Search Menu
DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information
Search Scholarly Publications

Title: Coherent two-dimensional Fourier transform spectroscopy using a 25 Tesla resistive magnet

Abstract

We performed nonlinear optical two-dimensional Fourier transform spectroscopy measurements using an optical resistive high-field magnet on GaAs quantum wells. Magnetic fields up to 25 T can be achieved using the split helix resistive magnet. Two-dimensional spectroscopy measurements based on the coherent four-wave mixing signal require phase stability. Therefore, these measurements are difficult to perform in environments prone to mechanical vibrations. Large resistive magnets use extensive quantities of cooling water, which causes mechanical vibrations, making two-dimensional Fourier transform spectroscopy very challenging. Here, we report on the strategies we used to overcome these challenges and maintain the required phase-stability throughout the measurement. A self-contained portable platform was used to set up the experiments within the time frame provided by a user facility. Furthermore, this platform was floated above the optical table in order to isolate it from vibrations originating from the resistive magnet. Finally, we present two-dimensional Fourier transform spectra obtained from GaAs quantum wells at magnetic fields up to 25 T and demonstrate the utility of this technique in providing important details, which are obscured in one dimensional spectroscopy.

Authors:
 [1];  [1]; ORCiD logo [2];  [1];  [1];  [3]; ORCiD logo [3]; ORCiD logo [4];  [5]; ORCiD logo [1]
+ Show Author Affiliations
  1. Univ. of South Florida, Tampa, FL (United States)
  2. California State Univ., East Bay, Hayward, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  3. Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Lab. (MagLab)
  4. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  5. Univ. of Alabama, Birmingham, AL (United States)
Publication Date:
Research Org.:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1633234
Alternate Identifier(s):
OSTI ID: 1524466
Grant/Contract Number:  
AC02-05CH11231; AC0205CH11231; SC0012635
Resource Type:
Accepted Manuscript
Journal Name:
Review of Scientific Instruments
Additional Journal Information:
Journal Volume: 90; Journal Issue: 6; Journal ID: ISSN 0034-6748
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION

Citation Formats

Paul, Jagannath, Stevens, Christopher. E., Smith, Ryan P., Dey, Prasenjit, Mapara, Varun, Semenov, Dimitry, McGill, Steven A., Kaindl, Robert A., Hilton, David J., and Karaiskaj, Denis. Coherent two-dimensional Fourier transform spectroscopy using a 25 Tesla resistive magnet. United States: N. p., 2019. Web. doi:10.1063/1.5055891.
Copy to clipboard
Paul, Jagannath, Stevens, Christopher. E., Smith, Ryan P., Dey, Prasenjit, Mapara, Varun, Semenov, Dimitry, McGill, Steven A., Kaindl, Robert A., Hilton, David J., & Karaiskaj, Denis. Coherent two-dimensional Fourier transform spectroscopy using a 25 Tesla resistive magnet. United States. https://doi.org/10.1063/1.5055891
Copy to clipboard
Paul, Jagannath, Stevens, Christopher. E., Smith, Ryan P., Dey, Prasenjit, Mapara, Varun, Semenov, Dimitry, McGill, Steven A., Kaindl, Robert A., Hilton, David J., and Karaiskaj, Denis. Tue . "Coherent two-dimensional Fourier transform spectroscopy using a 25 Tesla resistive magnet". United States. https://doi.org/10.1063/1.5055891. https://www.osti.gov/servlets/purl/1633234.
Copy to clipboard
@article{osti_1633234,
title = {Coherent two-dimensional Fourier transform spectroscopy using a 25 Tesla resistive magnet},
author = {Paul, Jagannath and Stevens, Christopher. E. and Smith, Ryan P. and Dey, Prasenjit and Mapara, Varun and Semenov, Dimitry and McGill, Steven A. and Kaindl, Robert A. and Hilton, David J. and Karaiskaj, Denis},
abstractNote = {We performed nonlinear optical two-dimensional Fourier transform spectroscopy measurements using an optical resistive high-field magnet on GaAs quantum wells. Magnetic fields up to 25 T can be achieved using the split helix resistive magnet. Two-dimensional spectroscopy measurements based on the coherent four-wave mixing signal require phase stability. Therefore, these measurements are difficult to perform in environments prone to mechanical vibrations. Large resistive magnets use extensive quantities of cooling water, which causes mechanical vibrations, making two-dimensional Fourier transform spectroscopy very challenging. Here, we report on the strategies we used to overcome these challenges and maintain the required phase-stability throughout the measurement. A self-contained portable platform was used to set up the experiments within the time frame provided by a user facility. Furthermore, this platform was floated above the optical table in order to isolate it from vibrations originating from the resistive magnet. Finally, we present two-dimensional Fourier transform spectra obtained from GaAs quantum wells at magnetic fields up to 25 T and demonstrate the utility of this technique in providing important details, which are obscured in one dimensional spectroscopy.},
doi = {10.1063/1.5055891},
journal = {Review of Scientific Instruments},
number = 6,
volume = 90,
place = {United States},
year = {Tue Jun 04 00:00:00 EDT 2019},
month = {Tue Jun 04 00:00:00 EDT 2019}
}
Copy to clipboard
Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1063/1.5055891
Copyright Statement
Other availability
Search WorldCat Search WorldCat to find libraries that may hold this journal
Citation Metrics:
Cited by: 1 work
Citation information provided by
Web of Science

