Hole doping and antiferromagnetic correlations above the Neel temperature of the topological semimetal (Sr1-xKx)MnSb2
- Ames Lab., Ames, IA (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Ames Lab. and Iowa State Univ., Ames, IA (United States)
We report that neutron diffraction and magnetic susceptibility studies of orthorhombic single crystal (Sr0.97K0.03) MnSb2 confirm the three-dimensional (3D) C-type antiferromagnetic (AFM) ordering of the Mn2+ moments at TN = 305 ± 3 K, which is slightly higher than that of the parent SrMnSb2 with TN = 297 ± 3 K. Susceptibility measurements of the K-doped and parent crystals above T N are characteristic of 2D AFM systems. This is consistent with high-temperature neutron diffraction of the parent compound that displays persisting 2D AFM correlations well above TN to at least ~ 560 K with no evidence of a ferromagnetic phase. Analysis of the de Haas–van Alphen magnetic oscillations of the K-doped crystal is consistent with hole doping.
- Research Organization:
- Ames Laboratory (AMES), Ames, IA (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Organization:
- USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES)
- Grant/Contract Number:
- AC02-07CH11358; AC05-00OR22725
- OSTI ID:
- 1556097
- Alternate ID(s):
- OSTI ID: 1545456; OSTI ID: 1550741
- Report Number(s):
- IS-J-9994; PRBMDO
- Journal Information:
- Physical Review B, Vol. 100, Issue 1; ISSN 2469-9950
- Publisher:
- American Physical Society (APS)Copyright Statement
- Country of Publication:
- United States
- Language:
- English
Similar Records
Crystal growth, microstructure, and physical properties of SrMnSb2
Suppression of antiferromagnetic order and strong ferromagnetic spin fluctuations in Ca(Co1-xNix)2-y As2 single crystals