DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Fuel performance of chromium-coated zirconium alloy and silicon carbide accident tolerant fuel claddings

Abstract

The U.S. Department of Energy’s Accident Tolerant Fuel program is focused on extending the time for fuel failure during postulated severe accidents compared to the standard UO2-Zr alloy fuel system. This research investigates the feasibility of two different chromium-coated cladding concepts, one of which is zirconium-alloy based and the other is composite-SiC based. Both claddings had 50µm coatings, deducted from the base layer thicknesses. The claddings were reported on, using the multi- physics fuel performance tool BISON, under steady-state PWR operating conditions as well as two transients: power ramp and a loss-of-coolant accident (LOCA). The chromium-coated claddings showed comparable thermo-mechanical performance to the reference Zircaloy-4 cladding. As chromium is reported to provide an order of magnitude improvement in oxidation resistance, it is expected to be a better alternative in accident scenarios. Simulation results for both concepts call for further experimental investigation as well as modeling of beyond design-basis accidents.

Authors:
 [1]; ORCiD logo [2]; ORCiD logo [2];  [1]
  1. Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
  2. Idaho National Lab. (INL), Idaho Falls, ID (United States)
Publication Date:
Research Org.:
Idaho National Laboratory (INL), Idaho Falls, ID (United States)
Sponsoring Org.:
USDOE Office of Nuclear Energy (NE)
OSTI Identifier:
1550920
Alternate Identifier(s):
OSTI ID: 1582698
Report Number(s):
INL-JOU-18-50119-Rev000
Journal ID: ISSN 0306-4549
Grant/Contract Number:  
AC07-05ID14517; NE0008416
Resource Type:
Accepted Manuscript
Journal Name:
Annals of Nuclear Energy (Oxford)
Additional Journal Information:
Journal Name: Annals of Nuclear Energy (Oxford); Journal Volume: 120; Journal Issue: C; Journal ID: ISSN 0306-4549
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS; Accident Tolerant Fuel; Chromium; Silicon Carbide; Cladding; Nuclear Fuel; Bison

Citation Formats

Wagih, Malik, Spencer, Benjamin, Hales, Jason, and Shirvan, Koroush. Fuel performance of chromium-coated zirconium alloy and silicon carbide accident tolerant fuel claddings. United States: N. p., 2018. Web. doi:10.1016/j.anucene.2018.06.001.
Wagih, Malik, Spencer, Benjamin, Hales, Jason, & Shirvan, Koroush. Fuel performance of chromium-coated zirconium alloy and silicon carbide accident tolerant fuel claddings. United States. https://doi.org/10.1016/j.anucene.2018.06.001
Wagih, Malik, Spencer, Benjamin, Hales, Jason, and Shirvan, Koroush. Thu . "Fuel performance of chromium-coated zirconium alloy and silicon carbide accident tolerant fuel claddings". United States. https://doi.org/10.1016/j.anucene.2018.06.001. https://www.osti.gov/servlets/purl/1550920.
@article{osti_1550920,
title = {Fuel performance of chromium-coated zirconium alloy and silicon carbide accident tolerant fuel claddings},
author = {Wagih, Malik and Spencer, Benjamin and Hales, Jason and Shirvan, Koroush},
abstractNote = {The U.S. Department of Energy’s Accident Tolerant Fuel program is focused on extending the time for fuel failure during postulated severe accidents compared to the standard UO2-Zr alloy fuel system. This research investigates the feasibility of two different chromium-coated cladding concepts, one of which is zirconium-alloy based and the other is composite-SiC based. Both claddings had 50µm coatings, deducted from the base layer thicknesses. The claddings were reported on, using the multi- physics fuel performance tool BISON, under steady-state PWR operating conditions as well as two transients: power ramp and a loss-of-coolant accident (LOCA). The chromium-coated claddings showed comparable thermo-mechanical performance to the reference Zircaloy-4 cladding. As chromium is reported to provide an order of magnitude improvement in oxidation resistance, it is expected to be a better alternative in accident scenarios. Simulation results for both concepts call for further experimental investigation as well as modeling of beyond design-basis accidents.},
doi = {10.1016/j.anucene.2018.06.001},
journal = {Annals of Nuclear Energy (Oxford)},
number = C,
volume = 120,
place = {United States},
year = {Thu Jun 14 00:00:00 EDT 2018},
month = {Thu Jun 14 00:00:00 EDT 2018}
}

Journal Article:

Citation Metrics:
Cited by: 63 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Steady State and Accident Transient Analysis Burning Weapons-Grade Plutonium in Thorium and Uranium with Silicon Carbide Cladding
journal, May 2016

  • Andrews, Nathan; Shirvan, Koroush; Pilat, Edward E.
  • Nuclear Technology, Vol. 194, Issue 2
  • DOI: 10.13182/NT15-41

