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Title: Progress and Perspectives of Electrochemical CO 2 Reduction on Copper in Aqueous Electrolyte

Authors:
 [1]; ORCiD logo [2];  [2];  [1];  [3];  [2];  [2]; ORCiD logo [4]; ORCiD logo [5]; ORCiD logo [5];  [6]; ORCiD logo [5]; ORCiD logo [2]
  1. SUNCAT Center for Interface Science and Catalysis, Department of Chemical Engineering, Stanford University, Stanford, California 94305, United States
  2. Section for Surface Physics and Catalysis, Department of Physics, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark
  3. Section for Surface Physics and Catalysis, Department of Physics, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark, Institute of Surface Chemistry and Catalysis, Ulm University, D-89069 Ulm, Germany
  4. Section for Surface Physics and Catalysis, Department of Physics, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark, Department of Materials, Imperial College London, Royal School of Mines, London SW7 2AZ, United Kingdom
  5. SUNCAT Center for Interface Science and Catalysis, Department of Chemical Engineering, Stanford University, Stanford, California 94305, United States, SUNCAT Center for Interface Science and Catalysis, SLAC National Accelerator Laboratory, Menlo Park, California 94025, United States
  6. SUNCAT Center for Interface Science and Catalysis, Department of Chemical Engineering, Stanford University, Stanford, California 94305, United States, Section for Surface Physics and Catalysis, Department of Physics, Technical University of Denmark, 2800 Kgs. Lyngby, Denmark, SUNCAT Center for Interface Science and Catalysis, SLAC National Accelerator Laboratory, Menlo Park, California 94025, United States
Publication Date:
Research Org.:
California Institute of Technology (CalTech), Pasadena, CA (United States); SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); European Research Council (ERC)
OSTI Identifier:
1529643
Alternate Identifier(s):
OSTI ID: 1529484; OSTI ID: 1546977
Grant/Contract Number:  
SC0004993; AC02-76SF00515; 9455; 8057-00018B
Resource Type:
Published Article
Journal Name:
Chemical Reviews
Additional Journal Information:
Journal Name: Chemical Reviews Journal Volume: 119 Journal Issue: 12; Journal ID: ISSN 0009-2665
Publisher:
American Chemical Society
Country of Publication:
United States
Language:
English
Subject:
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats

Nitopi, Stephanie, Bertheussen, Erlend, Scott, Soren B., Liu, Xinyan, Engstfeld, Albert K., Horch, Sebastian, Seger, Brian, Stephens, Ifan E. L., Chan, Karen, Hahn, Christopher, Nørskov, Jens K., Jaramillo, Thomas F., and Chorkendorff, Ib. Progress and Perspectives of Electrochemical CO 2 Reduction on Copper in Aqueous Electrolyte. United States: N. p., 2019. Web. doi:10.1021/acs.chemrev.8b00705.
Nitopi, Stephanie, Bertheussen, Erlend, Scott, Soren B., Liu, Xinyan, Engstfeld, Albert K., Horch, Sebastian, Seger, Brian, Stephens, Ifan E. L., Chan, Karen, Hahn, Christopher, Nørskov, Jens K., Jaramillo, Thomas F., & Chorkendorff, Ib. Progress and Perspectives of Electrochemical CO 2 Reduction on Copper in Aqueous Electrolyte. United States. https://doi.org/10.1021/acs.chemrev.8b00705
Nitopi, Stephanie, Bertheussen, Erlend, Scott, Soren B., Liu, Xinyan, Engstfeld, Albert K., Horch, Sebastian, Seger, Brian, Stephens, Ifan E. L., Chan, Karen, Hahn, Christopher, Nørskov, Jens K., Jaramillo, Thomas F., and Chorkendorff, Ib. Wed . "Progress and Perspectives of Electrochemical CO 2 Reduction on Copper in Aqueous Electrolyte". United States. https://doi.org/10.1021/acs.chemrev.8b00705.
@article{osti_1529643,
title = {Progress and Perspectives of Electrochemical CO 2 Reduction on Copper in Aqueous Electrolyte},
author = {Nitopi, Stephanie and Bertheussen, Erlend and Scott, Soren B. and Liu, Xinyan and Engstfeld, Albert K. and Horch, Sebastian and Seger, Brian and Stephens, Ifan E. L. and Chan, Karen and Hahn, Christopher and Nørskov, Jens K. and Jaramillo, Thomas F. and Chorkendorff, Ib},
abstractNote = {},
doi = {10.1021/acs.chemrev.8b00705},
journal = {Chemical Reviews},
number = 12,
volume = 119,
place = {United States},
year = {Wed May 22 00:00:00 EDT 2019},
month = {Wed May 22 00:00:00 EDT 2019}
}

