DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Topological superconductor in quasi-one-dimensional Tl 2 - x Mo 6 Se 6

Abstract

Here we propose that the quasi-one-dimensional molybdenum selenide compound Tl2-xMo6Se6 is a time-reversal-invariant topological superconductor induced by intersublattice pairing, even in the absence of spin-orbit coupling (SOC). No noticeable change in superconductivity is observed in Tl-deficient (0 ≤ x ≤ 0.1) compounds. At weak SOC, the superconductor prefers the triplet d vector lying perpendicular to the chain direction and two-dimensional E2u symmetry, which is driven to a nematic order by spontaneous rotation symmetry breaking. The locking energy of the d vector is estimated to be weak and hence the proof of its direction would rely on tunneling or phase-sensitive measurements.

Authors:
 [1];  [2];  [3];  [4];  [2];  [5];  [6]
  1. National Sun Yat-sen University, Kaohsiung (Taiwan)
  2. National University of Singapore (Singapore)
  3. Massachusetts Institute of Technology (MIT), Cambridge, MA (United States)
  4. University of Tokyo (Japan)
  5. National University of Singapore (Singapore); Institute of Physics, Academia Sinica, Nankang Taipei (Taiwan)
  6. Northeastern University, Boston, MA (United States)
Publication Date:
Research Org.:
Northeastern Univ., Boston, MA (United States); Temple Univ., Philadelphia, PA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Ministry of Science and Technology (MoST); Singapore National Research Foundation
OSTI Identifier:
1540755
Alternate Identifier(s):
OSTI ID: 1417074
Grant/Contract Number:  
FG02-07ER46352; SC0012575; AC02-05CH11231; 105- 2112-M-110-014-MY3; NRF-NRFF2013-03
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review. B
Additional Journal Information:
Journal Volume: 97; Journal Issue: 1; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; first-principles calculations; nematic order; phase diagrams; spin-orbit coupling; spin-triplet pairing; superconductivity

Citation Formats

Huang, Shin-Ming, Hsu, Chuang-Han, Xu, Su-Yang, Lee, Chi-Cheng, Shiau, Shiue-Yuan, Lin, Hsin, and Bansil, Arun. Topological superconductor in quasi-one-dimensional Tl2-xMo6Se6. United States: N. p., 2018. Web. doi:10.1103/physrevb.97.014510.
Huang, Shin-Ming, Hsu, Chuang-Han, Xu, Su-Yang, Lee, Chi-Cheng, Shiau, Shiue-Yuan, Lin, Hsin, & Bansil, Arun. Topological superconductor in quasi-one-dimensional Tl2-xMo6Se6. United States. https://doi.org/10.1103/physrevb.97.014510
Huang, Shin-Ming, Hsu, Chuang-Han, Xu, Su-Yang, Lee, Chi-Cheng, Shiau, Shiue-Yuan, Lin, Hsin, and Bansil, Arun. Tue . "Topological superconductor in quasi-one-dimensional Tl2-xMo6Se6". United States. https://doi.org/10.1103/physrevb.97.014510. https://www.osti.gov/servlets/purl/1540755.
@article{osti_1540755,
title = {Topological superconductor in quasi-one-dimensional Tl2-xMo6Se6},
author = {Huang, Shin-Ming and Hsu, Chuang-Han and Xu, Su-Yang and Lee, Chi-Cheng and Shiau, Shiue-Yuan and Lin, Hsin and Bansil, Arun},
abstractNote = {Here we propose that the quasi-one-dimensional molybdenum selenide compound Tl2-xMo6Se6 is a time-reversal-invariant topological superconductor induced by intersublattice pairing, even in the absence of spin-orbit coupling (SOC). No noticeable change in superconductivity is observed in Tl-deficient (0 ≤ x ≤ 0.1) compounds. At weak SOC, the superconductor prefers the triplet d vector lying perpendicular to the chain direction and two-dimensional E2u symmetry, which is driven to a nematic order by spontaneous rotation symmetry breaking. The locking energy of the d vector is estimated to be weak and hence the proof of its direction would rely on tunneling or phase-sensitive measurements.},
doi = {10.1103/physrevb.97.014510},
journal = {Physical Review. B},
number = 1,
volume = 97,
place = {United States},
year = {Tue Jan 16 00:00:00 EST 2018},
month = {Tue Jan 16 00:00:00 EST 2018}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 9 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Majorana Fermions and Topology in Superconductors
journal, July 2016

  • Sato, Masatoshi; Fujimoto, Satoshi
  • Journal of the Physical Society of Japan, Vol. 85, Issue 7
  • DOI: 10.7566/JPSJ.85.072001

Generalized Gradient Approximation Made Simple
journal, October 1996

  • Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
  • Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
  • DOI: 10.1103/PhysRevLett.77.3865

Strong Spin-Orbit Coupling Effects on the Fermi Surface of Sr 2 RuO 4 and Sr 2 RhO 4
journal, July 2008


Majorana fermions on a disordered triangular lattice
journal, October 2011


The Transition Between Real and Complex Superconducting Order Parameter Phases in UPt3
journal, June 2010


Thermodynamic evidence for nematic superconductivity in CuxBi2Se3
journal, October 2016

  • Yonezawa, Shingo; Tajiri, Kengo; Nakata, Suguru
  • Nature Physics, Vol. 13, Issue 2
  • DOI: 10.1038/nphys3907

Even Parity, Orbital Singlet, and Spin Triplet Pairing for Superconducting LaFeAsO 1 x F x
journal, July 2008


Odd-parity superconductivity from phonon-mediated pairing: Application to Cu x Bi 2 Se 3
journal, November 2014


Models of superconducting Cu:Bi 2 Se 3 : Single- versus two-band description
journal, March 2013


Majorana Fermions and a Topological Phase Transition in Semiconductor-Superconductor Heterostructures
journal, August 2010


Non-Abelian Statistics of Half-Quantum Vortices in p -Wave Superconductors
journal, January 2001


Topology of Andreev bound states with flat dispersion
journal, June 2011


Odd-parity topological superconductor with nematic order: Application to Cu x Bi 2 Se 3
journal, September 2014


Odd-Parity Topological Superconductors: Theory and Application to Cu x Bi 2 Se 3
journal, August 2010


Evaluation of Spin-Triplet Superconductivity in Sr 2 RuO 4
journal, January 2012

  • Maeno, Yoshiteru; Kittaka, Shunichiro; Nomura, Takuji
  • Journal of the Physical Society of Japan, Vol. 81, Issue 1
  • DOI: 10.1143/JPSJ.81.011009

Node-surface and node-line fermions from nonsymmorphic lattice symmetries
journal, February 2016


Topological Crystalline Insulators and Topological Superconductors: From Concepts to Materials
journal, March 2015


Types of topological surface states in nodal noncentrosymmetric superconductors
journal, January 2012


Observation of broken time-reversal symmetry in the heavy-fermion superconductor UPt3
journal, July 2014


Helical Liquids and Majorana Bound States in Quantum Wires
journal, October 2010


Superconductivity in quasi-one-dimensional Cs2Cr3As3 with large interchain distance
journal, January 2015


Unconventional superconductivity in quasi-one-dimensional Rb 2 Cr 3 As 3
journal, January 2015


A new pseudo-one-dimensional superconductor: Tℓ2Mo6Se6
journal, February 1980


High Resolution Polar Kerr Effect Measurements of Sr 2 RuO 4 : Evidence for Broken Time-Reversal Symmetry in the Superconducting State
journal, October 2006


The order parameter for the superconducting phases of UPt 3
journal, February 1994


New directions in the pursuit of Majorana fermions in solid state systems
journal, June 2012


The exotic superconductor Tl2Mo6Se6 investigated by low field magnetization measurements
journal, April 1988


NMR Investigation of the Quasi-One-Dimensional Superconductor K 2 Cr 3 As 3
journal, April 2015


Electronic structure of quasi-one-dimensional superconductor K2Cr3As3 from first-principles calculations
journal, November 2015

  • Jiang, Hao; Cao, Guanghan; Cao, Chao
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep16054

Topological odd-parity superconductors
journal, June 2010


p-wave superconductivity
journal, May 2000


Superconductivity without Inversion Symmetry: MnSi versus C e P t 3 S i
journal, March 2004


Evidence for nodal superconductivity in quasi-one-dimensional K 2 Cr 3 As 3
journal, June 2015


Superconducting Proximity Effect and Majorana Fermions at the Surface of a Topological Insulator
journal, March 2008


Predicted Realization of Cubic Dirac Fermion in Quasi-One-Dimensional Transition-Metal Monochalcogenides
journal, May 2017


Odd-Parity Superconductivity in Sr2RuO4
journal, November 2004


A disorder-enhanced quasi-one-dimensional superconductor
journal, July 2016

  • Petrović, A. P.; Ansermet, D.; Chernyshov, D.
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms12262

Superconductivity in Cu x Bi 2 Se 3 and its Implications for Pairing in the Undoped Topological Insulator
journal, February 2010


Phonon mode spectroscopy, electron-phonon coupling, and the metal-insulator transition in quasi-one-dimensional M 2 Mo 6 Se 6
journal, December 2010


Observation of Majorana fermions in ferromagnetic atomic chains on a superconductor
journal, October 2014


Vertical Line Nodes in the Superconducting Gap Structure of Sr 2 RuO 4
journal, March 2017


Majorana Kramers pair in a nematic vortex
journal, June 2017


Theory for superconductivity in alkali chromium arsenides A 2 Cr 3 As 3 (A = K, Rb, Cs)
journal, February 2017


Spin-rotation symmetry breaking in the superconducting state of CuxBi2Se3
journal, May 2016

  • Matano, K.; Kriener, M.; Segawa, K.
  • Nature Physics, Vol. 12, Issue 9
  • DOI: 10.1038/nphys3781

Superconductivity in Quasi-One-Dimensional K 2 Cr 3 As 3 with Significant Electron Correlations
journal, February 2015


Physical properties of several M2Mo6X6 compounds (M = GROUP IA METAL; X = Se, Te)
journal, October 1984