Spatial distribution, chemical state, solubility of rhenium in a reducing cement waste form: Implications for predicting technetium mobility in saltstone

Arai, Yuji; Meena, Amanda H.; Lenell, Brain; Powell, Brian A.; Kaplan, Daniel I.

doi:10.1016/j.apgeochem.2017.02.001

Title: Spatial distribution, chemical state, solubility of rhenium in a reducing cement waste form: Implications for predicting technetium mobility in saltstone

Journal Article · 01 October 2017 · Applied Geochemistry

DOI: https://doi.org/10.1016/j.apgeochem.2017.02.001 · OSTI ID:1550605

Arai, Yuji; Meena, Amanda H.; Lenell, Brain; Powell, Brian A.; Kaplan, Daniel I.

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Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-76SF00515; AC02-06CH11357; AC09-08SR22470

OSTI ID:: 1550605

Journal Information:: Applied Geochemistry, Journal Name: Applied Geochemistry Journal Issue: PB Vol. 85; ISSN 0883-2927

Publisher:: ElsevierCopyright Statement

Country of Publication:: United Kingdom

Language:: English

References (12)

Rhenium as analog for fissiogenic technetium: Eh-pH diagram (25°C, 1 bar) constraints Brookins, Douglas G. Applied Geochemistry, Vol. 1, Issue 4 https://doi.org/10.1016/0883-2927(86)90056-9	journal	July 1986
Application of portland cement-based materials to radioactive waste immobilization Atkins, M.; Glasser, F. P. Waste Management, Vol. 12, Issue 2-3 https://doi.org/10.1016/0956-053X(92)90044-J	journal	January 1992
Evolution of pore water chemistry during degradation of cement in a radioactive waste repository environment Berner, U. R. Waste Management, Vol. 12, Issue 2-3 https://doi.org/10.1016/0956-053X(92)90049-O	journal	January 1992
Experimental study of cement grout Rosquoët, F.; Alexis, A.; Khelidj, A. Cement and Concrete Research, Vol. 33, Issue 5 https://doi.org/10.1016/S0008-8846(02)01036-0	journal	May 2003
Effect of iron and carbonation on the diffusion of iodine and rhenium in waste encasement concrete and soil fill material under hydraulically unsaturated conditions Wellman, Dawn M.; Parker, Kent E.; Powers, Laura Applied Geochemistry, Vol. 23, Issue 8 https://doi.org/10.1016/j.apgeochem.2008.04.002	journal	August 2008
Chemical stabilization of chromate in blast furnace slag mixed cementitious materials Meena, Amanda H.; Kaplan, Daniel I.; Powell, Brian A. Chemosphere, Vol. 138 https://doi.org/10.1016/j.chemosphere.2015.06.008	journal	November 2015
Reductive capacity measurement of waste forms for secondary radioactive wastes Um, Wooyong; Yang, Jung-Seok; Serne, R. Jeffrey Journal of Nuclear Materials, Vol. 467 https://doi.org/10.1016/j.jnucmat.2015.09.045	journal	December 2015
Evaluation of Perrhenate Spectrophotometric Methods in Bicarbonate and Nitrate Media Lenell, Brian A.; Arai, Yuji Talanta, Vol. 150 https://doi.org/10.1016/j.talanta.2015.10.063	journal	April 2016
The biomedical chemistry of technetium and rhenium R. Dilworth, Jonathan; J. Parrott, Suzanne Chemical Society Reviews, Vol. 27, Issue 1 https://doi.org/10.1039/a827043z	journal	January 1998
Technetium Speciation in Cement Waste Forms Determined by X-ray Absorption Fine Structure Spectroscopy Allen, P. G.; Siemering, G. S.; Shuh, D. K. Radiochimica Acta, Vol. 76, Issue 1-2 https://doi.org/10.1524/ract.1997.76.12.77	journal	January 1997
Chemistry of rhenium as an analogue of technetium: Experimental studies of the dissolution of rhenium oxides in aqueous solutions Kim, E.; Boulègue, J. Radiochimica Acta, Vol. 91, Issue 4 https://doi.org/10.1524/ract.91.4.211.19968	journal	April 2003
The biogeochemistry of technetium: A review of the behavior of an artificial element in the natural environment Icenhower, J. P.; Qafoku, N. P.; Zachara, J. M. American Journal of Science, Vol. 310, Issue 8 https://doi.org/10.2475/08.2010.02	journal	October 2010

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