Frustrated Dipole Order Induces Noncollinear Proper Ferrielectricity in Two Dimensions
Abstract
Within Landau theory, magnetism and polarity are homotopic, displaying a one-to-one correspondence between most physical characteristics. Yet, despite widely reported noncollinear magnetism, spontaneous noncollinear electric dipole order as a ground state is rare. In this work, a dioxydihalides family is suggested to display noncollinear ferrielectricity, induced by competing ferroelectric and antiferroelectric soft modes. This intrinsic of dipoles generates unique physical properties, such as $$\mathbb{Z_{2}×Z_{2}}$$ topological domains, atomic-scale dipole vortices, and negative piezoelectricity.
- Authors:
-
- Southeast Univ., Nanjing (China); Univ. of Tennessee, Knoxville, TN (United States)
- Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Southeast Univ., Nanjing (China)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1557479
- Alternate Identifier(s):
- OSTI ID: 1547980
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review Letters
- Additional Journal Information:
- Journal Volume: 123; Journal Issue: 6; Journal ID: ISSN 0031-9007
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Lin, Ling-Fang, Zhang, Yang, Moreo, Adriana, Dagotto, Elbio, and Dong, Shuai. Frustrated Dipole Order Induces Noncollinear Proper Ferrielectricity in Two Dimensions. United States: N. p., 2019.
Web. doi:10.1103/PhysRevLett.123.067601.
Lin, Ling-Fang, Zhang, Yang, Moreo, Adriana, Dagotto, Elbio, & Dong, Shuai. Frustrated Dipole Order Induces Noncollinear Proper Ferrielectricity in Two Dimensions. United States. https://doi.org/10.1103/PhysRevLett.123.067601
Lin, Ling-Fang, Zhang, Yang, Moreo, Adriana, Dagotto, Elbio, and Dong, Shuai. Wed .
"Frustrated Dipole Order Induces Noncollinear Proper Ferrielectricity in Two Dimensions". United States. https://doi.org/10.1103/PhysRevLett.123.067601. https://www.osti.gov/servlets/purl/1557479.
@article{osti_1557479,
title = {Frustrated Dipole Order Induces Noncollinear Proper Ferrielectricity in Two Dimensions},
author = {Lin, Ling-Fang and Zhang, Yang and Moreo, Adriana and Dagotto, Elbio and Dong, Shuai},
abstractNote = {Within Landau theory, magnetism and polarity are homotopic, displaying a one-to-one correspondence between most physical characteristics. Yet, despite widely reported noncollinear magnetism, spontaneous noncollinear electric dipole order as a ground state is rare. In this work, a dioxydihalides family is suggested to display noncollinear ferrielectricity, induced by competing ferroelectric and antiferroelectric soft modes. This intrinsic of dipoles generates unique physical properties, such as $\mathbb{Z_{2}×Z_{2}}$ topological domains, atomic-scale dipole vortices, and negative piezoelectricity.},
doi = {10.1103/PhysRevLett.123.067601},
journal = {Physical Review Letters},
number = 6,
volume = 123,
place = {United States},
year = {Wed Aug 07 00:00:00 EDT 2019},
month = {Wed Aug 07 00:00:00 EDT 2019}
}
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Figures / Tables:
FIG. 1: (a-d) Sketch of the spin/dipole orders discussed in the text. (a) FM/FE parallel alignment; (b) AFM/AFE antiparallel alignment, fully compensated; (c-d) FiM/FiE: similar to (b) but with magnetization/polarization only partially compensated. (e, f) Structures of MOnX6−2n. (e) n = 3; (f) n = 2. The most stable vdWmore »
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