Figures / Tables:

FIG. 1 FIG. 1: Schematic of the experimental setup: The three laser beams are provided by the multidimensional optical nonlinear spectrometer (MONSTR). Three beams labeled as A∗, B, and C, where A∗ corresponds to the phase conjugate beam, are separated by the time delays τ and T, and are used to generatemore » the FWM signal. The beams are aligned in the three corners of a square. The FWM signal generated at the sample propagates along the missing corner (direction −$\vec{k}_a$ + $\vec{k_b}$ + $\vec{k_c}$) of the square and is heterodyne detected using the reference beam (Ref.). The combined FWM and Ref. beam is dispersed into a grating spectrometer and the resulting spectral interferogram is Fourier transformed leading to a two-dimensional spectrum. The samples are kept at 10 Kelvin inside the bore of the resistive 25 T split helix magnet. The magnetic fields up to 25 Tesla are applied perpendicular to the sample surface in Faraday geometry, facilitated by the sample mount.« less
All figures and tables (4 total)
Save / Share:
Export Metadata
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.

Works referenced in this record:

Coherently wired light-harvesting in photosynthetic marine algae at ambient temperature
journal, February 2010

  • Collini, Elisabetta; Wong, Cathy Y.; Wilk, Krystyna E.
  • Nature, Vol. 463, Issue 7281
  • DOI: 10.1038/nature08811

Quantum-beat spectroscopy of the Zeeman splitting of heavy- and light-hole excitons in GaAs/ Al x Ga 1 − x As quantum wells
journal, July 1993

A versatile ultrastable platform for optical multidimensional Fourier-transform spectroscopy
journal, July 2009

  • Bristow, A. D.; Karaiskaj, D.; Dai, X.
  • Review of Scientific Instruments, Vol. 80, Issue 7
  • DOI: 10.1063/1.3184103

Theory of excitons in cubic semiconductors in arbitrary magnetic fields: Application to GaAs
journal, July 1980

Fiber-coupled antennas for ultrafast coherent terahertz spectroscopy in low temperatures and high magnetic fields
journal, September 2002

  • Crooker, S. A.
  • Review of Scientific Instruments, Vol. 73, Issue 9
  • DOI: 10.1063/1.1498904

Ultrafast Spectroscopy of Semiconductors and Semiconductor Nanostructures
book, January 1999

Coulomb-interaction induced coupling of Landau levels in intrinsic and modulation-doped quantum wells
journal, June 2017

Electronic Dephasing in the Quantum Hall Regime
text, January 1999

  • Fromer, N. A.; Schüller, Christian; Chemla, D. S.
  • Universität Regensburg
  • DOI: 10.5283/epub.9498

Continuously tunable optical multidimensional Fourier-transform spectrometer
journal, February 2013

  • Dey, P.; Paul, J.; Bylsma, J.
  • Review of Scientific Instruments, Vol. 84, Issue 2
  • DOI: 10.1063/1.4792378

Vibronic coherence in oxygenic photosynthesis
journal, July 2014

  • Fuller, Franklin D.; Pan, Jie; Gelzinis, Andrius
  • Nature Chemistry, Vol. 6, Issue 8
  • DOI: 10.1038/nchem.2005

