputtering
journal, January 2017

3D metallic glass cellular structures
journal, February 2016

Progress of biodegradable metals
journal, October 2014

Assessing the corrosion of biodegradable magnesium implants: A critical review of current methodologies and their limitations
journal, March 2012

Indentation modulus of elastically anisotropic half spaces
journal, May 1993

Regulation of cell-cell fusion by nanotopography
journal, September 2016

Biodegradable Metals for Cardiovascular Stent Application: Interests and New Opportunities
journal, June 2011

Zinc-based bulk metallic glasses
journal, August 2010

The relative influence of the topography and chemistry of TiAl6V4 surfaces on osteoblastic cell behaviour
journal, August 2000

Relative influence of surface topography and surface chemistry on cell response to bone implant materials. Part 1: Physico-chemical effects
journal, March 2010

Ca–Mg–Zn bulk metallic glasses as bioresorbable metals
journal, July 2012

Correlations for predicting plasticity or brittleness of metallic glasses
journal, May 2007

Relative influence of surface topography and surface chemistry on cell response to bone implant materials. Part 2: Biological aspects
journal, March 2010

Magnesium biomaterials: past, present and future
journal, August 2012

Hardness and plastic deformation in a bulk metallic glass
journal, February 2005