Ultrafine Pt Nanoparticle-Decorated Pyrite-Type CoS 2 Nanosheet Arrays Coated on Carbon Cloth as a Bifunctional Electrode for Overall Water Splitting
Abstract
To improve the utilization efficiency of precious metals, metal-supported materials provide a direction for fabricating highly active and stable heterogeneous catalysts. Here, carbon cloth (CC)-supported Earth-abundant CoS2 nanosheet arrays (CoS2/CC) are presented as ideal substrates for ultrafine Pt deposition (Pt-CoS2/CC) to achieve remarkable performance toward the hydrogen and oxygen evolution reactions (HER/OER) in alkaline solutions. Notably, the Pt-CoS2/CC hybrid delivers an overpotential of 24 mV at 10 mA cm–2 and a mass activity of 3.89 A Ptmg–1, which is 4.7 times higher than that of commercial Pt/C, at an overpotential of 130 mV for catalyzing the HER. An alkali-electrolyzer using Pt-CoS2/CC as a bifunctional electrode enables a water-splitting current density of 10 mA cm–2 at a low voltage of 1.55 V and can sustain for more than 20 h, which is superior to that of the state-of-the-art Pt/C+RuO2 catalyst. Further experimental and theoretical simulation studies demonstrate that strong electronic interaction between Pt and CoS2 synergistically optimize hydrogen adsorption/desorption behaviors and facilitate the in situ generation of OER active species, enhancing the overall water-splitting performance. This research highlights the regulation of interfacial and electronic synergy in pursuit of highly efficient and durable supported catalysts for hydrogen and oxygen electrocatalytic applications.
- Authors:
-
[1];
- Tianjin Univ. (China)
- Shandong Univ., Jinan (China)
- Argonne National Lab. (ANL), Lemont, IL (United States)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- National Natural Science Foundation of China (NSFC); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V)
- OSTI Identifier:
- 1526674
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Energy Materials
- Additional Journal Information:
- Journal Volume: 8; Journal Issue: 24; Journal ID: ISSN 1614-6832
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; active sites; nanocomposite; Pt nanoparticles; pyrite CoS2; water splitting
Citation Formats
Han, Xiaopeng, Wu, Xiaoyu, Deng, Yida, Liu, Jian, Lu, Jun, Zhong, Cheng, and Hu, Wenbin. Ultrafine Pt Nanoparticle-Decorated Pyrite-Type CoS 2 Nanosheet Arrays Coated on Carbon Cloth as a Bifunctional Electrode for Overall Water Splitting. United States: N. p., 2018.
Web. doi:10.1002/aenm.201800935.
Han, Xiaopeng, Wu, Xiaoyu, Deng, Yida, Liu, Jian, Lu, Jun, Zhong, Cheng, & Hu, Wenbin. Ultrafine Pt Nanoparticle-Decorated Pyrite-Type CoS 2 Nanosheet Arrays Coated on Carbon Cloth as a Bifunctional Electrode for Overall Water Splitting. United States. https://doi.org/10.1002/aenm.201800935
Han, Xiaopeng, Wu, Xiaoyu, Deng, Yida, Liu, Jian, Lu, Jun, Zhong, Cheng, and Hu, Wenbin. Mon .
"Ultrafine Pt Nanoparticle-Decorated Pyrite-Type CoS 2 Nanosheet Arrays Coated on Carbon Cloth as a Bifunctional Electrode for Overall Water Splitting". United States. https://doi.org/10.1002/aenm.201800935. https://www.osti.gov/servlets/purl/1526674.
