Anchoring carbon nanotubes and post-hydroxylation treatment enhanced Ni nanofiber catalysts towards efficient hydrous hydrazine decomposition for effective hydrogen generation

Yang, Pan; Yang, Lijun; Gao, Qiang; Luo, Qiang; Zhao, Xiaochong; Mai, Xianmin; Fu, Qinglong; Dong, Mengyao; Wang, Jingchuan; Hao, Yawei; Yang, Ruizhu; Lai, Xinchun; Wu, Shide; Shao, Qian; Ding, Tao; Lin, Jing; Guo, Zhanhu

doi:10.1039/C9CC04559G

Title: Anchoring carbon nanotubes and post-hydroxylation treatment enhanced Ni nanofiber catalysts towards efficient hydrous hydrazine decomposition for effective hydrogen generation

Journal Article · 27 June 2019 · ChemComm

DOI: https://doi.org/10.1039/C9CC04559G · OSTI ID:1546532

Yang, Pan ^[1];

^[1];

^[2]; Luo, Qiang ^[3];

^[1]; Mai, Xianmin ^[4]; Fu, Qinglong ^[1]; Dong, Mengyao ^[5]; Wang, Jingchuan ^[1]; Hao, Yawei ^[1]; Yang, Ruizhu ^[1]; Lai, Xinchun ^[1]; Wu, Shide ^[6]; Shao, Qian ^[7]; Ding, Tao ^[8]; Lin, Jing ^[9];

^[10]

Chinese Academy of Engineering Physics, Jiangyou (China)
Max Planck Inst. for Chemical Energy Conversion, Mülheim (Germany)
Hainan Univ., Haikou (China); Univ. of Tennessee, Knoxville, TN (United States)
Southwest Minzu Univ., Chengdu (China)
Univ. of Tennessee, Knoxville, TN (United States); Zhengzhou Univ., Zhengzhou (China)
Zhengzhou Univ. of Light Industry, Zhengzhou (China)
Shandong Univ. of Science and Technology, Qingdao (China)
Henan Univ., Kaifeng (China)
Guangzhou Univ., Guangzhou (China)
Univ. of Tennessee, Knoxville, TN (United States)

For effective hydrogen generation with remarkable durability, carbon nanotubes (CNTs) grown on Ni nanofibers and their post hydroxylation treatment engendered active Ni nanofiber catalysts an efficient decomposition of hydrous hydrazine with a turnover frequency (TOF) of 19.4 h^-1 and an activation energy down to 51.05 KJ mol^-1.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE; National Natural Science Foundation of China (NNSFC)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1546532

Journal Information:: ChemComm, Journal Name: ChemComm Journal Issue: 61 Vol. 55; ISSN CHCOFS; ISSN 1359-7345

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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