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Title: Near room temperature antiferromagnetic ordering with a potential low-dimensional magnetism in AlMn 2 B 2

Abstract

Here, we report on self flux growth and characterization of single crystalline AlMn 2 B 2 . It is an orthorhombic (space group $Cmmm$), layered material with a platelike morphology. The anisotropic bulk magnetization data, electrical transport, and 11B nuclear magnetic resonance (NMR) data revealed an antiferromagnetic (AFM) transition at 313 ± 2 K . In the magnetization data, there is also a broad local maximum critically above the AFM transition that could be a signature of low-dimensional magnetic interactions in AlMn 2 B 2 .

Authors:
 [1];  [1];  [1];  [1];  [1];  [1]
  1. Ames Lab. and Iowa State Univ., Ames, IA (United States)
Publication Date:
Research Org.:
Ames Laboratory (AMES), Ames, IA (United States)
Sponsoring Org.:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Advanced Manufacturing Office (EE-5A); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division
OSTI Identifier:
1542871
Alternate Identifier(s):
OSTI ID: 1530004
Report Number(s):
IS-J-9976
Journal ID: ISSN 2475-9953; PRMHAR
Grant/Contract Number:  
AC02-07CH11358
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review Materials
Additional Journal Information:
Journal Volume: 3; Journal Issue: 6; Journal ID: ISSN 2475-9953
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Lamichhane, Tej N., Rana, Khusboo, Lin, Qisheng, Bud'ko, Sergey L., Furukawa, Yuji, and Canfield, Paul C. Near room temperature antiferromagnetic ordering with a potential low-dimensional magnetism in AlMn2B2. United States: N. p., 2019. Web. doi:10.1103/PhysRevMaterials.3.064415.
Lamichhane, Tej N., Rana, Khusboo, Lin, Qisheng, Bud'ko, Sergey L., Furukawa, Yuji, & Canfield, Paul C. Near room temperature antiferromagnetic ordering with a potential low-dimensional magnetism in AlMn2B2. United States. doi:10.1103/PhysRevMaterials.3.064415.
Lamichhane, Tej N., Rana, Khusboo, Lin, Qisheng, Bud'ko, Sergey L., Furukawa, Yuji, and Canfield, Paul C. Fri . "Near room temperature antiferromagnetic ordering with a potential low-dimensional magnetism in AlMn2B2". United States. doi:10.1103/PhysRevMaterials.3.064415.
@article{osti_1542871,
title = {Near room temperature antiferromagnetic ordering with a potential low-dimensional magnetism in AlMn2B2},
author = {Lamichhane, Tej N. and Rana, Khusboo and Lin, Qisheng and Bud'ko, Sergey L. and Furukawa, Yuji and Canfield, Paul C.},
abstractNote = {Here, we report on self flux growth and characterization of single crystalline AlMn2B2. It is an orthorhombic (space group $Cmmm$), layered material with a platelike morphology. The anisotropic bulk magnetization data, electrical transport, and 11B nuclear magnetic resonance (NMR) data revealed an antiferromagnetic (AFM) transition at 313 ± 2 K . In the magnetization data, there is also a broad local maximum critically above the AFM transition that could be a signature of low-dimensional magnetic interactions in AlMn2B2.},
doi = {10.1103/PhysRevMaterials.3.064415},
journal = {Physical Review Materials},
number = 6,
volume = 3,
place = {United States},
year = {2019},
month = {6}
}

Journal Article:
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    Works referencing / citing this record:

    Monte-Carlo study of correlations in quantum spin chains at non-zero temperature
    journal, August 1998

    • Kim, Y. J.; Greven, M.; Wiese, U. -J.
    • The European Physical Journal B, Vol. 4, Issue 3
    • DOI: 10.1007/s100510050382

    Nuclear magnetic relaxation in weakly ferro-and antiferromagnetic metals
    journal, July 1974


    Anisotropic magnetocaloric response in AlFe2B2
    journal, May 2018


    Magnetic ordering in the nano-laminar ternary Mn2AlB2 using neutron and X-ray diffraction
    journal, February 2019


    Investigation of magnetic properties and electronic structure of layered-structure borides Al T 2 B 2 ( T =Fe, Mn, Cr) and AlFe 2–x Mn x B 2
    journal, April 2015


    Magnetocaloric Effect in AlFe 2 B 2 : Toward Magnetic Refrigerants from Earth-Abundant Elements
    journal, June 2013

    • Tan, Xiaoyan; Chai, Ping; Thompson, Corey M.
    • Journal of the American Chemical Society, Vol. 135, Issue 25
    • DOI: 10.1021/ja404107p

    Origin of the spin reorientation transitions in (Fe1–xCox)2B alloys
    journal, February 2015

    • Belashchenko, Kirill D.; Ke, Liqin; Däne, Markus
    • Applied Physics Letters, Vol. 106, Issue 6
    • DOI: 10.1063/1.4908056

    Discovery of ferromagnetism with large magnetic anisotropy in ZrMnP and HfMnP
    journal, August 2016

    • Lamichhane, Tej N.; Taufour, Valentin; Masters, Morgan W.
    • Applied Physics Letters, Vol. 109, Issue 9
    • DOI: 10.1063/1.4961933

    Anisotropic thermal expansions of select layered ternary transition metal borides: MoAlB, Cr 2 AlB 2 , Mn 2 AlB 2 , and Fe 2 AlB 2
    journal, November 2018

    • Verger, L.; Kota, S.; Roussel, H.
    • Journal of Applied Physics, Vol. 124, Issue 20
    • DOI: 10.1063/1.5054379

    Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples
    journal, December 2015


    X-Ray diffraction on large single crystals using a powder diffractometer
    journal, June 2016


    Relation between the specific heat and susceptibility of an antiferromagnet
    journal, October 1962


    Magnetic frustration and magnetocaloric effect in AlFe 2− x Mn x B 2 ( x = 0–0.5) ribbons
    journal, July 2015