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Title: Fourth order expressions for the electronic absorption lineshape of molecular excitons

Authors:
ORCiD logo [1]
  1. Department of Chemistry and Biochemistry, Queens College, City University of New York, 65-30 Kissena Boulevard, Queens, New York 11367, USA and Ph.D. Programs in Chemistry and Physics, and Initiative for Theoretical Sciences, Graduate Center, City University of New York, 365 Fifth Avenue, New York, New York 10016, USA
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1545412
Grant/Contract Number:  
SC0001393
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Journal of Chemical Physics
Additional Journal Information:
Journal Name: Journal of Chemical Physics Journal Volume: 151 Journal Issue: 4; Journal ID: ISSN 0021-9606
Publisher:
American Institute of Physics
Country of Publication:
United States
Language:
English

Citation Formats

Jang, Seogjoo J. Fourth order expressions for the electronic absorption lineshape of molecular excitons. United States: N. p., 2019. Web. doi:10.1063/1.5100986.
Jang, Seogjoo J. Fourth order expressions for the electronic absorption lineshape of molecular excitons. United States. doi:10.1063/1.5100986.
Jang, Seogjoo J. Sun . "Fourth order expressions for the electronic absorption lineshape of molecular excitons". United States. doi:10.1063/1.5100986.
@article{osti_1545412,
title = {Fourth order expressions for the electronic absorption lineshape of molecular excitons},
author = {Jang, Seogjoo J.},
abstractNote = {},
doi = {10.1063/1.5100986},
journal = {Journal of Chemical Physics},
number = 4,
volume = 151,
place = {United States},
year = {2019},
month = {7}
}

Journal Article:
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This content will become publicly available on July 29, 2020
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Works referenced in this record:

Absorption lineshapes of molecular aggregates revisited
journal, April 2015

  • Gelzinis, Andrius; Abramavicius, Darius; Valkunas, Leonas
  • The Journal of Chemical Physics, Vol. 142, Issue 15
  • DOI: 10.1063/1.4918343

Extending the applicability of Redfield theories into highly non-Markovian regimes
journal, November 2015

  • Montoya-Castillo, Andrés; Berkelbach, Timothy C.; Reichman, David R.
  • The Journal of Chemical Physics, Vol. 143, Issue 19
  • DOI: 10.1063/1.4935443

The Time-Convolutionless Projection Operator Technique in the Quantum Theory of Dissipation and Decoherence
journal, July 2001

  • Breuer, Heinz-Peter; Kappler, Bernd; Petruccione, Francesco
  • Annals of Physics, Vol. 291, Issue 1
  • DOI: 10.1006/aphy.2001.6152

Lineshape theory of pigment-protein complexes: How the finite relaxation time of nuclei influences the exciton relaxation-induced lifetime broadening
journal, July 2016

  • Dinh, Thanh-Chung; Renger, Thomas
  • The Journal of Chemical Physics, Vol. 145, Issue 3
  • DOI: 10.1063/1.4958322

Coherent Two-Dimensional Optical Spectroscopy
journal, April 2008


On the accuracy of the Padé-resummed master equation approach to dissipative quantum dynamics
journal, April 2016

  • Chen, Hsing-Ta; Berkelbach, Timothy C.; Reichman, David R.
  • The Journal of Chemical Physics, Vol. 144, Issue 15
  • DOI: 10.1063/1.4946809

Linear and nonlinear spectroscopy from quantum master equations
journal, December 2017

  • Fetherolf, Jonathan H.; Berkelbach, Timothy C.
  • The Journal of Chemical Physics, Vol. 147, Issue 24
  • DOI: 10.1063/1.5006824

Optical properties of disordered molecular aggregates: A numerical study
journal, December 1991

  • Fidder, Henk; Knoester, Jasper; Wiersma, Douwe A.
  • The Journal of Chemical Physics, Vol. 95, Issue 11
  • DOI: 10.1063/1.461317

Resummed memory kernels in generalized system-bath master equations
journal, August 2014

  • Mavros, Michael G.; Van Voorhis, Troy
  • The Journal of Chemical Physics, Vol. 141, Issue 5
  • DOI: 10.1063/1.4891669

The absorption line shape for a molecular system stochastically coupled to a phonon thermal reservoir
journal, April 1988

  • Faid, Karim; Fox, Ronald F.
  • The Journal of Chemical Physics, Vol. 88, Issue 8
  • DOI: 10.1063/1.453770

Dynamics of non-Markovian open quantum systems
journal, January 2017


Energy transfer and spectral line shapes of impurities in crystals
journal, September 1975

  • Abram, I. I.; Silbey, R.
  • The Journal of Chemical Physics, Vol. 63, Issue 6
  • DOI: 10.1063/1.431683

Fourth-order quantum master equation and its Markovian bath limit
journal, February 2002

  • Jang, Seogjoo; Cao, Jianshu; Silbey, Robert J.
  • The Journal of Chemical Physics, Vol. 116, Issue 7
  • DOI: 10.1063/1.1445105

Single-Molecule Study of the Electronic Couplings in a Circular Array of Molecules: Light-Harvesting-2 Complex from Rhodospirillum Molischianum
journal, January 2003


Reference system master equation approaches to condensed phase charge transfer processes. I. General formulation
journal, December 2001

  • Golosov, Andrei A.; Reichman, David R.
  • The Journal of Chemical Physics, Vol. 115, Issue 21
  • DOI: 10.1063/1.1412611

Theory of single molecule line shapes of multichromophoric macromolecules
journal, May 2003

  • Jang, Seogjoo; Silbey, Robert J.
  • The Journal of Chemical Physics, Vol. 118, Issue 20
  • DOI: 10.1063/1.1569239

Optical line shapes of molecular aggregates: Hierarchical equations of motion method
journal, January 2009

  • Chen, Liping; Zheng, Renhui; Shi, Qiang
  • The Journal of Chemical Physics, Vol. 131, Issue 9
  • DOI: 10.1063/1.3213013

Two-dimensional optical spectroscopy of molecular aggregates
journal, January 2010

  • Butkus, Vytautas; Abramavicius, D.; Gelzinis, A.
  • Lithuanian Journal of Physics, Vol. 50, Issue 3
  • DOI: 10.3952/lithjphys.50305

Critical tests of a new master equation approach to nonadiabatic quantum dissipative systems
journal, January 2004


Analytic representations of bath correlation functions for ohmic and superohmic spectral densities using simple poles
journal, September 2014

  • Ritschel, Gerhard; Eisfeld, Alexander
  • The Journal of Chemical Physics, Vol. 141, Issue 9
  • DOI: 10.1063/1.4893931

Reduced dynamics of coupled harmonic and anharmonic oscillators using higher-order perturbation theory
journal, March 2007

  • Schröder, Markus; Schreiber, Michael; Kleinekathöfer, Ulrich
  • The Journal of Chemical Physics, Vol. 126, Issue 11
  • DOI: 10.1063/1.2538754

Stochastic Theory of Line Shape: Generalization of the Kubo-Anderson Model
journal, October 1968


Non-Markovian theories based on a decomposition of the spectral density
journal, January 2004

  • Kleinekathöfer, Ulrich
  • The Journal of Chemical Physics, Vol. 121, Issue 6
  • DOI: 10.1063/1.1770619

A reduced density-matrix theory of absorption line shape of molecular aggregate
journal, September 2005

  • Yang, Mino
  • The Journal of Chemical Physics, Vol. 123, Issue 12
  • DOI: 10.1063/1.2046668

On the conundrum of deriving exact solutions from approximate master equations
journal, May 2008


Quantum‐mechanical derivation of the Bloch equations: Beyond the weak‐coupling limit
journal, March 1991

  • Laird, Brian B.; Budimir, Jane; Skinner, James L.
  • The Journal of Chemical Physics, Vol. 94, Issue 6
  • DOI: 10.1063/1.460626

Excitons in Conjugated Oligomer Aggregates, Films, and Crystals
journal, May 2006


T 2 can be greater than 2 T 1 even at finite temperature
journal, March 1991

  • Laird, Brian B.; Skinner, James L.
  • The Journal of Chemical Physics, Vol. 94, Issue 6
  • DOI: 10.1063/1.460627

Higher-order kinetic expansion of quantum dissipative dynamics: Mapping quantum networks to kinetic networks
journal, July 2013

  • Wu, Jianlan; Cao, Jianshu
  • The Journal of Chemical Physics, Vol. 139, Issue 4
  • DOI: 10.1063/1.4812781

Probing Photophysical Processes in Individual Multichromophoric Dendrimers by Single-Molecule Spectroscopy
journal, September 2000

  • Hofkens, Johan; Maus, Michael; Gensch, Thomas
  • Journal of the American Chemical Society, Vol. 122, Issue 38
  • DOI: 10.1021/ja0012570

Convergence of high order memory kernels in the Nakajima-Zwanzig generalized master equation and rate constants: Case study of the spin-boson model
journal, April 2018

  • Xu, Meng; Yan, Yaming; Liu, Yanying
  • The Journal of Chemical Physics, Vol. 148, Issue 16
  • DOI: 10.1063/1.5022761

The non-Markovian quantum master equation in the collective-mode representation: Application to barrier crossing in the intermediate friction regime
journal, November 2005

  • Pomyalov, Anna; Tannor, David J.
  • The Journal of Chemical Physics, Vol. 123, Issue 20
  • DOI: 10.1063/1.2121649

Delocalized excitons in natural light-harvesting complexes
journal, August 2018


Nonequilibrium quantum dynamics in the condensed phase via the generalized quantum master equation
journal, July 2006

  • Zhang, Ming-Liang; Ka, Being J.; Geva, Eitan
  • The Journal of Chemical Physics, Vol. 125, Issue 4
  • DOI: 10.1063/1.2218342

Towards an exact theory of linear absorbance and circular dichroism of pigment-protein complexes: Importance of non-secular contributions
journal, January 2015

  • Dinh, Thanh-Chung; Renger, Thomas
  • The Journal of Chemical Physics, Vol. 142, Issue 3
  • DOI: 10.1063/1.4904928

A new approach to calculating the memory kernel of the generalized quantum master equation for an arbitrary system–bath coupling
journal, December 2003

  • Shi, Qiang; Geva, Eitan
  • The Journal of Chemical Physics, Vol. 119, Issue 23
  • DOI: 10.1063/1.1624830

Revealing the Electron–Phonon Coupling in a Conjugated Polymer by Single-Molecule Spectroscopy
journal, August 2007


Expanded Theory of H- and J-Molecular Aggregates: The Effects of Vibronic Coupling and Intermolecular Charge Transfer
journal, April 2018


Calculation of absorption spectra for light-harvesting systems using non-Markovian approaches as well as modified Redfield theory
journal, February 2006

  • Schröder, Markus; Kleinekathöfer, Ulrich; Schreiber, Michael
  • The Journal of Chemical Physics, Vol. 124, Issue 8
  • DOI: 10.1063/1.2171188