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Title: Designing polymers for advanced battery chemistries

Abstract

Electrochemical energy storage devices are becoming increasingly important to our global society, and polymer materials are key components of these devices. As the demand for high-energy density devices increases, innovative new materials that build on the fundamental understanding of physical phenomena and structure–property relationships will be required to enable high-capacity next-generation battery chemistries. In this Review, we discuss core polymer science principles that are used to facilitate progress in battery materials development. Specifically, we discuss the design of polymeric materials for desired mechanical properties, increased ionic and electronic conductivity and specific chemical interactions. We also discuss how polymer materials have been designed to create stable artificial interfaces and improve battery safety. Furthermore, the focus is on these design principles applied to advanced silicon, lithium-metal and sulfur battery chemistries.

Authors:
ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [2]; ORCiD logo [1]
  1. Stanford Univ., Stanford, CA (United States)
  2. Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)
Publication Date:
Research Org.:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1528897
Grant/Contract Number:  
AC02-76SF00515
Resource Type:
Accepted Manuscript
Journal Name:
Nature Reviews. Materials
Additional Journal Information:
Journal Volume: 4; Journal Issue: 5; Journal ID: ISSN 2058-8437
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
25 ENERGY STORAGE; 36 MATERIALS SCIENCE

Citation Formats

Lopez, Jeffrey, Mackanic, David G., Cui, Yi, and Bao, Zhenan. Designing polymers for advanced battery chemistries. United States: N. p., 2019. Web. doi:10.1038/s41578-019-0103-6.
Lopez, Jeffrey, Mackanic, David G., Cui, Yi, & Bao, Zhenan. Designing polymers for advanced battery chemistries. United States. doi:10.1038/s41578-019-0103-6.
Lopez, Jeffrey, Mackanic, David G., Cui, Yi, and Bao, Zhenan. Wed . "Designing polymers for advanced battery chemistries". United States. doi:10.1038/s41578-019-0103-6.
@article{osti_1528897,
title = {Designing polymers for advanced battery chemistries},
author = {Lopez, Jeffrey and Mackanic, David G. and Cui, Yi and Bao, Zhenan},
abstractNote = {Electrochemical energy storage devices are becoming increasingly important to our global society, and polymer materials are key components of these devices. As the demand for high-energy density devices increases, innovative new materials that build on the fundamental understanding of physical phenomena and structure–property relationships will be required to enable high-capacity next-generation battery chemistries. In this Review, we discuss core polymer science principles that are used to facilitate progress in battery materials development. Specifically, we discuss the design of polymeric materials for desired mechanical properties, increased ionic and electronic conductivity and specific chemical interactions. We also discuss how polymer materials have been designed to create stable artificial interfaces and improve battery safety. Furthermore, the focus is on these design principles applied to advanced silicon, lithium-metal and sulfur battery chemistries.},
doi = {10.1038/s41578-019-0103-6},
journal = {Nature Reviews. Materials},
number = 5,
volume = 4,
place = {United States},
year = {2019},
month = {4}
}

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