Search Menu
DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information
Search Scholarly Publications

Title: Time-resolved ionization measurements with intense ultrashort XUV and X-ray free-electron laser pulses

Abstract

Abstract Modern free-electron lasers (FEL) operating in XUV (extreme ultraviolet) or X-ray range allow an access to novel research areas. One instance is the ultrafast ionization of a solid by an intense femtosecond FEL pulse in XUV which consequently leads to a change of the complex index of refraction on an ultrashort timescale. The photoionization and subsequent impact ionization resulting in electronic and atomic dynamics are modeled with our hybrid code XTANT(X-ray thermal and non-thermal transitions) and a Monte Carlo code XCASCADE(X-ray-induced electron cascades). The simulations predict the temporal kinetics of FEL-induced electron cascades and thus yield temporally and spatially resolved information on the induced changes of the optical properties. In a series of experiments at FERMI and LCLS, single shot measurements with spatio-temporal encoding of the ionization process have been performed by a correlation of the FEL pump pulse with an optical femtosecond probe pulse. An excellent agreement between the experiment and the simulation has been found. Furthermore, we demonstrate that such kind of experiments forms the basis for pulse duration and arrival time jitter monitoring as currently under development for XUV-FELs.

Authors:
 [1];  [2];  [3];  [4];  [5];  [5];  [6];  [6];  [6];  [6];  [6];  [6];  [7];  [5];  [8];  [8];  [9];  [8];  [10]
+ Show Author Affiliations
  1. Hochschule Emden/Leer Univ. of Applied Sciences (Germany); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
  2. Hochschule Emden/Leer Univ. of Applied Sciences (Germany)
  3. Hochschule Emden/Leer Univ. of Applied Sciences (Germany); Inst. of the Helmholtz-Zentrum Dresden-Rossendorf (Germany)
  4. Academy of Sciences of the Czech Republic (ASCR), Prague (Czech Republic)
  5. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
  6. Elettra Sincrotrone Trieste (Italy)
  7. Univ. of Hamburg (Germany)
  8. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  9. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Polish Academy of Sciences (PAS), Krakow (Poland)
  10. Hochschule Emden/Leer Univ. of Applied Sciences (Germany); Carl von Ossietzky Univ. (Germany)
Publication Date:
Research Org.:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org.:
USDOE; German Ministry of Education and Research
OSTI Identifier:
1547231
Grant/Contract Number:  
AC02-76SF00515
Resource Type:
Accepted Manuscript
Journal Name:
Laser and Particle Beams
Additional Journal Information:
Journal Volume: 37; Journal Issue: 2; Journal ID: ISSN 0263-0346
Publisher:
Cambridge University Press
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Free-electron laser; XUV; X-ray

Citation Formats

Tkachenko, Victor, Büscher, Martin, Höppner, Hauke, Medvedev, Nikita, Lipp, Vladimir, Rossi, Giulio Maria, Capotondi, Flavio, Finetti, Paola, Pedersoli, Emanuele, Nikolov, Ivaylo, Danailov, Mitcho, Giannessi, Luca, Prandolini, Mark J., Toleikis, Sven, Mecseki, Katalin, Windeler, Matthew, Ziaja, Beata, Tavella, Franz, and Teubner, Ulrich. Time-resolved ionization measurements with intense ultrashort XUV and X-ray free-electron laser pulses. United States: N. p., 2019. Web. doi:10.1017/s0263034619000326.
Copy to clipboard
Tkachenko, Victor, Büscher, Martin, Höppner, Hauke, Medvedev, Nikita, Lipp, Vladimir, Rossi, Giulio Maria, Capotondi, Flavio, Finetti, Paola, Pedersoli, Emanuele, Nikolov, Ivaylo, Danailov, Mitcho, Giannessi, Luca, Prandolini, Mark J., Toleikis, Sven, Mecseki, Katalin, Windeler, Matthew, Ziaja, Beata, Tavella, Franz, & Teubner, Ulrich. Time-resolved ionization measurements with intense ultrashort XUV and X-ray free-electron laser pulses. United States. https://doi.org/10.1017/s0263034619000326
Copy to clipboard
Tkachenko, Victor, Büscher, Martin, Höppner, Hauke, Medvedev, Nikita, Lipp, Vladimir, Rossi, Giulio Maria, Capotondi, Flavio, Finetti, Paola, Pedersoli, Emanuele, Nikolov, Ivaylo, Danailov, Mitcho, Giannessi, Luca, Prandolini, Mark J., Toleikis, Sven, Mecseki, Katalin, Windeler, Matthew, Ziaja, Beata, Tavella, Franz, and Teubner, Ulrich. Mon . "Time-resolved ionization measurements with intense ultrashort XUV and X-ray free-electron laser pulses". United States. https://doi.org/10.1017/s0263034619000326. https://www.osti.gov/servlets/purl/1547231.
Copy to clipboard
@article{osti_1547231,
title = {Time-resolved ionization measurements with intense ultrashort XUV and X-ray free-electron laser pulses},
author = {Tkachenko, Victor and Büscher, Martin and Höppner, Hauke and Medvedev, Nikita and Lipp, Vladimir and Rossi, Giulio Maria and Capotondi, Flavio and Finetti, Paola and Pedersoli, Emanuele and Nikolov, Ivaylo and Danailov, Mitcho and Giannessi, Luca and Prandolini, Mark J. and Toleikis, Sven and Mecseki, Katalin and Windeler, Matthew and Ziaja, Beata and Tavella, Franz and Teubner, Ulrich},
abstractNote = {Abstract Modern free-electron lasers (FEL) operating in XUV (extreme ultraviolet) or X-ray range allow an access to novel research areas. One instance is the ultrafast ionization of a solid by an intense femtosecond FEL pulse in XUV which consequently leads to a change of the complex index of refraction on an ultrashort timescale. The photoionization and subsequent impact ionization resulting in electronic and atomic dynamics are modeled with our hybrid code XTANT(X-ray thermal and non-thermal transitions) and a Monte Carlo code XCASCADE(X-ray-induced electron cascades). The simulations predict the temporal kinetics of FEL-induced electron cascades and thus yield temporally and spatially resolved information on the induced changes of the optical properties. In a series of experiments at FERMI and LCLS, single shot measurements with spatio-temporal encoding of the ionization process have been performed by a correlation of the FEL pump pulse with an optical femtosecond probe pulse. An excellent agreement between the experiment and the simulation has been found. Furthermore, we demonstrate that such kind of experiments forms the basis for pulse duration and arrival time jitter monitoring as currently under development for XUV-FELs.},
doi = {10.1017/s0263034619000326},
journal = {Laser and Particle Beams},
number = 2,
volume = 37,
place = {United States},
year = {2019},
month = {4}
}
Copy to clipboard
Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1017/s0263034619000326
Copyright Statement
Other availability
Search WorldCat Search WorldCat to find libraries that may hold this journal
Citation Metrics:
Cited by: 1 work
Citation information provided by
Web of Science
Save / Share:
Export Metadata
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.

