The ultrafast X-ray spectroscopic revolution in chemical dynamics
Abstract
There have been rapid developments in short-pulse X-ray sources in the past two decades, which have enabled the study of nuclear and electronic dynamics by ultrafast X-ray spectroscopies with unprecedented time resolution ranging from nanoseconds to attoseconds. In this Perspective, we discuss some of the major achievements in the study of nuclear and electronic dynamics with X-ray pulses produced by high-harmonic, free-electron-laser and synchrotron sources. The particular dynamic processes probed by X-ray radiation highlighted in this Perspective are electronic coherences on attosecond to femtosecond timescales, chemical reactions, such as dissociations, and pericyclic ring-openings, spin-crossover dynamics, ligand-exchange dynamics and structural deformations in excited states. X-ray spectroscopic probing of chemical dynamics holds promising use for the future owing to the ongoing developments of new spectroscopies, such as four-wave mixing, and the continuous improvements in emerging laboratory-based, high-harmonic sources and large-scale, facility-based, free-electron lasers.
- Authors:
-
[3];
[3]
- Univ. of California, Berkeley, CA (United States); Advanced Research Center for Nanolithography, Amsterdam (Netherlands)
- Univ. of California, Berkeley, CA (United States)
- Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office; National Science Foundation (NSF); US Air Force Office of Scientific Research (AFOSR); Army Research Office (ARO); Swiss National Science Foundation (SNSF)
- OSTI Identifier:
- 1532322
- Grant/Contract Number:
- AC02-05CH11231; FA9550-15-1-0037; FA9550-14-1-0154; CHE-1361226; CHE-1660417
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Reviews Chemistry
- Additional Journal Information:
- Journal Volume: 2; Journal Issue: 6; Journal ID: ISSN 2397-3358
- Publisher:
- Springer Nature
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Kraus, Peter M., Zürch, Michael, Cushing, Scott K., Neumark, Daniel M., and Leone, Stephen R. The ultrafast X-ray spectroscopic revolution in chemical dynamics. United States: N. p., 2018.
Web. doi:10.1038/s41570-018-0008-8.
Kraus, Peter M., Zürch, Michael, Cushing, Scott K., Neumark, Daniel M., & Leone, Stephen R. The ultrafast X-ray spectroscopic revolution in chemical dynamics. United States. https://doi.org/10.1038/s41570-018-0008-8
Kraus, Peter M., Zürch, Michael, Cushing, Scott K., Neumark, Daniel M., and Leone, Stephen R. Tue .
"The ultrafast X-ray spectroscopic revolution in chemical dynamics". United States. https://doi.org/10.1038/s41570-018-0008-8. https://www.osti.gov/servlets/purl/1532322.
@article{osti_1532322,
title = {The ultrafast X-ray spectroscopic revolution in chemical dynamics},
author = {Kraus, Peter M. and Zürch, Michael and Cushing, Scott K. and Neumark, Daniel M. and Leone, Stephen R.},
abstractNote = {There have been rapid developments in short-pulse X-ray sources in the past two decades, which have enabled the study of nuclear and electronic dynamics by ultrafast X-ray spectroscopies with unprecedented time resolution ranging from nanoseconds to attoseconds. In this Perspective, we discuss some of the major achievements in the study of nuclear and electronic dynamics with X-ray pulses produced by high-harmonic, free-electron-laser and synchrotron sources. The particular dynamic processes probed by X-ray radiation highlighted in this Perspective are electronic coherences on attosecond to femtosecond timescales, chemical reactions, such as dissociations, and pericyclic ring-openings, spin-crossover dynamics, ligand-exchange dynamics and structural deformations in excited states. X-ray spectroscopic probing of chemical dynamics holds promising use for the future owing to the ongoing developments of new spectroscopies, such as four-wave mixing, and the continuous improvements in emerging laboratory-based, high-harmonic sources and large-scale, facility-based, free-electron lasers.},
doi = {10.1038/s41570-018-0008-8},
journal = {Nature Reviews Chemistry},
number = 6,
volume = 2,
place = {United States},
year = {Tue May 29 00:00:00 EDT 2018},
month = {Tue May 29 00:00:00 EDT 2018}
}
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