Self referencing attosecond interferometer with zeptosecond precision
Abstract
In this work we demonstrate the generation of two intense, ultrafast laser pulses that allow a controlled interferometric measurement of higher harmonic generation pulses with 12.8 attoseconds in resolution (half the atomic unit of time) and a precision as low as 680 zeptoseconds (10–21 seconds). We create two replicas of a driving femtosecond pulse which share the same optical path except at the focus where they converge to two foci. An attosecond pulse train emerges from each focus through the process of high harmonic generation. The two attosecond pulse trains from each focus interfere in the far field producing a clear interference pattern in the extreme ultraviolet region. By controlling the relative optical phase (carrier envelope phase for pulsed fields) between the two driving laser pulses we are able to actively influence the delay between the pulses and are able to perform very stable and precise pump-probe experiments. Because of the phase shaping operation occurs homogeneously across the entire spatial profile, we effectively create two indistinguishable intense laser pulses or a common path interferometer for attosecond pulses. Commonality across the two beams means that they are extremely stable to environmental and mechanical fluctuations up to a Rayleigh range from themore »
- Authors:
- Publication Date:
- Research Org.:
- Kansas State Univ., Manhattan, KS (United States); Univ. of Connecticut, Storrs, CT (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1545179
- Alternate Identifier(s):
- OSTI ID: 1610057
- Grant/Contract Number:
- FG02-86ER13491; SC0019098
- Resource Type:
- Published Article
- Journal Name:
- Optics Express
- Additional Journal Information:
- Journal Name: Optics Express Journal Volume: 27 Journal Issue: 16; Journal ID: ISSN 1094-4087
- Publisher:
- Optical Society of America (OSA)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Optics
Citation Formats
Tross, Jan, Kolliopoulos, Georgios, and Trallero-Herrero, Carlos A. Self referencing attosecond interferometer with zeptosecond precision. United States: N. p., 2019.
Web. doi:10.1364/OE.27.022960.
Tross, Jan, Kolliopoulos, Georgios, & Trallero-Herrero, Carlos A. Self referencing attosecond interferometer with zeptosecond precision. United States. https://doi.org/10.1364/OE.27.022960
Tross, Jan, Kolliopoulos, Georgios, and Trallero-Herrero, Carlos A. Fri .
"Self referencing attosecond interferometer with zeptosecond precision". United States. https://doi.org/10.1364/OE.27.022960.
@article{osti_1545179,
title = {Self referencing attosecond interferometer with zeptosecond precision},
author = {Tross, Jan and Kolliopoulos, Georgios and Trallero-Herrero, Carlos A.},
abstractNote = {In this work we demonstrate the generation of two intense, ultrafast laser pulses that allow a controlled interferometric measurement of higher harmonic generation pulses with 12.8 attoseconds in resolution (half the atomic unit of time) and a precision as low as 680 zeptoseconds (10–21 seconds). We create two replicas of a driving femtosecond pulse which share the same optical path except at the focus where they converge to two foci. An attosecond pulse train emerges from each focus through the process of high harmonic generation. The two attosecond pulse trains from each focus interfere in the far field producing a clear interference pattern in the extreme ultraviolet region. By controlling the relative optical phase (carrier envelope phase for pulsed fields) between the two driving laser pulses we are able to actively influence the delay between the pulses and are able to perform very stable and precise pump-probe experiments. Because of the phase shaping operation occurs homogeneously across the entire spatial profile, we effectively create two indistinguishable intense laser pulses or a common path interferometer for attosecond pulses. Commonality across the two beams means that they are extremely stable to environmental and mechanical fluctuations up to a Rayleigh range from the focus. In our opinion this represents an ideal source for homodyne and heterodyne spectroscopic measurements with sub-attosecond precision.},
doi = {10.1364/OE.27.022960},
journal = {Optics Express},
number = 16,
volume = 27,
place = {United States},
year = {2019},
month = {7}
}
https://doi.org/10.1364/OE.27.022960
Web of Science
Works referenced in this record:
Atomic transient recorder
journal, February 2004
- Kienberger, R.; Goulielmakis, E.; Uiberacker, M.
- Nature, Vol. 427, Issue 6977
Atomic scale temporal structure inherent to high-order harmonic generation
journal, July 1993
- Harris, S. E.; Macklin, J. J.; Hänsch, T. W.
- Optics Communications, Vol. 100, Issue 5-6
Time-Resolved Dynamics in N2O4 Probed Using High Harmonic Generation
journal, November 2008
- Li, W.; Zhou, X.; Lock, R.
- Science, Vol. 322, Issue 5905
Phase-locked pulses for two-dimensional spectroscopy by a birefringent delay line
journal, January 2012
- Brida, Daniele; Manzoni, Cristian; Cerullo, Giulio
- Optics Letters, Vol. 37, Issue 15
Electronic wavefunctions probed by all-optical attosecond interferometry
journal, December 2018
- Azoury, Doron; Kneller, Omer; Rozen, Shaked
- Nature Photonics, Vol. 13, Issue 1
Theory of high-harmonic generation by low-frequency laser fields
journal, March 1994
- Lewenstein, M.; Balcou, Ph.; Ivanov, M. Yu.