Works referenced in this record:

Photon energy dependence of graphitization threshold for diamond irradiated with an intense XUV FEL pulse
journal, August 2013

Highly coherent and stable pulses from the FERMI seeded free-electron laser in the extreme ultraviolet
journal, September 2012

Pulse Duration of Seeded Free-Electron Lasers
journal, June 2017

Femtosecond X-ray induced electron kinetics in dielectrics: application for FEL-pulse-duration monitor
journal, January 2015

The free-electron laser FLASH
journal, January 2015

  • Schreiber, Siegfried; Faatz, Bart
  • High Power Laser Science and Engineering, Vol. 3
  • DOI: 10.1017/hpl.2015.16

First lasing and operation of an ångstrom-wavelength free-electron laser
journal, August 2010

Transient Changes of Optical Properties in Semiconductors in Response to Femtosecond Laser Pulses
journal, August 2016

  • Tkachenko, Victor; Medvedev, Nikita; Ziaja, Beata
  • Applied Sciences, Vol. 6, Issue 9
  • DOI: 10.3390/app6090238

The European X-ray free-electron laser facility in Hamburg
journal, December 2011

  • Altarelli, M.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 269, Issue 24
  • DOI: 10.1016/j.nimb.2011.04.034

Nonthermal phase transitions in semiconductors induced by a femtosecond extreme ultraviolet laser pulse
journal, January 2013

Soft x-ray induced femtosecond solid-to-solid phase transition
journal, September 2017

Single-shot timing measurement of extreme-ultraviolet free-electron laser pulses
journal, March 2008

Hard X-ray free-electron laser with femtosecond-scale timing jitter
journal, October 2017

Hard X-ray induced fast secondary electron cascading processes in solids
journal, September 2018

  • Mecseki, K.; Höppner, H.; Büscher, M.
  • Applied Physics Letters, Vol. 113, Issue 11
  • DOI: 10.1063/1.5046070

Thermal and nonthermal melting of silicon under femtosecond x-ray irradiation
journal, February 2015

First light from SACLA
journal, July 2011

Sub-10 fs gating of optical pulses
journal, July 2001

  • Teubner, U.; Wagner, U.; Förster, E.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 34, Issue 15
  • DOI: 10.1088/0953-4075/34/15/306

Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers
journal, February 2013

Transient optical properties of semiconductors under femtosecond x-ray irradiation
journal, April 2016

Picosecond relaxation of X-ray excited GaAs
journal, September 2017

Multistep transition of diamond to warm dense matter state revealed by femtosecond X-ray diffraction
journal, March 2018

Tight-binding calculation of the optical absorption cross section of spherical and ellipsoidal silicon nanocrystals
journal, August 2005

    Sort by:
    [ × clear filter / sort ]

    Works referencing / citing this record:

      Sort by:
      [ × clear filter / sort ]

      Similar Records in DOE PAGES and OSTI.GOV collections: