Integrated model development for safeguarding pyroprocessing facility: Part I-model development and validation

Zhou, Wentao; Wang, Yafei; Zhang, Jinsuo

doi:10.1016/j.anucene.2017.09.050

Title: Integrated model development for safeguarding pyroprocessing facility: Part I-model development and validation

Authors:: Zhou, Wentao; Wang, Yafei; Zhang, Jinsuo

Publication Date:: 2018-02-01

Sponsoring Org.:: USDOE

OSTI Identifier:: 1549038

Grant/Contract Number:: 13-4908

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Annals of Nuclear Energy

Additional Journal Information:: Journal Name: Annals of Nuclear Energy Journal Volume: 112 Journal Issue: C; Journal ID: ISSN 0306-4549

Publisher:: Elsevier

Country of Publication:: United Kingdom

Language:: English

Citation Formats


                    Zhou, Wentao, Wang, Yafei, and Zhang, Jinsuo. Integrated model development for safeguarding pyroprocessing facility: Part I-model development and validation.  United Kingdom: N. p., 2018. 
Web.  doi:10.1016/j.anucene.2017.09.050.

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                    Zhou, Wentao, Wang, Yafei, & Zhang, Jinsuo. Integrated model development for safeguarding pyroprocessing facility: Part I-model development and validation.  United Kingdom.  https://doi.org/10.1016/j.anucene.2017.09.050

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                    Zhou, Wentao, Wang, Yafei, and Zhang, Jinsuo. Thu .  
"Integrated model development for safeguarding pyroprocessing facility: Part I-model development and validation".  United Kingdom.  https://doi.org/10.1016/j.anucene.2017.09.050.

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@article{osti_1549038,

  title        = {Integrated model development for safeguarding pyroprocessing facility: Part I-model development and validation},

  author       = {Zhou, Wentao and Wang, Yafei and Zhang, Jinsuo},

  abstractNote = {},

  doi          = {10.1016/j.anucene.2017.09.050},

  journal      = {Annals of Nuclear Energy},

  number       = C,

  volume       = 112,

  place        = {United Kingdom},

  year         = {2018},

  month        = {2}

}

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Title: Integrated model development for safeguarding pyroprocessing facility: Part I-model development and validation

Citation Formats

Criticality Safety Evaluation of Materials Concerning Pyroprocessing journal, June 2011

Molten fluoride salt and liquid metal multistage extraction model journal, May 2017

Numerical assessment of pyrochemical process performance for PEACER system journal, June 2010

Electrochemical Behavior of Zr on a Liquid Cd Electrode in LiCl–KCl Eutectic Melts journal, January 2008

Direct Calculation of Concentration-Dependent Activity Coefficient of UCl 3 in Molten LiCl-KCl journal, January 2015

Prediction of Diffusion Coefficients in Porous Media Using Tortuosity Factors Based on Interfacial Areas journal, July 2002

Thermodynamic Properties of U, Np, Pu, and Am in Molten LiCl‐KCl Eutectic and Liquid Cadmium journal, August 1996

Development of trail, a simulation code for the molten salt electrorefining of spent nuclear fuel journal, June 1993

Modeling of anodic dissolution of U–Pu–Zr ternary alloy in the molten LiCl–KCl electrolyte journal, February 2005

Distribution of plutonium, americium, and several rare earth fission product elements between liquid cadmium and LiClKCl eutectic journal, September 1993

Thermochemical modelling of electrotransport of uranium and plutonium in an electrorefiner journal, January 1998

Thermodynamic evaluation of LiCl-KCl-PuCl3 system journal, February 2017

A Computational Meta-Analysis of UCl3Cyclic Voltammograms in LiCl-KCl Electrolyte journal, January 2014

Electrochemical Measurement of Diffusion Coefficient of Pu in Liquid Cd journal, January 2014

Exchange Current Density and Diffusion Layer Thickness in Molten LiCl-KCl Eutectic: A Modeling Perspective for Pyroprocessing of Metal Fuels journal, September 2016

PRAGAMAN: A Computer Code for Simulation of Electrotransport during Molten Salt Electrorefining journal, June 2010

Determining the Exchange Current Density and Tafel Constant for Uranium in LiCl/KCl Eutectic journal, October 2014

Study on Exchange Current Density and Transfer Coefficient of Uranium in LiCl-KCl Molten Salt journal, January 2015

Diffusion behavior of actinide and lanthanide elements in molten salt for reductive extraction journal, October 2007

Uranium Transport to Solid Electrodes in Pyrochemical Reprocessing of Nuclear Fuel journal, January 1992

The thermodynamics of pyrochemical processes for liquid metal reactor fuel cycles journal, June 1988

The rotating cylinder electrode journal, May 1974

Application of the rotating cylinder electrode in molten LiCl-KCl eutectic containing uranium(III)- and magnesium(II)-chloride journal, April 2017

Electrochemistry of actinides and fission products in molten salts—Data review journal, April 2014

Chemical diffusion coefficient calculation of U3+ in LiCl-KCl molten salt journal, August 2016

Anodic dissolution of U, Zr and U–Zr alloy and convolution voltammetry of Zr4+|Zr2+ couple in molten LiCl–KCl eutectic journal, October 2011

Three-dimensional multispecies current density simulation of molten-salt electrorefining journal, July 2010

