Temperature and voltage measurement in quantum systems far from equilibrium
Abstract
In this work, we show that a local measurement of temperature and voltage for a quantum system in steady state, arbitrarily far from equilibrium, with arbitrary interactions within the system, is unique when it exists. This is interpreted as a consequence of the second law of thermodynamics. We further derive a necessary and sufficient condition for the existence of a solution. In this regard, we find that a positive temperature solution exists whenever there is no net population inversion. However, when there is a net population inversion, we may characterize the system with a unique negative temperature. Voltage and temperature measurements are treated on an equal footing: They are simultaneously measured in a noninvasive manner, via a weakly coupled thermoelectric probe, defined by requiring vanishing charge and heat dissipation into the probe. Our results strongly suggest that a local temperature measurement without a simultaneous local voltage measurement, or vice versa, is a misleading characterization of the state of a nonequilibrium quantum electron system. These results provide a firm mathematical foundation for voltage and temperature measurements far from equilibrium.
- Authors:
-
- Univ. of Arizona, Tucson, AZ (United States)
- Publication Date:
- Research Org.:
- Univ. of Arizona, Tucson, AZ (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1535779
- Alternate Identifier(s):
- OSTI ID: 1329348
- Grant/Contract Number:
- SC0006699
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review B
- Additional Journal Information:
- Journal Volume: 94; Journal Issue: 15; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; nonequilibrium & irreversible thermodynamics; open quantum systems; quantum thermodynamics; quantum transport
Citation Formats
Shastry, Abhay, and Stafford, Charles A. Temperature and voltage measurement in quantum systems far from equilibrium. United States: N. p., 2016.
Web. doi:10.1103/physrevb.94.155433.
Shastry, Abhay, & Stafford, Charles A. Temperature and voltage measurement in quantum systems far from equilibrium. United States. https://doi.org/10.1103/physrevb.94.155433
Shastry, Abhay, and Stafford, Charles A. Wed .
"Temperature and voltage measurement in quantum systems far from equilibrium". United States. https://doi.org/10.1103/physrevb.94.155433. https://www.osti.gov/servlets/purl/1535779.
@article{osti_1535779,
title = {Temperature and voltage measurement in quantum systems far from equilibrium},
author = {Shastry, Abhay and Stafford, Charles A.},
abstractNote = {In this work, we show that a local measurement of temperature and voltage for a quantum system in steady state, arbitrarily far from equilibrium, with arbitrary interactions within the system, is unique when it exists. This is interpreted as a consequence of the second law of thermodynamics. We further derive a necessary and sufficient condition for the existence of a solution. In this regard, we find that a positive temperature solution exists whenever there is no net population inversion. However, when there is a net population inversion, we may characterize the system with a unique negative temperature. Voltage and temperature measurements are treated on an equal footing: They are simultaneously measured in a noninvasive manner, via a weakly coupled thermoelectric probe, defined by requiring vanishing charge and heat dissipation into the probe. Our results strongly suggest that a local temperature measurement without a simultaneous local voltage measurement, or vice versa, is a misleading characterization of the state of a nonequilibrium quantum electron system. These results provide a firm mathematical foundation for voltage and temperature measurements far from equilibrium.},
doi = {10.1103/physrevb.94.155433},
journal = {Physical Review B},
number = 15,
volume = 94,
place = {United States},
year = {Wed Oct 19 00:00:00 EDT 2016},
month = {Wed Oct 19 00:00:00 EDT 2016}
}
Web of Science
Works referenced in this record:
Quantitative Measurement with Scanning Thermal Microscope by Preventing the Distortion Due to the Heat Transfer through the Air
journal, October 2011
- Kim, Kyeongtae; Chung, Jaehun; Hwang, Gwangseok
- ACS Nano, Vol. 5, Issue 11
Scanning thermal profiler
journal, December 1986
- Williams, C. C.; Wickramasinghe, H. K.
- Applied Physics Letters, Vol. 49, Issue 23
Quantum Theory of an Optical Maser. I. General Theory
journal, July 1967
- Scully, Marlan O.; Lamb, Willis E.