Journal Article:
Free Publicly Available Full Text
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https://doi.org/10.1021/acs.chemrev.8b00705

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  • Journal of Materials Chemistry A, Vol. 3, Issue 47
  • DOI: 10.1039/C5TA06804E

Electrochemical Carbon Dioxide Reduction at Nanostructured Gold, Copper, and Alloy Materials
journal, March 2017

  • Vickers, James W.; Alfonso, Dominic; Kauffman, Douglas R.
  • Energy Technology, Vol. 5, Issue 6
  • DOI: 10.1002/ente.201600580

Reduction of carbon dioxide to methane and ethene—an on-line MS study with rotating electrodes
journal, April 1990


The Evolution of the Polycrystalline Copper Surface, First to Cu(111) and Then to Cu(100), at a Fixed CO 2 RR Potential: A Study by Operando EC-STM
journal, December 2014

  • Kim, Youn-Geun; Baricuatro, Jack Hess; Javier, Alnald
  • Langmuir, Vol. 30, Issue 50
  • DOI: 10.1021/la504445g

Activity Descriptors for CO 2 Electroreduction to Methane on Transition-Metal Catalysts
journal, January 2012

  • Peterson, Andrew A.; Nørskov, Jens K.
  • The Journal of Physical Chemistry Letters, Vol. 3, Issue 2
  • DOI: 10.1021/jz201461p

Alkalinity Initiated Decomposition of Mediating Imidazolium Ions in High Current Density CO 2 Electrolysis
journal, October 2016

  • Neubauer, Sebastian S.; Schmid, Bernhard; Reller, Christian
  • ChemElectroChem, Vol. 4, Issue 1
  • DOI: 10.1002/celc.201600461

Metal-Free Carbon Materials for CO 2 Electrochemical Reduction
journal, September 2017


Low-Overpotential Electroreduction of Carbon Monoxide Using Copper Nanowires
journal, June 2017


Regulating the Product Distribution of CO Reduction by the Atomic-Level Structural Modification of the Cu Electrode Surface
journal, June 2016


Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
journal, November 2004

  • Nørskov, J. K.; Rossmeisl, J.; Logadottir, A.
  • The Journal of Physical Chemistry B, Vol. 108, Issue 46
  • DOI: 10.1021/jp047349j

A comprehensive review on PEM water electrolysis
journal, April 2013

  • Carmo, Marcelo; Fritz, David L.; Mergel, Jürgen
  • International Journal of Hydrogen Energy, Vol. 38, Issue 12, p. 4901-4934
  • DOI: 10.1016/j.ijhydene.2013.01.151

Frontiers, Opportunities, and Challenges in Biochemical and Chemical Catalysis of CO 2 Fixation
journal, June 2013

  • Appel, Aaron M.; Bercaw, John E.; Bocarsly, Andrew B.
  • Chemical Reviews, Vol. 113, Issue 8
  • DOI: 10.1021/cr300463y

Structure Sensitivity of the Electrochemical Reduction of Carbon Monoxide on Copper Single Crystals
journal, April 2013

  • Schouten, Klaas Jan P.; Pérez Gallent, Elena; Koper, Marc T. M.
  • ACS Catalysis, Vol. 3, Issue 6
  • DOI: 10.1021/cs4002404

Cyclic Voltammograms for H on Pt(111) and Pt(100) from First Principles
journal, September 2007


One-step electrosynthesis of ethylene and ethanol from CO2 in an alkaline electrolyzer
journal, January 2016