Magnetoexcitons in a narrow single GaAs- Ga 0.5 Al 0.5 As quantum well grown by molecular-beam epitaxy
journal, March 1988

Electronic resonance with anticorrelated pigment vibrations drives photosynthetic energy transfer outside the adiabatic framework
journal, December 2012

  • Tiwari, Vivek; Peters, William K.; Jonas, David M.
  • Proceedings of the National Academy of Sciences, Vol. 110, Issue 4
  • DOI: 10.1073/pnas.1211157110

Valley- and spin-polarized Landau levels in monolayer WSe2
journal, October 2016

Direct measurement of exciton valley coherence in monolayer WSe2
journal, February 2016

  • Hao, Kai; Moody, Galan; Wu, Fengcheng
  • Nature Physics, Vol. 12, Issue 7
  • DOI: 10.1038/nphys3674

Magneto-optical Investigation of the Free-Exciton Reflectance from High-Purity Epitaxial GaAs
journal, November 1973

Evidence for wavelike energy transfer through quantum coherence in photosynthetic systems
journal, April 2007

  • Engel, Gregory S.; Calhoun, Tessa R.; Read, Elizabeth L.
  • Nature, Vol. 446, Issue 7137
  • DOI: 10.1038/nature05678

Coherent multi-dimensional spectroscopy: Experimental considerations, direct comparisons and new capabilities
journal, September 2017

Concepts and Methods of 2D Infrared Spectroscopy
book, January 2011

2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line
journal, January 2014

  • Réhault, Julien; Maiuri, Margherita; Manzoni, Cristian
  • Optics Express, Vol. 22, Issue 8
  • DOI: 10.1364/oe.22.009063

Two-Quantum 2D FT Electronic Spectroscopy of Biexcitons in GaAs Quantum Wells
journal, May 2009

Fourier transform spectroscopy in the vibrational fingerprint region with a birefringent interferometer
text, January 2017

  • Réhault, J.; Borrego-Varillas, R.; Oriana, A.
  • Optical Society of America
  • DOI: 10.5167/uzh-157853

2D IR spectroscopy with phase-locked pulse pairs from a birefringent delay line
text, January 2014

  • Réhault, Julien; Maiuri, Margherita; Manzoni, Cristian
  • Optical Society of America
  • DOI: 10.5167/uzh-157851

Digital gamma-ray spectroscopy based on FPGA technology
journal, April 2002

  • Bolić, Miodrag; Drndarević, Vujo
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 482, Issue 3
  • DOI: 10.1016/s0168-9002(01)01925-8

Structure of the Amide I Band of Peptides Measured by Femtosecond Nonlinear-Infrared Spectroscopy
journal, July 1998

  • Hamm, Peter; Lim, Manho; Hochstrasser, Robin M.
  • The Journal of Physical Chemistry B, Vol. 102, Issue 31
  • DOI: 10.1021/jp9813286

Two-dimensional electronic spectroscopy with birefringent wedges
journal, December 2014

  • Réhault, Julien; Maiuri, Margherita; Oriana, Aurelio
  • Review of Scientific Instruments, Vol. 85, Issue 12
  • DOI: 10.1063/1.4902938

Two-dimensional infrared spectroscopy of peptides by phase-controlled femtosecond vibrational photon echoes
journal, July 2000

  • Asplund, M. C.; Zanni, M. T.; Hochstrasser, R. M.
  • Proceedings of the National Academy of Sciences, Vol. 97, Issue 15
  • DOI: 10.1073/pnas.140227997

Physics of strain effects in semiconductors and metal-oxide-semiconductor field-effect transistors
journal, May 2007

  • Sun, Y.; Thompson, S. E.; Nishida, T.
  • Journal of Applied Physics, Vol. 101, Issue 10
  • DOI: 10.1063/1.2730561

Active phase stabilization in Fourier-transform two-dimensional infrared spectroscopy
journal, January 2005

  • Volkov, Victor; Schanz, Roland; Hamm, Peter
  • Optics Letters, Vol. 30, Issue 15
  • DOI: 10.1364/ol.30.002010

Magneto-reflectance of the 1S exciton ground states in InP and GaAs
journal, April 1974

Neutral and charged inter-valley biexcitons in monolayer MoSe2
journal, June 2017

