Multidimensional photon correlation spectroscopy of cavity polaritons
Abstract
Significance We propose a spectroscopic technique that can track the time-dependent state of a dressed molecule in an optical cavity (polariton) by measuring coincidence of two emitted photons. The proposed technique offers an independent control of the spectral and temporal resolution; single-photon detection allows for low-intensity measurements, which do not disturb the state of the cavity field, and time-dependent atom/cavity coupling provides a control tool. Tracking the evolution of the polariton states with time-dependent atom/cavity coupling should be of interest in photochemistry and photobiology and could improve fundamental understanding of many physical processes in strongly coupled atom/radiation states. Possible applications include chemical sensors and quantum information processing.
- Authors:
-
[2]
- State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, China,
- Department of Chemistry, University of California, Irvine, CA 92697,, Department of Physics and Astronomy, University of California, Irvine, CA 92697
- Publication Date:
- Research Org.:
- Univ. of California, Irvine, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences, and Biosciences Division; National Science Foundation (NSF)
- OSTI Identifier:
- 1418899
- Alternate Identifier(s):
- OSTI ID: 1527163
- Grant/Contract Number:
- FG02-04ER15571; CHE-1663822
- Resource Type:
- Published Article
- Journal Name:
- Proceedings of the National Academy of Sciences of the United States of America
- Additional Journal Information:
- Journal Name: Proceedings of the National Academy of Sciences of the United States of America Journal Volume: 115 Journal Issue: 7; Journal ID: ISSN 0027-8424
- Publisher:
- Proceedings of the National Academy of Sciences
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 74 ATOMIC AND MOLECULAR PHYSICS; multidimensional spectroscopy; photon correlation; cavity polaritons
Citation Formats
Dorfman, Konstantin E., and Mukamel, Shaul. Multidimensional photon correlation spectroscopy of cavity polaritons. United States: N. p., 2018.
Web. doi:10.1073/pnas.1719443115.
Dorfman, Konstantin E., & Mukamel, Shaul. Multidimensional photon correlation spectroscopy of cavity polaritons. United States. https://doi.org/10.1073/pnas.1719443115
Dorfman, Konstantin E., and Mukamel, Shaul. Wed .
"Multidimensional photon correlation spectroscopy of cavity polaritons". United States. https://doi.org/10.1073/pnas.1719443115.
@article{osti_1418899,
title = {Multidimensional photon correlation spectroscopy of cavity polaritons},
author = {Dorfman, Konstantin E. and Mukamel, Shaul},
abstractNote = {Significance We propose a spectroscopic technique that can track the time-dependent state of a dressed molecule in an optical cavity (polariton) by measuring coincidence of two emitted photons. The proposed technique offers an independent control of the spectral and temporal resolution; single-photon detection allows for low-intensity measurements, which do not disturb the state of the cavity field, and time-dependent atom/cavity coupling provides a control tool. Tracking the evolution of the polariton states with time-dependent atom/cavity coupling should be of interest in photochemistry and photobiology and could improve fundamental understanding of many physical processes in strongly coupled atom/radiation states. Possible applications include chemical sensors and quantum information processing.},
doi = {10.1073/pnas.1719443115},
journal = {Proceedings of the National Academy of Sciences of the United States of America},
number = 7,
volume = 115,
place = {United States},
year = {Wed Jan 31 00:00:00 EST 2018},
month = {Wed Jan 31 00:00:00 EST 2018}
}
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https://doi.org/10.1073/pnas.1719443115
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Cited by: 22 works
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Figures / Tables:
Fig. 1: (Top) Atom in the cavity emitting photons into the longitudinal cavity mode as well as noncavity vertical modes. Two TF-resolved detectors outside of the cavity register noncavity modes photon coincidence events. One photon number-resolving detector on the main optical axis measures photon number of the cavity mode photons.more »
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