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Title: Thermoreversible Siloxane Networks: Soft Biomaterials with Widely Tunable Viscoelasticity

Authors:
 [1];  [1]; ORCiD logo [2]; ORCiD logo [2]; ORCiD logo [1]
  1. Department of Chemical EngineeringUniversity of Rochester 4311 Wegmans Hall Rochester NY 14627 USA
  2. Department of Biomedical EngineeringUniversity of Rochester 308 Robert B. Goergen Hall Rochester NY 14627 USA
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1542517
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Advanced Functional Materials
Additional Journal Information:
Journal Name: Advanced Functional Materials Journal Volume: 29 Journal Issue: 38; Journal ID: ISSN 1616-301X
Publisher:
Wiley Blackwell (John Wiley & Sons)
Country of Publication:
Germany
Language:
English

Citation Formats

Meng, Yuan, Xu, Weijing, Newman, Maureen R., Benoit, Danielle S. W., and Anthamatten, Mitchell. Thermoreversible Siloxane Networks: Soft Biomaterials with Widely Tunable Viscoelasticity. Germany: N. p., 2019. Web. doi:10.1002/adfm.201903721.
Meng, Yuan, Xu, Weijing, Newman, Maureen R., Benoit, Danielle S. W., & Anthamatten, Mitchell. Thermoreversible Siloxane Networks: Soft Biomaterials with Widely Tunable Viscoelasticity. Germany. doi:10.1002/adfm.201903721.
Meng, Yuan, Xu, Weijing, Newman, Maureen R., Benoit, Danielle S. W., and Anthamatten, Mitchell. Mon . "Thermoreversible Siloxane Networks: Soft Biomaterials with Widely Tunable Viscoelasticity". Germany. doi:10.1002/adfm.201903721.
@article{osti_1542517,
title = {Thermoreversible Siloxane Networks: Soft Biomaterials with Widely Tunable Viscoelasticity},
author = {Meng, Yuan and Xu, Weijing and Newman, Maureen R. and Benoit, Danielle S. W. and Anthamatten, Mitchell},
abstractNote = {},
doi = {10.1002/adfm.201903721},
journal = {Advanced Functional Materials},
number = 38,
volume = 29,
place = {Germany},
year = {2019},
month = {7}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI: 10.1002/adfm.201903721

Citation Metrics:
Cited by: 7 works
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Works referenced in this record:

Attempt toward 1D Cross-Linked Thermoplastic Elastomers:  Structure and Mechanical Properties of a New System
journal, March 2005

  • Colombani, Olivier; Barioz, Chantal; Bouteiller, Laurent
  • Macromolecules, Vol. 38, Issue 5
  • DOI: 10.1021/ma048006m

Highly Conformable, Transparent Electrodes for Epidermal Electronics
journal, June 2018


Segmented organosiloxane copolymers: 2 Thermal and mechanical properties of siloxane—urea copolymers
journal, December 1984


Hydrogels with tunable stress relaxation regulate stem cell fate and activity
journal, November 2015

  • Chaudhuri, Ovijit; Gu, Luo; Klumpers, Darinka
  • Nature Materials, Vol. 15, Issue 3
  • DOI: 10.1038/nmat4489

Unidirectional Dimerization and Stacking of Ureidopyrimidinone End Groups in Polycaprolactone Supramolecular Polymers
journal, November 2007

  • van Beek, D. J. M.; Spiering, A. J. H.; Peters, Gerrit W. M.
  • Macromolecules, Vol. 40, Issue 23
  • DOI: 10.1021/ma0712394

Shape-Memory Effects in Polymer Networks Containing Reversibly Associating Side-Groups
journal, October 2007


Transfer printing by kinetic control of adhesion to an elastomeric stamp
journal, December 2005

  • Meitl, Matthew A.; Zhu, Zheng-Tao; Kumar, Vipan
  • Nature Materials, Vol. 5, Issue 1, p. 33-38
  • DOI: 10.1038/nmat1532

Reversible Polymers Formed from Self-Complementary Monomers Using Quadruple Hydrogen Bonding
journal, November 1997


The Influence of Hydrogen Bonding Side-Groups on Viscoelastic Behavior of Linear and Network Polymers
journal, January 2014

  • Lewis, Christopher L.; Stewart, Kathleen; Anthamatten, Mitchell
  • Macromolecules, Vol. 47, Issue 2
  • DOI: 10.1021/ma402368s

Solvent-free, supersoft and superelastic bottlebrush melts and networks
journal, November 2015

  • Daniel, William F. M.; Burdyńska, Joanna; Vatankhah-Varnoosfaderani, Mohammad
  • Nature Materials, Vol. 15, Issue 2
  • DOI: 10.1038/nmat4508

Competing Fracture in Kinetically Controlled Transfer Printing
journal, December 2007

  • Feng, Xue; Meitl, Matthew A.; Bowen, Audrey M.
  • Langmuir, Vol. 23, Issue 25
  • DOI: 10.1021/la701555n