@article{osti_1526674,
title = {Ultrafine Pt Nanoparticle-Decorated Pyrite-Type CoS 2 Nanosheet Arrays Coated on Carbon Cloth as a Bifunctional Electrode for Overall Water Splitting},
author = {Han, Xiaopeng and Wu, Xiaoyu and Deng, Yida and Liu, Jian and Lu, Jun and Zhong, Cheng and Hu, Wenbin},
abstractNote = {To improve the utilization efficiency of precious metals, metal-supported materials provide a direction for fabricating highly active and stable heterogeneous catalysts. Here, carbon cloth (CC)-supported Earth-abundant CoS2 nanosheet arrays (CoS2/CC) are presented as ideal substrates for ultrafine Pt deposition (Pt-CoS2/CC) to achieve remarkable performance toward the hydrogen and oxygen evolution reactions (HER/OER) in alkaline solutions. Notably, the Pt-CoS2/CC hybrid delivers an overpotential of 24 mV at 10 mA cm–2 and a mass activity of 3.89 A Ptmg–1, which is 4.7 times higher than that of commercial Pt/C, at an overpotential of 130 mV for catalyzing the HER. An alkali-electrolyzer using Pt-CoS2/CC as a bifunctional electrode enables a water-splitting current density of 10 mA cm–2 at a low voltage of 1.55 V and can sustain for more than 20 h, which is superior to that of the state-of-the-art Pt/C+RuO2 catalyst. Further experimental and theoretical simulation studies demonstrate that strong electronic interaction between Pt and CoS2 synergistically optimize hydrogen adsorption/desorption behaviors and facilitate the in situ generation of OER active species, enhancing the overall water-splitting performance. This research highlights the regulation of interfacial and electronic synergy in pursuit of highly efficient and durable supported catalysts for hydrogen and oxygen electrocatalytic applications.},
doi = {10.1002/aenm.201800935},
journal = {Advanced Energy Materials},
number = 24,
volume = 8,
place = {United States},
year = {Mon Jul 02 00:00:00 EDT 2018},
month = {Mon Jul 02 00:00:00 EDT 2018}
}
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Ultrafine α‐Phase Molybdenum Carbide Decorated with Platinum Nanoparticles for Efficient Hydrogen Production in Acidic and Alkaline Media
journal, February 2019
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- Advanced Science, Vol. 6, Issue 8
Mesoporous Decoration of Freestanding Palladium Nanotube Arrays Boosts the Electrocatalysis Capabilities toward Formic Acid and Formate Oxidation
journal, May 2019
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- Advanced Energy Materials, Vol. 9, Issue 25
Ni/Fe Codoped In 2 S 3 Nanosheet Arrays Boost Photo‐Electrochemical Performance of Planar Si Photocathodes
journal, August 2019
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- Advanced Energy Materials, Vol. 9, Issue 38
Perowskitoxid‐Elektroden zur leistungsstarken photoelektrochemischen Wasserspaltung
journal, August 2019
- Wang, Wei; Xu, Meigui; Xu, Xiaomin
- Angewandte Chemie, Vol. 132, Issue 1
Tunable Periodically Ordered Mesoporosity in Palladium Membranes Enables Exceptional Enhancement of Intrinsic Electrocatalytic Activity for Formic Acid Oxidation
journal, January 2020
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- Angewandte Chemie, Vol. 132, Issue 13
Perovskite Oxide Based Electrodes for High‐Performance Photoelectrochemical Water Splitting
journal, August 2019
- Wang, Wei; Xu, Meigui; Xu, Xiaomin
- Angewandte Chemie International Edition, Vol. 59, Issue 1
Tuning Interfacial Structures for Better Catalysis of Water Electrolysis
journal, May 2019
- Xiang, Rui; Peng, Lishan; Wei, Zidong
- Chemistry – A European Journal, Vol. 25, Issue 42
Controlled Synthesis of Ni‐Doped MoS 2 Hybrid Electrode for Synergistically Enhanced Water‐Splitting Process
journal, December 2019
- Wang, Ying; Sun, Wenming; Ling, Xiaofei
- Chemistry – A European Journal
Direct Growth of CNTs@CoS x Se 2(1− x ) on Carbon Cloth for Overall Water Splitting
journal, July 2019
- Zhang, Yuanyuan; Qiu, Yunfeng; Ji, Xinyang
- ChemSusChem, Vol. 12, Issue 16
In Situ Fabrication of Heterostructure on Nickel Foam with Tuned Composition for Enhancing Water‐Splitting Performance
journal, October 2018
- Zheng, Xuerong; Zhang, Yiqi; Liu, Hui
- Small, Vol. 14, Issue 50
Nickel@Nitrogen-Doped Carbon@MoS 2 Nanosheets: An Efficient Electrocatalyst for Hydrogen Evolution Reaction
journal, January 2019
- Shah, Sayyar Ali; Shen, Xiaoping; Xie, Minghua
- Small, Vol. 15, Issue 9
Surface and Interface Engineering: Molybdenum Carbide–Based Nanomaterials for Electrochemical Energy Conversion
journal, September 2019
- Ge, Riyue; Huo, Juanjuan; Sun, Mingjie
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NiS‐Decorated ZnO/ZnS Nanorod Heterostructures for Enhanced Photocatalytic Hydrogen Production: Insight into the Role of NiS
journal, April 2020