  • Hao, Kai; Specht, Judith F.; Nagler, Philipp
  • Nature Communications, Vol. 8, Issue 1
  • DOI: 10.1038/ncomms15552

Advances in multi-dimensional coherent spectroscopy of semiconductor nanostructures
journal, May 2017

Exciton states of semiconductors in a high magnetic field
journal, February 1974

Vibrational and electronic dynamics of nitrogen–vacancy centres in diamond revealed by two-dimensional ultrafast spectroscopy
journal, September 2013

  • Huxter, V. M.; Oliver, T. A. A.; Budker, D.
  • Nature Physics, Vol. 9, Issue 11
  • DOI: 10.1038/nphys2753

High electron mobility, quantum Hall effect and anomalous optical response in atomically thin InSe
journal, November 2016

  • Bandurin, Denis A.; Tyurnina, Anastasia V.; Yu, Geliang L.
  • Nature Nanotechnology, Vol. 12, Issue 3
  • DOI: 10.1038/nnano.2016.242

Many-body and correlation effects in semiconductors
journal, May 2001

  • Chemla, D. S.; Shah, Jagdeep
  • Nature, Vol. 411, Issue 6837
  • DOI: 10.1038/35079000

Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields
journal, September 2018

Development of FPGA-based digital signal processing system for radiation spectroscopy
journal, January 2013

Coherent Two-Dimensional Optical Spectroscopy
journal, April 2008

Coherent Spectroscopy of Semiconductors
conference, January 2016

Femtosecond spectroscopy of carrier-spin relaxation in GaAs- Al x Ga 1 − x As quantum wells
journal, September 1991

Two-dimensional spectroscopy using diffractive optics based phased-locked photon echoes
journal, March 2004

T WO -D IMENSIONAL F EMTOSECOND S PECTROSCOPY
journal, October 2003

Exciton, heavy-hole, and electron g factors in type-I GaAs/ Al x Ga 1 − x As quantum wells
journal, February 1992

Intrinsic homogeneous linewidth and broadening mechanisms of excitons in monolayer transition metal dichalcogenides
journal, September 2015

  • Moody, Galan; Kavir Dass, Chandriker; Hao, Kai
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms9315

An FPGA-based module for multiphoton coincidence counting
conference, May 2012

  • Branning, David; Beck, Mark
  • SPIE Defense, Security, and Sensing, SPIE Proceedings
  • DOI: 10.1117/12.919495

Sensitivity of 2D IR Spectra to Peptide Helicity: A Concerted Experimental and Simulation Study of an Octapeptide
journal, September 2009

  • Sengupta, Neelanjana; Maekawa, Hiroaki; Zhuang, Wei
  • The Journal of Physical Chemistry B, Vol. 113, Issue 35
  • DOI: 10.1021/jp901504r

The Design of Powerful Electromagnets Part IV. The New Magnet Laboratory at M. I. T.
journal, December 1939

  • Bitter, F.
  • Review of Scientific Instruments, Vol. 10, Issue 12
  • DOI: 10.1063/1.1751470

Coherent measurements of high-order electronic correlations in quantum wells
journal, August 2010

Coulomb correlations in a two-dimensional electron gas in large magnetic fields
text, January 2002

  • Former, N. A.; Schüller, Christian; Lai, W. C.
  • Universität Regensburg
  • DOI: 10.5283/epub.9567

Perturbation-Theory Investigation of the Exciton Ground State of Cubic Semiconductors in a Magnetic Field
journal, April 1973

Transient Linear Birefringence in GaAs Quantum Wells: Magnetic Field Dependence of Coherent Exciton Spin Dynamics
journal, April 1996

Two-dimensional spectroscopy of electronic couplings in photosynthesis
journal, March 2005

  • Brixner, Tobias; Stenger, Jens; Vaswani, Harsha M.
  • Nature, Vol. 434, Issue 7033
  • DOI: 10.1038/nature03429

Broadband ultrafast terahertz spectroscopy in the 25 T Split Florida-Helix
journal, July 2018

  • Curtis, Jeremy A.; Burch, Ashlyn D.; Barman, Biplob
  • Review of Scientific Instruments, Vol. 89, Issue 7
  • DOI: 10.1063/1.5023384