- Physical Review, Vol. 159, Issue 2
Electron transport in a one dimensional conductor with inelastic scattering by self-consistent reservoirs
journal, May 2007
- Roy, Dibyendu; Dhar, Abhishek
- Physical Review B, Vol. 75, Issue 19
Quantitative Thermometry of Nanoscale Hot Spots
journal, January 2012
- Menges, Fabian; Riel, Heike; Stemmer, Andreas
- Nano Letters, Vol. 12, Issue 2, p. 596-601
Onset of Energy Dissipation in Ballistic Atomic Wires
journal, May 2002
- Agraït, Nicolás; Untiedt, Carlos; Rubio-Bollinger, Gabino
- Physical Review Letters, Vol. 88, Issue 21
Local and effective temperatures of quantum driven systems
journal, January 2010
- Caso, Alvaro; Arrachea, Liliana; Lozano, Gustavo S.
- Physical Review B, Vol. 81, Issue 4
Semiclassical theory of shot noise in mesoscopic conductors
journal, August 1996
- de Jong, M. J. M.; Beenakker, C. W. J.
- Physica A: Statistical Mechanics and its Applications, Vol. 230, Issue 1-2
High-resolution spatial mapping of the temperature distribution of a Joule self-heated graphene nanoribbon
journal, October 2011
- Yu, Young-Jun; Han, Melinda Y.; Berciaud, Stéphane
- Applied Physics Letters, Vol. 99, Issue 18
Tunneling through a controllable vacuum gap
journal, January 1982
- Binnig, G.; Rohrer, H.; Gerber, Ch.
- Applied Physics Letters, Vol. 40, Issue 2
Energy Gap Induced by Friedel Oscillations Manifested as Transport Asymmetry at Monolayer-Bilayer Graphene Boundaries
journal, February 2014
- Clark, Kendal W.; Zhang, X. -G.; Gu, Gong
- Physical Review X, Vol. 4, Issue 1
Optical Methods of Atomic Orientation and of Magnetic Resonance*
journal, January 1957
- Kastler, Alfred
- Journal of the Optical Society of America, Vol. 47, Issue 6
Small normal-metal loop coupled to an electron reservoir
journal, August 1985
- Büttiker, M.
- Physical Review B, Vol. 32, Issue 3
Four-terminal resistance of a ballistic quantum wire
journal, May 2001
- de Picciotto, R.; Stormer, H. L.; Pfeiffer, L. N.
- Nature, Vol. 411, Issue 6833
Tunable quantum temperature oscillations in graphene nanostructures
journal, March 2015
- Bergfield, Justin P.; Ratner, Mark A.; Stafford, Charles A.
- Physical Review B, Vol. 91, Issue 12
Cold spots in quantum systems far from equilibrium: Local entropies and temperatures near absolute zero
journal, December 2015
- Shastry, Abhay; Stafford, Charles A.
- Physical Review B, Vol. 92, Issue 24
Local Transport Measurements at Mesoscopic Length Scales Using Scanning Tunneling Potentiometry
journal, June 2013
- Wang, Weigang; Munakata, Ko; Rozler, Michael
- Physical Review Letters, Vol. 110, Issue 23
Spatial extent of a Landauer residual-resistivity dipole in graphene quantified by scanning tunnelling potentiometry
journal, March 2015
- Willke, Philip; Druga, Thomas; Ulbrich, Rainer G.
- Nature Communications, Vol. 6, Issue 1
Experimental measurement of scattering coefficients in mesoscopic conductors
journal, October 1992
- Shepard, K. L.; Roukes, M. L.; van der Gaag, B. P.
- Physical Review B, Vol. 46, Issue 15
Vibrational and electronic heating in nanoscale junctions
journal, December 2010
- Ward, Daniel R.; Corley, David A.; Tour, James M.
- Nature Nanotechnology, Vol. 6, Issue 1
Reciprocal Relations in Irreversible Processes. I.
journal, February 1931
- Onsager, Lars
- Physical Review, Vol. 37, Issue 4
The probe technique far from equilibrium: Magnetic field symmetries of nonlinear transport
journal, December 2013
- Bedkihal, Salil; Bandyopadhyay, Malay; Segal, Dvira
- The European Physical Journal B, Vol. 86, Issue 12
Spectral mapping of thermal conductivity through nanoscale ballistic transport
journal, June 2015
- Hu, Yongjie; Zeng, Lingping; Minnich, Austin J.
- Nature Nanotechnology, Vol. 10, Issue 8
Ballistic thermal rectification in asymmetric three-terminal mesoscopic dielectric systems
journal, October 2010
- Ming, Yi; Wang, Zhe Xian; Ding, Ze Jun
- New Journal of Physics, Vol. 12, Issue 10
Temperature in non-equilibrium states: a review of open problems and current proposals
journal, October 2003
- Casas-Vázquez, J.; Jou, D.
- Reports on Progress in Physics, Vol. 66, Issue 11
Quantum heat transfer in harmonic chains with self-consistent reservoirs: Exact numerical simulations
journal, July 2011
- Bandyopadhyay, Malay; Segal, Dvira
- Physical Review E, Vol. 84, Issue 1
ThermoElectric Transport Properties of a Chain of Quantum Dots with Self-Consistent Reservoirs
journal, February 2009
- Jacquet, Philippe A.
- Journal of Statistical Physics, Vol. 134, Issue 4
Local temperature of out-of-equilibrium quantum electron systems
journal, July 2014
- Meair, J.; Bergfield, J. P.; Stafford, C. A.
- Physical Review B, Vol. 90, Issue 3
Four-Point Resistance of Individual Single-Wall Carbon Nanotubes
journal, October 2005
- Gao, B.; Chen, Y. F.; Fuhrer, M. S.
- Physical Review Letters, Vol. 95, Issue 19
Thermopower with broken time-reversal symmetry
journal, November 2011
- Saito, Keiji; Benenti, Giuliano; Casati, Giulio
- Physical Review B, Vol. 84, Issue 20
Local temperature of an interacting quantum system far from equilibrium
journal, June 2016
- Stafford, Charles A.
- Physical Review B, Vol. 93, Issue 24
Scanning tunneling microscopy
journal, March 1983
- Binnig, G.; Rohrer, H.
- Surface Science, Vol. 126, Issue 1-3
Local potentiometry using a multiprobe scanning tunneling microscope
journal, August 2008
- Bannani, A.; Bobisch, C. A.; Möller, R.
- Review of Scientific Instruments, Vol. 79, Issue 8
Thermoelectric transport of mesoscopic conductors coupled to voltage and thermal probes
journal, November 2011
- Sánchez, David; Serra, Llorenç
- Physical Review B, Vol. 84, Issue 20
Many-body theory of electronic transport in single-molecule heterojunctions
journal, June 2009
- Bergfield, J. P.; Stafford, C. A.
- Physical Review B, Vol. 79, Issue 24
Definition and measurement of the electrical and thermal resistances
journal, July 1981
- Engquist, H. - L.; Anderson, P. W.
- Physical Review B, Vol. 24, Issue 2
Voltage and dephasing probes in mesoscopic conductors: A study of full-counting statistics
journal, January 2007
- Förster, Heidi; Samuelsson, Peter; Pilgram, Sebastian
- Physical Review B, Vol. 75, Issue 3
Asymmetry in the Magnetoconductance of Metal Wires and Loops
journal, October 1986
- Benoit, A. D.; Washburn, S.; Umbach, C. P.
- Physical Review Letters, Vol. 57, Issue 14
Nonequilibrium Many-Body Theory of Quantum Systems
book, March 2013
- Stefanucci, Gianluca; van Leeuwen, Robert
Scanning tunneling potentiometry
journal, February 1986
- Muralt, P.; Pohl, D. W.
- Applied Physics Letters, Vol. 48, Issue 8
Thermoelectric corrections to quantum voltage measurement
journal, December 2014
- Bergfield, Justin P.; Stafford, Charles A.
- Physical Review B, Vol. 90, Issue 23
Local temperatures and heat flow in quantum driven systems
journal, April 2011
- Caso, Alvaro; Arrachea, Liliana; Lozano, Gustavo S.
- Physical Review B, Vol. 83, Issue 16
Role of quantum coherence in series resistors
journal, March 1986
- Büttiker, M.
- Physical Review B, Vol. 33, Issue 5
Interfacial Charge States in Graphene on SiC Studied by Noncontact Scanning Nonlinear Dielectric Potentiometry
journal, June 2015
- Yamasue, Kohei; Fukidome, Hirokazu; Funakubo, Kazutoshi
- Physical Review Letters, Vol. 114, Issue 22
Scanning Probe Microscopy
book, January 2007
- Kalinin, Sergei; Gruverman, Alexei
- Springer New York, NY
Heat conduction in molecular transport junctions
journal, April 2007
- Galperin, Michael; Nitzan, Abraham; Ratner, Mark A.
- Physical Review B, Vol. 75, Issue 15
Ultra-High Vacuum Scanning Thermal Microscopy for Nanometer Resolution Quantitative Thermometry
journal, May 2012
- Kim, Kyeongtae; Jeong, Wonho; Lee, Woochul
- ACS Nano, Vol. 6, Issue 5, p. 4248-4257
Thermoelectric Signatures of Coherent Transport in Single-Molecule Heterojunctions
journal, August 2009
- Bergfield, J. P.; Stafford, C. A.
- Nano Letters, Vol. 9, Issue 8
Chemical potential oscillations near a barrier in the presence of transport
journal, August 1989
- Büttiker, M.
- Physical Review B, Vol. 40, Issue 5
Ueber eine veränderte Form des zweiten Hauptsatzes der mechanischen Wärmetheorie
journal, January 1854
- Clausius, R.
- Annalen der Physik und Chemie, Vol. 169, Issue 12
Infrared and Optical Masers
journal, December 1958
- Schawlow, A. L.; Townes, C. H.
- Physical Review, Vol. 112, Issue 6
Heat dissipation in atomic-scale junctions
journal, June 2013
- Lee, Woochul; Kim, Kyeongtae; Jeong, Wonho
- Nature, Vol. 498, Issue 7453
Thermoelectric Effects in Nanoscale Junctions
journal, January 2009
- Dubi, Yonatan; Di Ventra, Massimiliano
- Nano Letters, Vol. 9, Issue 1
Conductance of a disordered linear chain including inelastic scattering events
journal, April 1990
- D’Amato, Jorge L.; Pastawski, Horacio M.
- Physical Review B, Vol. 41, Issue 11
Quantum-statistical current correlations in multilead chaotic cavities
journal, July 1997
- van Langen, S. A.; Büttiker, M.
- Physical Review B, Vol. 56, Issue 4
Probing Maxwell’s Demon with a Nanoscale Thermometer
journal, May 2013
- Bergfield, Justin P.; Story, Shauna M.; Stafford, Robert C.
- ACS Nano, Vol. 7, Issue 5
Fourier’s law: Insight from a simple derivation
journal, April 2009
- Dubi, Y.; Di Ventra, M.
- Physical Review E, Vol. 79, Issue 4
Anisotropy in Conductance of a Quasi-One-Dimensional Metallic Surface State Measured by a Square Micro-Four-Point Probe Method
journal, July 2003
- Kanagawa, Taizo; Hobara, Rei; Matsuda, Iwao
- Physical Review Letters, Vol. 91, Issue 3
Radiative heat transfer in the extreme near field
journal, December 2015
- Kim, Kyeongtae; Song, Bai; Fernández-Hurtado, Víctor
- Nature, Vol. 528, Issue 7582
Atomic Force Microscope
journal, March 1986
- Binnig, G.; Quate, C. F.; Gerber, Ch.
- Physical Review Letters, Vol. 56, Issue 9
Multichannel Landauer formula for thermoelectric transport with application to thermopower near the mobility edge
journal, January 1986
- Sivan, U.; Imry, Y.
- Physical Review B, Vol. 33, Issue 1
Voltage distribution and phase-breaking scattering in the quantum Hall regime
journal, July 1996
- Ando, Tsuneya
- Surface Science, Vol. 361-362
Efficiency of three-terminal thermoelectric transport under broken time-reversal symmetry
journal, April 2013
- Balachandran, Vinitha; Benenti, Giuliano; Casati, Giulio
- Physical Review B, Vol. 87, Issue 16
Understanding Non-equilibrium Thermodynamics
book, January 2008
- Lebon, G.; Jou, D.; Casas-Vázquez, J.
Quantum Thermodynamics: A Nonequilibrium Green’s Function Approach
journal, February 2015
- Esposito, Massimiliano; Ochoa, Maicol A.; Galperin, Michael
- Physical Review Letters, Vol. 114, Issue 8
Scanning Thermal Microscopy
journal, August 1999
- Majumdar, A.
- Annual Review of Materials Science, Vol. 29, Issue 1
Landauer formula for the current through an interacting electron region
journal, April 1992
- Meir, Yigal; Wingreen, Ned S.
- Physical Review Letters, Vol. 68, Issue 16
Coherent and sequential tunneling in series barriers
journal, January 1988
- Buttiker, M.