Stability and Lifetime of Quadruply Hydrogen Bonded 2-Ureido-4[1 H ]-pyrimidinone Dimers
journal, August 2000

  • Söntjens, Serge H. M.; Sijbesma, Rint P.; van Genderen, Marcel H. P.
  • Journal of the American Chemical Society, Vol. 122, Issue 31
  • DOI: 10.1021/ja000435m

A review of shape memory polymers bearing reversible binding groups
journal, February 2016

  • Lewis, Christopher L.; Dell, Elizabeth M.
  • Journal of Polymer Science Part B: Polymer Physics, Vol. 54, Issue 14
  • DOI: 10.1002/polb.23994

Self-Assembly of Ureido-Pyrimidinone Dimers into One-Dimensional Stacks by Lateral Hydrogen Bonding
journal, February 2010

  • Nieuwenhuizen, Marko M. L.; de Greef, Tom F. A.; van der Bruggen, Rob L. J.
  • Chemistry - A European Journal, Vol. 16, Issue 5
  • DOI: 10.1002/chem.200902107

Dynamics of reversibly crosslinked chains
journal, July 1989


Cooperative End-to-End and Lateral Hydrogen-Bonding Motifs in Supramolecular Thermoplastic Elastomers
journal, June 2006

  • Kautz, Holger; van Beek, D. J. M.; Sijbesma, Rint P.
  • Macromolecules, Vol. 39, Issue 13, p. 4265-4267
  • DOI: 10.1021/ma060706z

Materials and Mechanics for Stretchable Electronics
journal, March 2010


PDMS-based microfluidic devices for biomedical applications
journal, July 2002


Harnessing Supramolecular and Peptidic Self-Assembly for the Construction of Reinforced Polymeric Tissue Scaffolds
journal, April 2017


The influence of substrate creep on mesenchymal stem cell behaviour and phenotype
journal, September 2011


Recent developments in PDMS surface modification for microfluidic devices
journal, January 2010

  • Zhou, Jinwen; Ellis, Amanda Vera; Voelcker, Nicolas Hans
  • ELECTROPHORESIS, Vol. 31, Issue 1
  • DOI: 10.1002/elps.200900475

Hierarchical formation of helical supramolecular polymers via stacking of hydrogen-bonded pairs in water
journal, April 2002

  • Brunsveld, L.; Vekemans, J. A. J. M.; Hirschberg, J. H. K. K.
  • Proceedings of the National Academy of Sciences, Vol. 99, Issue 8
  • DOI: 10.1073/pnas.072659099

Self-assembly and morphology of polydimethylsiloxane supramolecular thermoplastic elastomers
journal, June 2008

  • Botterhuis, Nicole E.; van Beek, D. J. M.; van Gemert, Gaby M. L.
  • Journal of Polymer Science Part A: Polymer Chemistry, Vol. 46, Issue 12
  • DOI: 10.1002/pola.22680

Thermoreversible Poly(alkyl acrylates) Consisting of Self-Complementary Multiple Hydrogen Bonding
journal, February 2003

  • Yamauchi, Koji; Lizotte, Jeremy R.; Long, Timothy E.
  • Macromolecules, Vol. 36, Issue 4
  • DOI: 10.1021/ma0212801

Supramolecular Polymers
journal, December 2001

  • Brunsveld, L.; Folmer, B. J. B.; Meijer, E. W.
  • Chemical Reviews, Vol. 101, Issue 12
  • DOI: 10.1021/cr990125q

Soft Poly(dimethylsiloxane) Elastomers from Architecture-Driven Entanglement Free Design
journal, August 2015

  • Cai, Li-Heng; Kodger, Thomas E.; Guerra, Rodrigo E.
  • Advanced Materials, Vol. 27, Issue 35
  • DOI: 10.1002/adma.201502771

Recent progress in soft lithography
journal, February 2005


The effect of time-dependent deformation of viscoelastic hydrogels on myogenic induction and Rac1 activity in mesenchymal stem cells
journal, February 2014


Hydrogel substrate stress-relaxation regulates the spreading and proliferation of mouse myoblasts
journal, October 2017


Substrate stress relaxation regulates cell spreading
journal, February 2015

  • Chaudhuri, Ovijit; Gu, Luo; Darnell, Max
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms7365

Ionomer dynamics and the sticky Rouse model
journal, September 2013

  • Chen, Quan; Tudryn, Gregory J.; Colby, Ralph H.
  • Journal of Rheology, Vol. 57, Issue 5
  • DOI: 10.1122/1.4818868

Thermoplastic elastomers by hydrogen bonding. 3. Interrelations between molecular parameters and rheological properties
journal, October 1987

  • De Lucca Freitas, Liane Lucy; Stadler, Reimund
  • Macromolecules, Vol. 20, Issue 10
  • DOI: 10.1021/ma00176a027

Dynamics of reversible networks
journal, August 1991

  • Leibler, Ludwik; Rubinstein, Michael; Colby, Ralph H.
  • Macromolecules, Vol. 24, Issue 16
  • DOI: 10.1021/ma00016a034