Tuning the Luminescence of Layered Halide Perovskites

Smith, Matthew D.; Connor, Bridget A.; Karunadasa, Hemamala I.

doi:10.1021/acs.chemrev.8b00477

Title: Tuning the Luminescence of Layered Halide Perovskites

Journal Article · 28 January 2019 · Chemical Reviews

DOI: https://doi.org/10.1021/acs.chemrev.8b00477 · OSTI ID:1528780

^[1]; Connor, Bridget A. ^[1];

^[1]

Stanford Univ., CA (United States). Dept. of Chemistry

Layered halide perovskites offer a versatile platform for manipulating light through synthetic design. Although most layered perovskites absorb strongly in the ultraviolet (UV) or near-UV region, their emission can range from the UV to the infrared region of the electromagnetic spectrum. This emission can be very narrow, displaying high color purity, or it can be extremely broad, spanning the entire visible spectrum and providing high color rendition (or accurately reproducing illuminated colors). The origin of the photoluminescence can vary enormously. Strongly correlated electron–hole pairs, permanent lattice defects, transient light-induced defects, and ligand-field transitions in the inorganic layers and molecular chromophores in the organic layers can be involved in the emission mechanism. Here in this review, we highlight the different types of photoluminescence that may be attained from layered halide perovskites, with an emphasis on how the emission may be systematically tuned through changes to the bulk crystalline lattice: changes in composition, structure, and dimensionality.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE; Alfred P. Sloan; National Science Foundation (NSF)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1528780

Journal Information:: Chemical Reviews, Vol. 119, Issue 5; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 488 works

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