A Low-Decontamination Approach to a Proliferation-Resistant Fuel Cycle journal, December 1978

A phase-field simulation of uranium dendrite growth on the cathode in the electrorefining process journal, July 2011

Thermodynamic assessment of the LiCl–KCl–CeCl3 system journal, June 2015

Kinetic model for electrorefining, part II: Model applications and case studies journal, January 2014

Kinetic model for electrorefining, part I: Model development and validation journal, January 2014

Transient modeling of spent nuclear fuel electrorefining with liquid metal electrode journal, August 2017

Study of Molten Salt Electrorefining ofU-Pu-Zr Alloy Fuel journal, November 2002

Electrochemical processing of spent nuclear fuels: An overview of oxide reduction in pyroprocessing technology journal, December 2015

Development of a 1D transient electrorefiner model for pyroprocess simulation journal, September 2014

Experimental investigations and thermodynamic modelling of KCl–LiCl–UCl3 system journal, June 2014

Analyses of Anodic Behavior of Metallic Fast Reactor Fuel Using a Multidiffusion Layer Model journal, December 2010

Criticality Safety Evaluation of Materials Concerning Pyroprocessing
journal, June 2011

Molten fluoride salt and liquid metal multistage extraction model
journal, May 2017

Numerical assessment of pyrochemical process performance for PEACER system
journal, June 2010

Electrochemical Behavior of Zr on a Liquid Cd Electrode in LiCl–KCl Eutectic Melts
journal, January 2008

Direct Calculation of Concentration-Dependent Activity Coefficient of UCl ₃ in Molten LiCl-KCl
journal, January 2015

Prediction of Diffusion Coefficients in Porous Media Using Tortuosity Factors Based on Interfacial Areas
journal, July 2002

Thermodynamic Properties of U, Np, Pu, and Am in Molten LiCl‐KCl Eutectic and Liquid Cadmium
journal, August 1996

Development of trail, a simulation code for the molten salt electrorefining of spent nuclear fuel
journal, June 1993

Modeling of anodic dissolution of U–Pu–Zr ternary alloy in the molten LiCl–KCl electrolyte
journal, February 2005

Distribution of plutonium, americium, and several rare earth fission product elements between liquid cadmium and LiClKCl eutectic
journal, September 1993

Thermochemical modelling of electrotransport of uranium and plutonium in an electrorefiner
journal, January 1998

Thermodynamic evaluation of LiCl-KCl-PuCl3 system
journal, February 2017

A Computational Meta-Analysis of UCl₃Cyclic Voltammograms in LiCl-KCl Electrolyte
journal, January 2014

Electrochemical Measurement of Diffusion Coefficient of Pu in Liquid Cd
journal, January 2014

Exchange Current Density and Diffusion Layer Thickness in Molten LiCl-KCl Eutectic: A Modeling Perspective for Pyroprocessing of Metal Fuels
journal, September 2016

PRAGAMAN: A Computer Code for Simulation of Electrotransport during Molten Salt Electrorefining
journal, June 2010

Determining the Exchange Current Density and Tafel Constant for Uranium in LiCl/KCl Eutectic
journal, October 2014

Study on Exchange Current Density and Transfer Coefficient of Uranium in LiCl-KCl Molten Salt
journal, January 2015

Diffusion behavior of actinide and lanthanide elements in molten salt for reductive extraction
journal, October 2007

Uranium Transport to Solid Electrodes in Pyrochemical Reprocessing of Nuclear Fuel
journal, January 1992

The thermodynamics of pyrochemical processes for liquid metal reactor fuel cycles
journal, June 1988

The rotating cylinder electrode
journal, May 1974

Application of the rotating cylinder electrode in molten LiCl-KCl eutectic containing uranium(III)- and magnesium(II)-chloride
journal, April 2017

Electrochemistry of actinides and fission products in molten salts—Data review
journal, April 2014

Chemical diffusion coefficient calculation of U3+ in LiCl-KCl molten salt
journal, August 2016

Anodic dissolution of U, Zr and U–Zr alloy and convolution voltammetry of Zr4+|Zr2+ couple in molten LiCl–KCl eutectic
journal, October 2011

Three-dimensional multispecies current density simulation of molten-salt electrorefining
journal, July 2010

A Low-Decontamination Approach to a Proliferation-Resistant Fuel Cycle
journal, December 1978

A phase-field simulation of uranium dendrite growth on the cathode in the electrorefining process
journal, July 2011

Thermodynamic assessment of the LiCl–KCl–CeCl3 system
journal, June 2015

Kinetic model for electrorefining, part II: Model applications and case studies
journal, January 2014

Kinetic model for electrorefining, part I: Model development and validation
journal, January 2014

Transient modeling of spent nuclear fuel electrorefining with liquid metal electrode
journal, August 2017

Study of Molten Salt Electrorefining ofU-Pu-Zr Alloy Fuel
journal, November 2002

Electrochemical processing of spent nuclear fuels: An overview of oxide reduction in pyroprocessing technology
journal, December 2015

Development of a 1D transient electrorefiner model for pyroprocess simulation
journal, September 2014

Experimental investigations and thermodynamic modelling of KCl–LiCl–UCl3 system
journal, June 2014

Analyses of Anodic Behavior of Metallic Fast Reactor Fuel Using a Multidiffusion Layer Model
journal, December 2010