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Title: Hole doping and antiferromagnetic correlations above the Neel temperature of the topological semimetal (Sr1-xKx)MnSb2

Journal Article · · Physical Review B
 [1];  [1];  [1];  [2];  [3];  [3];  [3]
  1. Ames Lab., Ames, IA (United States)
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  3. Ames Lab. and Iowa State Univ., Ames, IA (United States)

We report that neutron diffraction and magnetic susceptibility studies of orthorhombic single crystal (Sr0.97K0.03) MnSb2 confirm the three-dimensional (3D) C-type antiferromagnetic (AFM) ordering of the Mn2+ moments at TN = 305 ± 3 K, which is slightly higher than that of the parent SrMnSb2 with TN = 297 ± 3 K. Susceptibility measurements of the K-doped and parent crystals above T N are characteristic of 2D AFM systems. This is consistent with high-temperature neutron diffraction of the parent compound that displays persisting 2D AFM correlations well above TN to at least ~ 560 K with no evidence of a ferromagnetic phase. Analysis of the de Haas–van Alphen magnetic oscillations of the K-doped crystal is consistent with hole doping.

Research Organization:
Ames Laboratory (AMES), Ames, IA (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-07CH11358; AC05-00OR22725
OSTI ID:
1556097
Alternate ID(s):
OSTI ID: 1545456; OSTI ID: 1550741
Report Number(s):
IS-J-9994; PRBMDO
Journal Information:
Physical Review B, Vol. 100, Issue 1; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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Figures / Tables (5)