Distinct evolution of the carbonaceous and non-carbonaceous reservoirs: Insights from Ru, Mo, and W isotopes

Worsham, Emily A.; Burkhardt, Christoph; Budde, Gerrit; Fischer-Gödde, Mario; Kruijer, Thomas S.; Kleine, Thorsten

doi:10.1016/j.epsl.2019.06.001

Title: Distinct evolution of the carbonaceous and non-carbonaceous reservoirs: Insights from Ru, Mo, and W isotopes

Journal Article · 20 June 2019 · Earth and Planetary Science Letters

DOI: https://doi.org/10.1016/j.epsl.2019.06.001 · OSTI ID:1529822

^[1]; Burkhardt, Christoph ^[1];

^[1]; Fischer-Gödde, Mario ^[2];

^[3]; Kleine, Thorsten ^[1]

Univ. of Münster, Münster (Germany). Inst. für Planetologie
Univ. of Münster, Münster (Germany). Inst. für Planetologie; Univ. of Köln, Köln (Germany). Inst. für Geologie und Mineralogie
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

Recent work has identified a nucleosynthetic isotope dichotomy between “carbonaceous” (CC) and “non-carbonaceous” (NC) meteorites. Here in this paper, we report new Ru isotope data for rare iron meteorite groups belonging to the NC and CC suites. We show that by studying the relative isotopic characteristics of Ru, Mo, and W in iron meteorites, it is possible to constrain the processes leading to the distinct isotope heterogeneities in both reservoirs. In NC meteorites, internally normalized, mass-independent isotope ratios of Mo and Ru are correlated, but those of Mo and W are not. In CC meteorites, Mo and W isotope ratios are correlated, but those of Mo and Ru are not; specifically, Mo isotopic compositions are variable and those of Ru are more restricted. The contrasting behaviors of Ru and W relative to Mo in the two reservoirs likely require processing of the presolar carriers under distinct redox conditions. This provides further evidence that NC and CC meteorites originated from spatially separated reservoirs that evolved under different prevailing conditions.

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Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC52-07NA27344

OSTI ID:: 1529822

Report Number(s):: LLNL-JRNL-755889; 943143

Journal Information:: Earth and Planetary Science Letters, Vol. 521, Issue C; ISSN 0012-821X

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Data for: Distinct evolution of the carbonaceous and non-carbonaceous reservoirs: Insights from Ru, Mo, and W isotopes Worsham, Emily https://doi.org/10.17632/tbgwzjjsfy.1 The current record is supplemented by this dataset	dataset	January 2020
Data for: Distinct evolution of the carbonaceous and non-carbonaceous reservoirs: Insights from Ru, Mo, and W isotopes Worsham, Emily https://doi.org/10.17632/tbgwzjjsfy The current record is supplemented by this dataset	dataset	January 2020