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- Solar RRL, Vol. 4, Issue 4
A ruthenium(IV) disulfide based non-enzymatic sensor for selective and sensitive amperometric determination of dopamine
journal, June 2019
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- Microchimica Acta, Vol. 186, Issue 7
Engineering borate modified NiFe layer double hydroxide nanoarrays as “hydroxyl ions hungry” electrocatalysts for enhanced oxygen evolution
journal, January 2019
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Enhanced electrocatalytic activity of water oxidation in an alkaline medium via Fe doping in CoS 2 nanosheets
journal, January 2019
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- Chemical Communications, Vol. 55, Issue 17
Controllable synthesis of nickel sulfide nanocatalysts and their phase-dependent performance for overall water splitting
journal, January 2019
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- Nanoscale, Vol. 11, Issue 12
Bifunctional iron disulfide nanoellipsoids for high energy density supercapacitor and electrocatalytic oxygen evolution applications
journal, January 2019
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- Inorganic Chemistry Frontiers, Vol. 6, Issue 3
Nanoscale hetero-interfaces between metals and metal compounds for electrocatalytic applications
journal, January 2019
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- Journal of Materials Chemistry A, Vol. 7, Issue 10
Ultrafine cobalt nitride nanoparticles supported on carbon nanotubes as efficient electrocatalyst for rechargeable zinc–air batteries
journal, January 2019
- Xu, Ruizhi; Luo, Fang; Li, Min
- Chemical Communications, Vol. 55, Issue 89
The chemically reduced CuO–Co 3 O 4 composite as a highly efficient electrocatalyst for oxygen evolution reaction in alkaline media
journal, January 2019
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- Catalysis Science & Technology, Vol. 9, Issue 22
Optimization of the facet structure of cobalt oxide catalysts for enhanced hydrogen evolution reaction
journal, January 2020
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- Catalysis Science & Technology, Vol. 10, Issue 4
Fully reversible lithium storage of tin oxide enabled by self-doping and partial amorphization
journal, January 2019
- Pang, Yuepeng; Wang, Jing; Yang, Junhe
- Nanoscale, Vol. 11, Issue 27
Electrodepositing Pd on NiFe layered double hydroxide for improved water electrolysis
journal, January 2019
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A new metal–organic open framework enabling facile synthesis of carbon encapsulated transition metal phosphide/sulfide nanoparticle electrocatalysts
journal, January 2019
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Nanosheets assembled into nickel sulfide nanospheres with enriched Ni 3+ active sites for efficient water-splitting and zinc–air batteries
journal, January 2019
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Recent advances and challenges in divalent and multivalent metal electrodes for metal–air batteries
journal, January 2019
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Fe nanodot-decorated MoS 2 nanosheets on carbon cloth: an efficient and flexible electrode for ambient ammonia synthesis
journal, January 2019
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- Journal of Materials Chemistry A, Vol. 7, Issue 48
Nature of Carbon Materials Used as Nondoped Electrodes for Oxygen Reduction Reaction and Supercapacitor Applications
journal, January 2019
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- Journal of The Electrochemical Society, Vol. 166, Issue 2
Structure Design and Composition Engineering of Carbon‐Based Nanomaterials for Lithium Energy Storage
journal, March 2020
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Engineering Multimetallic Aerogels for pH‐Universal HER and ORR Electrocatalysis
journal, March 2020
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Anchoring ultrafine PtNi nanoparticles on N-doped graphene for highly efficient hydrogen evolution reaction
journal, January 2019
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- Catalysis Science & Technology, Vol. 9, Issue 18
Advances in the development of power supplies for the Internet of Everything
journal, June 2019
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Tunable Periodically Ordered Mesoporosity in Palladium Membranes Enables Exceptional Enhancement of Intrinsic Electrocatalytic Activity for Formic Acid Oxidation
journal, March 2020
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- Angewandte Chemie International Edition, Vol. 59, Issue 13
Finite-Element Analysis on Percolation Performance of Foam Zinc
journal, September 2018
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- ACS Omega, Vol. 3, Issue 9