Coherent 2D IR Spectroscopy:  Molecular Structure and Dynamics in Solution
journal, July 2003

  • Khalil, M.; Demirdöven, N.; Tokmakoff, A.
  • The Journal of Physical Chemistry A, Vol. 107, Issue 27
  • DOI: 10.1021/jp0219247

Phase-locked pulses for two-dimensional spectroscopy by a birefringent delay line
conference, May 2013

  • Manzoni, Cristian; Brida, Daniele; Cerullo, Giulio
  • 2013 Conference on Lasers & Electro-Optics Europe & International Quantum Electronics Conference CLEO EUROPE/IQEC
  • DOI: 10.1109/cleoe-iqec.2013.6801061

Inherently phase-stable coherent two-dimensional spectroscopy using only conventional optics
journal, January 2008

  • Selig, Ulrike; Langhojer, Florian; Dimler, Frank
  • Optics Letters, Vol. 33, Issue 23
  • DOI: 10.1364/ol.33.002851

Absorption quantum beats of magnetoexcitons in GaAs heterostructures
journal, May 1991

Fourier transform spectroscopy in the vibrational fingerprint region with a birefringent interferometer
journal, January 2017

  • Réhault, J.; Borrego-Varillas, R.; Oriana, A.
  • Optics Express, Vol. 25, Issue 4
  • DOI: 10.1364/oe.25.004403

Transitions of epitaxially lifted-off bulk GaAs and GaAs/AlGaAs quantum well under thermal-induced compressive and tensile strain
journal, November 2008

  • Mateo, C. M. N.; Ibañez, J. J.; Fernando, J. G.
  • Journal of Applied Physics, Vol. 104, Issue 10
  • DOI: 10.1063/1.3006437

Perturbation-Theory Investigation of the Exciton Ground State of Cubic Semiconductors in a Magnetic Field
journal, October 1973

Conformations of N -Acetyl- l -Prolinamide by Two-Dimensional Infrared Spectroscopy †
journal, October 2006

  • Sul, Soohwan; Karaiskaj, Denis; Jiang, Ying
  • The Journal of Physical Chemistry B, Vol. 110, Issue 40
  • DOI: 10.1021/jp062039h

Biexciton formation and exciton coherent coupling in layered GaSe
journal, April 2015

  • Dey, P.; Paul, J.; Moody, G.
  • The Journal of Chemical Physics, Vol. 142, Issue 21
  • DOI: 10.1063/1.4917169

Electronic coherence lineshapes reveal hidden excitonic correlations in photosynthetic light harvesting
journal, March 2012

  • Wong, Cathy Y.; Alvey, Richard M.; Turner, Daniel B.
  • Nature Chemistry, Vol. 4, Issue 5
  • DOI: 10.1038/nchem.1302

M ULTIDIMENSIONAL F EMTOSECOND C ORRELATION S PECTROSCOPIES OF E LECTRONIC AND V IBRATIONAL E XCITATIONS
journal, October 2000

Theory of degenerate 1 s excitons in zinc-blende-type crystals in a magnetic field: Exchange interaction and cubic anisotropy
journal, February 1975

Strain-induced splitting of the valence band in epitaxially lifted-off GaAs films
journal, April 2007

  • Mateo, Cherry May N.; Garcia, Alipio T.; Ramos, Flo Rykiel M.
  • Journal of Applied Physics, Vol. 101, Issue 7
  • DOI: 10.1063/1.2716869

Observation of Multiple Magnetorotons in the Fractional Quantum Hall Effect
text, January 2001

  • Dennis, B. S.; Kang, Moonsoo; Pfeiffer, L. N.
  • The American Physical Society
  • DOI: 10.17877/de290r-8538

Coherent Spectroscopy of Semiconductors
conference, January 2016

Observation of inter-Landau-level quantum coherence in semiconductor quantum wells
text, January 2008

Evidence for a Bilayer Quantum Wigner Solid
text, January 1996

    Sort by:
    [ × clear filter / sort ]

    Figures / Tables found in this record:

    FIG. 1 (p. 3)figure
    FIG. 2 (p. 4)figure
    FIG. 3 (p. 5)figure
    FIG. 4 (p. 6)figure
      [ × clear filter / sort ]
      Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.

      Similar Records in DOE PAGES and OSTI.GOV collections: