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Title: Facet-selective adsorption of Fe( ii ) on hematite visualized by nanoscale secondary ion mass spectrometry

Abstract

Novel isotopic labelling and imaging techniques are used to directly observe the autocatalytic reaction and facet-selective adsorption of Fe( ii ) onto individual hematite (Fe 2 O 3 ) crystallites.

Authors:
ORCiD logo [1]; ORCiD logo [2]; ORCiD logo [2]; ORCiD logo [1]
  1. Physical Sciences Division, Pacific Northwest National Laboratory, Richland, USA
  2. Earth and Biological Sciences Directorate, Pacific Northwest National Laboratory, Richland, USA
Publication Date:
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1531183
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Environmental Science: Nano
Additional Journal Information:
Journal Name: Environmental Science: Nano Journal Volume: 6 Journal Issue: 8; Journal ID: ISSN 2051-8153
Publisher:
Royal Society of Chemistry (RSC)
Country of Publication:
United Kingdom
Language:
English

Citation Formats

Taylor, Sandra D., Kovarik, Libor, Cliff, John B., and Rosso, Kevin M. Facet-selective adsorption of Fe( ii ) on hematite visualized by nanoscale secondary ion mass spectrometry. United Kingdom: N. p., 2019. Web. doi:10.1039/C9EN00562E.
Taylor, Sandra D., Kovarik, Libor, Cliff, John B., & Rosso, Kevin M. Facet-selective adsorption of Fe( ii ) on hematite visualized by nanoscale secondary ion mass spectrometry. United Kingdom. doi:10.1039/C9EN00562E.
Taylor, Sandra D., Kovarik, Libor, Cliff, John B., and Rosso, Kevin M. Thu . "Facet-selective adsorption of Fe( ii ) on hematite visualized by nanoscale secondary ion mass spectrometry". United Kingdom. doi:10.1039/C9EN00562E.
@article{osti_1531183,
title = {Facet-selective adsorption of Fe( ii ) on hematite visualized by nanoscale secondary ion mass spectrometry},
author = {Taylor, Sandra D. and Kovarik, Libor and Cliff, John B. and Rosso, Kevin M.},
abstractNote = {Novel isotopic labelling and imaging techniques are used to directly observe the autocatalytic reaction and facet-selective adsorption of Fe( ii ) onto individual hematite (Fe 2 O 3 ) crystallites.},
doi = {10.1039/C9EN00562E},
journal = {Environmental Science: Nano},
number = 8,
volume = 6,
place = {United Kingdom},
year = {2019},
month = {8}
}

Journal Article:
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Works referenced in this record:

An ab initio model of electron transport in hematite (╬▒-Fe2O3) basal planes
journal, April 2003

  • Rosso, Kevin M.; Smith, Dayle M. A.; Dupuis, Michel
  • The Journal of Chemical Physics, Vol. 118, Issue 14, p. 6455-6466
  • DOI: 10.1063/1.1558534