Mechanical performance of SiC three-layer cladding in PWRs
journal, December 2016


Improving Accident Tolerance of Nuclear Fuel with Coated Mo-alloy Cladding
journal, February 2016


Fabrication of SiC–SiC composites for fuel cladding in advanced reactor designs
journal, May 2012


Characterization of SiC–SiC composites for accident tolerant fuel cladding
journal, November 2015


Lattice contractions associated with the neutron irradiation of self-bonded silicon carbide
journal, September 1967


Mechanical properties of neutron-irradiated model and commercial FeCrAl alloys
journal, June 2017


Accident-Tolerant-Fuel Performance Analysis of APMT Steel Clad/UO 2 Fuel and APMT Steel Clad/UN-U 3 Si 5 Fuel Concepts
journal, April 2016

  • Galloway, Jack; Unal, Cetin
  • Nuclear Science and Engineering, Vol. 182, Issue 4
  • DOI: 10.13182/NSE15-7

An investigation of FeCrAl cladding behavior under normal operating and loss of coolant conditions
journal, August 2017


MOOSE: A parallel computational framework for coupled systems of nonlinear equations
journal, October 2009


BISON Theory Manual The Equations behind Nuclear Fuel Analysis
report, September 2016


Mechanical and thermomechanical properties of commercially pure chromium and chromium alloys
journal, February 2002


Japan's post-Fukushima challenge – implications from the German experience on renewable energy policy
journal, June 2012


Investigation of the C-ring test for measuring hoop tensile strength of nuclear grade ceramic composites
journal, September 2014


The implications of Fukushima
journal, July 2011


Thermophysical and mechanical properties of near-stoichiometric fiber CVI SiC/SiC composites after neutron irradiation at elevated temperatures
journal, August 2010


Observation and possible mechanism of irradiation induced creep in ceramics
journal, March 2013


Continuous SiC fiber, CVI SiC matrix composites for nuclear applications: Properties and irradiation effects
journal, May 2014


KAERI’s Development of LWR Accident-Tolerant Fuel
journal, May 2014

  • Koo, Yang-Hyun; Yang, Jae-Ho; Park, Jeong-Yong
  • Nuclear Technology, Vol. 186, Issue 2
  • DOI: 10.13182/NT13-89

Safety Assessment of SiC Cladding Oxidation under Loss-of-Coolant Accident Conditions in Light Water Reactors
journal, August 2013

  • Lee, Youho; McKrell, Thomas J.; Yue, Chao
  • Nuclear Technology, Vol. 183, Issue 2
  • DOI: 10.13182/NT12-122

On High Temperature Oxidation of Chromium
journal, January 1980

  • Lillerud, K. P.
  • Journal of The Electrochemical Society, Vol. 127, Issue 11
  • DOI: 10.1149/1.2129478

Tensile properties of a SiCf/SiC composite
journal, October 1996


High temperature oxidation of fuel cladding candidate materials in steam–hydrogen environments
journal, September 2013


Properties of Silicon Carbide for Nuclear Fuel Particle Coatings
journal, September 1977


Development of Cr cold spray–coated fuel cladding with enhanced accident tolerance
journal, March 2018

  • Ševeček, Martin; Gurgen, Anil; Seshadri, Arunkumar
  • Nuclear Engineering and Technology, Vol. 50, Issue 2
  • DOI: 10.1016/j.net.2017.12.011

Thermal conductivity degradation of ceramic materials due to low temperature, low dose neutron irradiation
journal, April 2005


Handbook of SiC properties for fuel performance modeling
journal, September 2007


Stress analysis and probabilistic assessment of multi-layer SiC-based accident tolerant nuclear fuel cladding
journal, November 2015


Advanced oxidation-resistant iron-based alloys for LWR fuel cladding
journal, May 2014


Irradiation and the ductility of chromium
journal, August 1968


Multidimensional multiphysics simulation of nuclear fuel behavior
journal, April 2012


Neutronics and fuel performance evaluation of accident tolerant FeCrAl cladding under normal operation conditions
journal, November 2015


Development and property evaluation of nuclear grade wrought FeCrAl fuel cladding for light water reactors
journal, December 2015


Accident tolerant fuels for LWRs: A perspective
journal, May 2014


Works referencing / citing this record:

Oxidation behavior of RF magnetron sputtered Cr–SiC–Cr composites coating on zircaloy fuel cladding
journal, July 2019


Effectiveness of Cr-Coated Zr-Alloy Clad in Delaying Fuel Degradation for a PWR During a Station Blackout Event
journal, August 2019


The technological challenge for current generation nuclear reactors
journal, September 2019

  • D’Auria, Francesco; Debrecin, Nenad; Glaeser, Horst
  • Nuclear Energy and Technology, Vol. 5, Issue 3
  • DOI: 10.3897/nucet.5.38117