- IBM Journal of Research and Development, Vol. 32, Issue 1
Magnetic field symmetries of nonlinear transport with elastic and inelastic scattering
journal, October 2013
- Bedkihal, Salil; Bandyopadhyay, Malay; Segal, Dvira
- Physical Review B, Vol. 88, Issue 15
Strong Bounds on Onsager Coefficients and Efficiency for Three-Terminal Thermoelectric Transport in a Magnetic Field
journal, February 2013
- Brandner, Kay; Saito, Keiji; Seifert, Udo
- Physical Review Letters, Vol. 110, Issue 7
Temperature and voltage probes far from equilibrium
journal, March 2012
- Jacquet, Ph. A.; Pillet, C. -A.
- Physical Review B, Vol. 85, Issue 12
The effective temperature
journal, November 2011
- Cugliandolo, Leticia F.
- Journal of Physics A: Mathematical and Theoretical, Vol. 44, Issue 48
Giant Thermoelectric Effect from Transmission Supernodes
journal, August 2010
- Bergfield, Justin P.; Solis, Michelle A.; Stafford, Charles A.
- ACS Nano, Vol. 4, Issue 9
Atomic Force Microscope. [原子間力顕微鏡]
journal, January 1991
- Tsuda, Nobuhiro
- Journal of the Japan Society for Precision Engineering, Vol. 57, Issue 7
Scanning tunneling microscopy
journal, April 1985
- Binnig, G.; Rohrer, H.
- Surface Science Letters, Vol. 152-153
Scanning Probe Microscopy
journal, January 2008
- Morita, Seizo
- Journal of the Vacuum Society of Japan, Vol. 51, Issue 12
Scanning tunneling microscopy
journal, January 2000
- Binnig, G.; Rohrer, H.
- IBM Journal of Research and Development, Vol. 44, Issue 1.2
ThermoElectric Transport Properties of a Chain of Quantum Dots with Self-Consistent Reservoirs
text, January 2008
- Jacquet, Philippe A.
- arXiv
Ballistic Thermal Rectification in Asymmetric Three-Terminal Mesoscopic Dielectric Systems
text, January 2009
- Ming, Yi; Wang, Zhe Xian; Ding, Ze Jun
- arXiv
Giant Thermoelectric Effect from Transmission Supernodes
text, January 2010
- Bergfield, J. P.; Solis, M.; Stafford, C. A.
- arXiv
Quantum heat transfer in harmonic chains with self consistent reservoirs: Exact numerical simulations
text, January 2011
- Bandyopadhyay, Malay; Segal, Dvira
- arXiv
Temperature and Voltage Probes Far from Equilibrium
text, January 2011
- Jacquet, Ph. A.; Pillet, C. -A.
- arXiv
Strong bounds on Onsager coefficients and efficiency for three terminal thermoelectric transport in a magnetic field
text, January 2013
- Brandner, Kay; Saito, Keiji; Seifert, Udo
- arXiv
Cold spots in quantum systems far from equilibrium: local entropies and temperatures near absolute zero
text, January 2015
- Shastry, Abhay; Stafford, Charles A.
- arXiv
Four-point resistance of individual single-wall carbon nanotubes
text, January 2005
- Gao, B.; Chen, Y. F.; Fuhrer, M. S.
- arXiv
Heat conduction in molecular transport junctions
text, January 2006
- Galperin, Michael; Ratner, Mark A.; Nitzan, Abraham
- arXiv
Semiclassical theory of shot noise in mesoscopic conductors
text, January 1996
- de Jong, M. J. M.; Beenakker, C. W. J.
- arXiv
Works referencing / citing this record:
The third law of thermodynamics in open quantum systems
journal, August 2019
- Shastry, Abhay; Xu, Yiheng; Stafford, Charles A.
- The Journal of Chemical Physics, Vol. 151, Issue 6
Thermionic cooling devices based on resonant-tunneling AlGaAs/GaAs heterostructure
journal, January 2018
- Bescond, M.; Logoteta, D.; Michelini, F.
- Journal of Physics: Condensed Matter, Vol. 30, Issue 6
Quantum thermodynamics of nanoscale steady states far from equilibrium
journal, April 2018
- Taniguchi, Nobuhiko
- Physical Review B, Vol. 97, Issue 15
Quantum thermodynamics of nanoscale steady states far from equilibrium
text, January 2017
- Taniguchi, Nobuhiko
- arXiv