- Physical Review A, Vol. 49, Issue 3
High-order harmonic generation from atoms and ions in the high intensity regime
journal, June 1992
- Krause, Jeffrey L.; Schafer, Kenneth J.; Kulander, Kenneth C.
- Physical Review Letters, Vol. 68, Issue 24
Molecular Recollision Interferometry in High Harmonic Generation
journal, February 2008
- Zhou, Xibin; Lock, Robynne; Li, Wen
- Physical Review Letters, Vol. 100, Issue 7
Attosecond control of electronic processes by intense light fields
journal, February 2003
- Baltuška, A.; Udem, Th.; Uiberacker, M.
- Nature, Vol. 421, Issue 6923, p. 611-615
Linked attosecond phase interferometry for molecular frame measurements
journal, February 2013
- Bertrand, J. B.; Wörner, H. J.; Salières, P.
- Nature Physics, Vol. 9, Issue 3
High-order harmonic generation in rare gases with a 1-ps 1053-nm laser
journal, February 1993
- L’Huillier, Anne; Balcou, Ph.
- Physical Review Letters, Vol. 70, Issue 6
Zeptosecond precision pulse shaping
journal, January 2011
- Köhler, Jens; Wollenhaupt, Matthias; Bayer, Tim
- Optics Express, Vol. 19, Issue 12
Methods for the measurement of the duration of high-harmonic pulses
journal, November 1997
- Constant, Eric; Taranukhin, Vladimir D.; Stolow, Albert
- Physical Review A, Vol. 56, Issue 5
Generation of a strong attosecond pulse train with an orthogonally polarized two-color laser field
journal, September 2005
- Kim, Chul Min; Kim, I. Jong; Nam, Chang Hee
- Physical Review A, Vol. 72, Issue 3
Generalized phase-matching conditions for high harmonics: The role of field-gradient forces
journal, April 1997
- Balcou, Philippe; Sali`eres, Pascal; L'Huillier, Anne
- Physical Review A, Vol. 55, Issue 4
Observation of a Train of Attosecond Pulses from High Harmonic Generation
journal, June 2001
- Paul, P. M.
- Science, Vol. 292, Issue 5522
High-harmonic phase spectroscopy using a binary diffractive optical element
journal, April 2014
- Camper, A.; Ruchon, T.; Gauthier, D.
- Physical Review A, Vol. 89, Issue 4
Attosecond Streak Camera
journal, April 2002
- Itatani, J.; Quéré, F.; Yudin, G. L.
- Physical Review Letters, Vol. 88, Issue 17
Phase-Locked High-Order Harmonic Sources
journal, August 1997
- Zerne, Raoul; Altucci, Carlo; Bellini, Marco
- Physical Review Letters, Vol. 79, Issue 6
Single-shot autocorrelator for extreme-ultraviolet radiation
journal, January 2014
- Kolliopoulos, G.; Tzallas, P.; Bergues, B.
- Journal of the Optical Society of America B, Vol. 31, Issue 5
Attosecond Synchronization of High-Harmonic Soft X-rays
journal, November 2003
- Mairesse, Y.
- Science, Vol. 302, Issue 5650
Attosecond metrology
journal, November 2001
- Hentschel, M.; Kienberger, R.; Spielmann, Ch.
- Nature, Vol. 414, Issue 6863, p. 509-513
Selection of an electron path of high-order harmonic generation in a two-colour femtosecond laser field
journal, July 2006
- Kim, Chul Min; Nam, Chang Hee
- Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 39, Issue 16
Vectorial optical field reconstruction by attosecond spatial interferometry
journal, May 2017
- Carpeggiani, P.; Reduzzi, M.; Comby, A.
- Nature Photonics, Vol. 11, Issue 6
Direct observation of attosecond light bunching
journal, November 2003
- Tzallas, P.; Charalambidis, D.; Papadogiannis, N. A.
- Nature, Vol. 426, Issue 6964
Isolated Single-Cycle Attosecond Pulses
journal, October 2006
- Sansone, G.; Benedetti, E.; Calegari, F.
- Science, Vol. 314, Issue 5798
Attosecond correlation dynamics
journal, November 2016
- Ossiander, M.; Siegrist, F.; Shirvanyan, V.
- Nature Physics, Vol. 13, Issue 3
Frequency-resolved optical gating for complete reconstruction of attosecond bursts
journal, January 2005
- Mairesse, Y.; Quéré, F.
- Physical Review A, Vol. 71, Issue 1
Tomographic imaging of molecular orbitals
journal, December 2004
- Itatani, J.; Levesque, J.; Zeidler, D.
- Nature, Vol. 432, Issue 7019
High harmonic interferometry of multi-electron dynamics in molecules
journal, July 2009
- Smirnova, Olga; Mairesse, Yann; Patchkovskii, Serguei
- Nature, Vol. 460, Issue 7258
Petahertz optical oscilloscope
journal, November 2013
- Kim, Kyung Taec; Zhang, Chunmei; Shiner, Andrew D.
- Nature Photonics, Vol. 7, Issue 12
Octave-spanning hyperspectral coherent diffractive imaging in the extreme ultraviolet range
journal, January 2015
- Meng, Yijian; Zhang, Chunmei; Marceau, Claude
- Optics Express, Vol. 23, Issue 22